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Abstract

During LBA-CLAIRE-98, we found atmospheric layers with aged biomass smoke at altitudes>10 km over Suriname, CO, C02, acetonitrile, methyl chloride, hydrocarbons, NO, O(3), and aerosols were strongly enhanced in these layers. We estimate that 80-95% of accumulation mode aerosols had been removed during convective transport. Trajectories show that the plumes originated from large fires near the BraziI/Venezuela border during March 1998. This smoke was entrained into deep convection over the northern Amazon, transported out over the Pacific, and then returned to South America by the circulation around a large upper-level anticyclone. Our observations provide evidence for the importance of deep convection in the equatorial region as a mechanism to transport large amounts of pyrogenic pollutants into the upper troposphere. The entrainment of biomass smoke into tropical convective clouds may have significant effects on cloud micro-physics and climate dynamics.

Additional information

Authors: ANDREAE M.O, Max Planck Institute for Chemistry ,Mainz (DE);FISCHER H, Max Planck Institute for Chemistry ,Mainz (DE);HOOR P, Max Planck Institute for Chemistry ,Mainz (DE);KORMANN R, Max Planck Institute for Chemistry ,Mainz (DE);LANGE L, Max Planck Institute for Chemistry ,Mainz (DE);WILLIAMS J, Max Planck Institute for Chemistry ,Mainz (DE);ARTAXO P, Instituto de Fisica, Universidade de Sao Paulo (BR);LONGO K, Instituto de Fisica, Universidade de Sao Paulo (BR);GRGOIRE J.M, Environment Institute, JRC/CEC, Ispra (IT);HANSEL A, Institute of Ion Physics, Innbruck University (AT);LINDINGER W, Institute of Ion Physics, Innbruck University (AT);KREJCI R, Inst. Applied Environm. Research, Stockholm University (SE);STRÍM J, Inst. Applied Environm. Research, Stockholm University (SE);LELIEVELD J, Inst. For Marine and Atmospheric Reasearch, Utrecht (NL);PETERS W, Inst. For Marine and Atmospheric Reasearch, Utrecht (NL);DE REUS MSCHEEREN B, Inst. For Marine and Atmospheric Reasearch, Utrecht (NL);FREITAS S.R, Dept. Ciencias Atmosfericas, Universidade de Sao Paulo (BR);SILVA DIAS M.A.F, Dept. Ciencias Atmosfericas, Universidade de Sao Paulo (BR);VAN VELTHOVEN P.F.J, Royal Netherlands Meteorological Institute, De Bilt (NL);STRIM J, Inst. Applied Environm. Research, Stockholm University (SE)
Bibliographic Reference: An article published in: Geophysical Research Letters. Vol.28 No.6. (2001) pp.951-954
Record Number: 200013394 / Last updated on: 2001-06-27
Category: PUBLICATION
Original language: en
Available languages: en