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Unravelling the Nature of Green Organic “On-Water” Catalysis via Novel Quantum Chemical Methods

Project description

Novel quantum chemical methods for green organic 'on-water' catalysis

The ERC-funded GreenOnWaterCat project aims to revolutionise the understanding of green ‘on-water’ catalysis and to unravel its microscopic origin. To this end, several novel theoretical methods will be developed and implemented, enabling unprecedented large-scale quantum molecular dynamics simulations. The project has three additional objectives: to elucidate the experimental measurements and characterise the corresponding atomic structure; to propose novel synthetic processes that exploit the on-water concept, such as catalysis at the organic/metal oxide interface; and to investigate the possibility of on-water catalysis using two water-insoluble solid reactants. The expected results will help render water a very attractive solvent in the design of novel synthetic processes and even more useful for industrial applications.

Objective

The target of the research program, GreenOnWaterCat, is to revolutionize the understanding of green “on-water” catalysis and to unravel its microscopic origin. To enable these goals to be reached, several novel theoretical methods will be developed and implemented that will enable for unprecedented large-scale quantum molecular dynamics simulations, where both the electronic and nuclear Schrödinger equations are solved simultaneously. In addition, these methods will also allow the efficient computation of various state-of-the-art vibrational spectroscopies “on-the-fly”, at essentially no additional computational cost. Furthermore, new analysis techniques permit to assign the spectra and explain their correlation with the atomic structure in order to gain invaluable insights and eventually grasp the relationships between the dynamics and structure of “on-water” catalysis and vibrational spectroscopies. Since the latter offers a convenient connection to experiment, the unique results are of utmost value in order to explain the experimental findings. In consequence, new synthetic processes based on the “on-water” phenomenon will be proposed and investigated. The expected results will be most helpful so that water will soon become not only a viable, but also very attractive solvent in the design of novel synthetic processes and to make it even more useful for industrial applications.
Beside the development and implementation of novel computational methods, which will be made publicly available, the additional outcomes expected are as follows:

• To conclusively explain the underlying mechanism of the “on-water” rate phenomenon for the first time
• To elucidate the experimental measurements and characterize the corresponding atomic structure
• To propose novel synthetic processes which exploit the “on-water” concept, such as catalysis at the organic/metal oxide interface
• To investigate the possibility of “on-water” catalysis using two water-insoluble solid reactants

Fields of science (EuroSciVoc)

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Programme(s)

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Topic(s)

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Funding Scheme

Funding scheme (or “Type of Action”) inside a programme with common features. It specifies: the scope of what is funded; the reimbursement rate; specific evaluation criteria to qualify for funding; and the use of simplified forms of costs like lump sums.

ERC-STG - Starting Grant

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Call for proposal

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(opens in new window) ERC-2016-STG

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Host institution

UNIVERSITAET PADERBORN
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 1 499 875,00
Address
WARBURGER STRASSE 100
33098 Paderborn
Germany

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Region
Nordrhein-Westfalen Detmold Paderborn
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 1 499 875,00

Beneficiaries (1)

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