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Understanding the fate of Arctic atmospheric mercury (Hg) deposition – A Hg stable isotope investigation of redox processes and Hg re-emissions

Objective

Mercury (Hg) is a pollutant of global concern for human and ecosystem health. This is particularly true in the Arctic where indigenous populations are excessively exposed to dietary Hg from fish and marine mammal consumption. The deposition of Hg from the atmosphere to Earth surfaces and its re-emission via biogeochemical reduction processes determine Hg concentrations in Earth surface reservoirs, such as soils, snow, and runoff into Arctic lakes and surface Ocean. In order to predict the impact of anthropogenic Hg emissions on net atmospheric Hg deposition and ultimately Hg concentrations in biota, it is important to understand these deposition and re-emission processes. The reduction of deposited Hg2+ to volatile gaseous Hg0 and the oxidation of gaseous Hg0 to reactive Hg2+, which is rapidly deposited from the atmosphere, control the global fate of Hg. Major knowledge gaps concerning the mechanisms of these redox processes exist.
Different photochemical and non-photochemical Hg2+ reduction mechanisms were found to fractionate Hg stable isotopes in distinct, identifiable ways. Also, different atmospheric Hg0 and Hg2+ pools have been shown to have distinguishable Hg isotope signatures. Hg isotopes can thus provide new insights in the sources of Hg and redox transformation processes at the Earth-atmosphere interface, which are inaccessible by means of concentration and flux measurements alone. In the MEROXRE project proposed here we will combine the latest innovations in gaseous Hg measurements in porous media (soils, snow) with state-of-the-art Hg isotope techniques to investigate:
(i) Hg isotope fractionation of Hg2+ reduction and gaseous Hg0 oxidation in interstitial snow air and soil pores.
(ii) Hg isotope fractionation factors associated with net gaseous Hg0 re-emission fluxes from soil and snow
(iii) the importance of gaseous Hg0 oxidation and Hg2+ reduction and re-emission for the global Hg cycle by incorporating the results in a global Hg isotope model.

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Keywords

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Topic(s)

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Funding Scheme

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MSCA-IF - Marie Skłodowska-Curie Individual Fellowships (IF)

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Call for proposal

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(opens in new window) H2020-MSCA-IF-2014

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Coordinator

CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 173 076,00
Address
RUE MICHEL ANGE 3
75794 Paris
France

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Region
Ile-de-France Ile-de-France Hauts-de-Seine
Activity type
Research Organisations
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 173 076,00
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