Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses

Livrables

Attosecond dynamics in small and large molecules

Pump-probe experiment with femtosecond and attosecond time resolution on large molecules will be conducted. The experimental results will be compared with theoretical models, focusing on the kinetic energy release obtained in attosecond XUV-IR pump-probe spectroscopy. The dominant ionization and dissociative pathways will be theoretically identified.

Nonadiabatic strong-field ionization dynamics

Nonadiabatic effects in the strong-field ionization of hydrocarbons molecules will be investigated using HHG.

Supervisory Board of the network

The Supervisory Board of the network will meet for the first time during the kickoff meeting JanuaryFebruary 2015 The Supervisory Board will be composed by the will be composed of the scientistsincharge of the beneficiaries and partner organizations the WP Coordinators Prof Nora Berrah and a representative of the ESRs elected by the young fellows The SB will agree on common guidelines regarding the individual training of the fellows and it will provide the guidelines for the drafting of the CDPs of the individual ESRsDuring this first meeting a training for unbiased selection and dissemination of common best practises to supervisors will be provided kickoff meeting

Structural and dynamical effects in HHG

The interplay between structural and dynamical effects in high-order harmonic generation (HHG) spectroscopy will be elucidated. Advanced alignment techniques will be investigated for the implementation of high-order HHG-based tomography of nonplanar molecules. From the theoretical side, a simulation code for HHG-based spectroscopy of multi-electron dynamics will be developed, considering also the extended harmonic cut-off achieved using mid-IR systems as driving pulses.

High-repetition rate photoelectron spectroscopy

Acquisition of photoelectron/photoion pump-probe data with full energy, angular and temporal resolution using the developed high repetition rate (200 kHz) attosecond source . The network will be involved in the development of new apparatuses and technologies for the generation of ultrashort XUV pulses including novel schemes for the stabilisation of the CEP of high-energy, high-repetition rate laser systems operating up to 10 kHz, the demonstration of thin-disk laser pump delivering up to E=200 mJ energy.

Dissemination and outreach activities plan

A plan for the outreach activities of the ESRs will be drafted This will be based on the activities to be performed in secondary schools using the Photonics Explorer Kit Additional outreach activities for example the participation to specific event such as the Researchers night will be also considered

Time-resolved dynamics in conformer selected beams

Conformer selection will be accomplished and time-resolved dynamics in different conformers will be characterized by pump-probe experiment with attosecond and femtosecond resolution.

Influence of the environment on ultrafast eletronic/nuclear dynamics

1) Experimental evidences of electronic relaxation mechanism (for example Interatomic Coulombic Decay) induced by intense XUV light pulses in atomic clusters/dimers will be obtained. 2) The influence of the helium environment on the rotational, vibrational and electronic dynamics of embedded molecules will be characterized

Demonstration of coherent control schemes using XUV FELs

The consortium will demonstrate new schemes for the generation of multi-color coherent XUV radiation exploiting FELs. Using this approach, the network will investigated coherent control schemes in the XUV spectral range. In particular, the combination of multi-color coherent XUV radiation will be used to control the photoionization process and electronic dynamics in inner-valence shells in atoms and, eventually also in molecules. Finally we will also investigate novel approaches for the generation of attosecond pulse trains using XUV FELs.

Improved HHG tomography of linear molecules

HHG tomography strongly depends on the quality of alignment of molecules in cold gas jets. We will investigate strategies for a reliable reconstruction of molecular orbitals by HHG in simple linear molecules, even in presence of degraded alignment conditions.

Attosecond XUV-pump-XUV-probe on molecules

The ultrafast autoionization dynamics of small molecules such as H2/D2 (hydrogen and deuterium) will be characterized exploiting high-energy low repetition rate laser systems.

Dynamical structure by HHG

Dynamical structure information in simple molecules using XUV light generated by HHG will be obtained

Website design and development, and Social Media presence

The Webpage of the network will be designed during the first four months The webpage will be used to advertise the network activities the open positions until the recruitment of all ESRs and to disseminate the videoclips virtual lab tours and video tutorials and to communicate the list of speakers of the webinars At the same time the LinkedIn group of the network will be created and maintained

Publications

Coherent diffractive imaging of single helium nanodroplets with a high harmonic generation source

Auteurs: Daniela Rupp, Nils Monserud, Bruno Langbehn, Mario Sauppe, Julian Zimmermann, Yevheniy Ovcharenko, Thomas Möller, Fabio Frassetto, Luca Poletto, Andrea Trabattoni, Francesca Calegari, Mauro Nisoli, Katharina Sander, Christian Peltz, Marc J. Vrakking, Thomas Fennel, Arnaud Rouzée
Publié dans: Nature Communications, Numéro 8/1, 2017, Page(s) Article number: 493, ISSN 2041-1723
Éditeur: Nature Publishing Group
DOI: 10.1038/s41467-017-00287-z

Original Ti:Sa 10 kHz front-end design delivering 17 fs, 170 mrad CEP stabilized pulses up to 5 W

Auteurs: A. Golinelli, X. Chen, E. Gontier, B. Bussière, O. Tcherbakoff, M. Natile, P. d’Oliveira, P.-M. Paul, J.-F. Hergott
Publié dans: Optics Letters, Numéro 42/12, 2017, Page(s) 2326, ISSN 0146-9592
Éditeur: Optical Society of America
DOI: 10.1364/OL.42.002326

Coulomb-explosion imaging of concurrent CH 2 BrI photodissociation dynamics

Auteurs: Michael Burt, Rebecca Boll, Jason W. L. Lee, Kasra Amini, Hansjochen Köckert, Claire Vallance, Alexander S. Gentleman, Stuart R. Mackenzie, Sadia Bari, Cédric Bomme, Stefan Düsterer, Benjamin Erk, Bastian Manschwetus, Erland Müller, Dimitrios Rompotis, Evgeny Savelyev, Nora Schirmel, Simone Techert, Rolf Treusch, Jochen Küpper, Sebastian Trippel, Joss Wiese, Henrik Stapelfeldt, Barbara Cunha
Publié dans: Physical Review A, Numéro 96/4, 2017, ISSN 2469-9926
Éditeur: PHYSICAL REVIEW A
DOI: 10.1103/PhysRevA.96.043415

Optical Parametric Amplification Techniques for the Generation of High-Energy Few-Optical-Cycles IR Pulses for Strong Field Applications

Auteurs: Anna Ciriolo, Matteo Negro, Michele Devetta, Eugenio Cinquanta, Davide Faccialà, Aditya Pusala, Sandro De Silvestri, Salvatore Stagira, Caterina Vozzi
Publié dans: Applied Sciences, Numéro 7/3, 2017, Page(s) 265, ISSN 2076-3417
Éditeur: Applied Sciences
DOI: 10.3390/app7030265

Micro-focusing of broadband high-order harmonic radiation by a double toroidal mirror

Auteurs: Coudert-Alteirac, Hélène; Dacasa, Hugo; Campi, Filippo; Kueny, Emma; Farkas, Balázs; Brunner, Fabian; Maclot, Sylvain; Manschwetus, Bastian; Wikmark, Hampus; Lahl, Jan; Rading, Linnea; Peschel, Jasper; Major, Balázs; Varjú, Katalin; Dovillaire, Guillaume; Zeitoun, Philippe; Johnsson, Per; L'Huillier, Anne; Rudawski, Piotr
Publié dans: Applied Sciences, Numéro 7/11, 1159, 2018, ISSN 2076-3417
Éditeur: Applied Sciences
DOI: 10.3204/PUBDB-2017-11919

A Versatile Velocity Map Ion-Electron Covariance Imaging Spectrometer for High-Intensity XUV Experiments

Auteurs: Linnea Rading, Jan Lahl, Sylvain Maclot, Filippo Campi, Hélène Coudert-Alteirac, Bart Oostenrijk, Jasper Peschel, Hampus Wikmark, Piotr Rudawski, Mathieu Gisselbrecht, Per Johnsson
Publié dans: Applied Sciences, Numéro 8/6, 2018, Page(s) 998, ISSN 2076-3417
Éditeur: Applied Sciences
DOI: 10.3390/app8060998

Photoexcitation circular dichroism in chiral molecules

Auteurs: S. Beaulieu, A. Comby, D. Descamps, B. Fabre, G. A. Garcia, R. Géneaux, A. G. Harvey, F. Légaré, Z. Mašín, L. Nahon, A. F. Ordonez, S. Petit, B. Pons, Y. Mairesse, O. Smirnova, V. Blanchet
Publié dans: Nature Physics, Numéro 14/5, 2018, Page(s) 484-489, ISSN 1745-2473
Éditeur: Nature Publishing Group
DOI: 10.1038/s41567-017-0038-z

Monte Carlo wave-packet approach to trace nuclear dynamics in molecular excited states by XUV-pump–IR-probe spectroscopy

Auteurs: Qingli Jing, Roger Y. Bello, Fernando Martín, Alicia Palacios, Lars Bojer Madsen
Publié dans: Physical Review A, Numéro 97/4, 2018, ISSN 2469-9926
Éditeur: PHYSICAL REVIEW A
DOI: 10.1103/PhysRevA.97.043426

Spatial Control of Multiphoton Electron Excitations in InAs Nanowires by Varying Crystal Phase and Light Polarization

Auteurs: Erik Mårsell, Emil Boström, Anne Harth, Arthur Losquin, Chen Guo, Yu-Chen Cheng, Eleonora Lorek, Sebastian Lehmann, Gustav Nylund, Martin Stankovski, Cord L. Arnold, Miguel Miranda, Kimberly A. Dick, Johan Mauritsson, Claudio Verdozzi, Anne L’Huillier, Anders Mikkelsen
Publié dans: Nano Letters, Numéro 18/2, 2018, Page(s) 907-915, ISSN 1530-6984
Éditeur: American Chemical Society
DOI: 10.1021/acs.nanolett.7b04267

Phase control of attosecond pulses in a train

Auteurs: Chen Guo, Anne Harth, Stefanos Carlström, Yu-Chen Cheng, Sara Mikaelsson, Erik Mårsell, Christoph Heyl, Miguel Miranda, Mathieu Gisselbrecht, Mette B Gaarde, Kenneth J Schafer, Anders Mikkelsen, Johan Mauritsson, Cord L Arnold, Anne L’Huillier
Publié dans: Journal of Physics B: Atomic, Molecular and Optical Physics, Numéro 51/3, 2018, Page(s) 034006, ISSN 0953-4075
Éditeur: Institute of Physics Publishing
DOI: 10.1088/1361-6455/aa9953

Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom

Auteurs: Felix Brauße, Gildas Goldsztejn, Kasra Amini, Rebecca Boll, Sadia Bari, Cédric Bomme, Mark Brouard, Michael Burt, Barbara Cunha de Miranda, Stefan Düsterer, Benjamin Erk, Marie Géléoc, Romain Geneaux, Alexander S. Gentleman, Renaud Guillemin, Iyas Ismail, Per Johnsson, Loïc Journel, Thomas Kierspel, Hansjochen Köckert, Jochen Küpper, Pascal Lablanquie, Jan Lahl, Jason W. L. Lee, Stuart R.
Publié dans: Physical Review A, Numéro 97/4, 2018, Page(s) 043429, ISSN 2469-9934
Éditeur: American Physical Society
DOI: 10.1103/PhysRevA.97.043429

Compact 200 kHz HHG source driven by a few-cycle OPCPA

Auteurs: Anne Harth, Chen Guo, Yu-Chen Cheng, Arthur Losquin, Miguel Miranda, Sara Mikaelsson, Christoph M Heyl, Oliver Prochnow, Jan Ahrens, Uwe Morgner, Anne L’Huillier, Cord L Arnold
Publié dans: Journal of Optics, Numéro 20/1, 2018, Page(s) 014007, ISSN 2040-8978
Éditeur: Institute of Physics Publishing
DOI: 10.1088/2040-8986/aa9b04

Thin-disk pumped optical parametric chirped pulse amplifier delivering CEP-stable multi-mJ few-cycle pulses at 6 kHz

Auteurs: Stephan Prinz, Maximilian Schnitzenbaumer, Dionysios Potamianos, Marcel Schultze, Sebastian Stark, Matthias Häfner, Catherine Y. Teisset, Christoph Wandt, Knut Michel, Reinhard Kienberger, Birgitta Bernhardt, Thomas Metzger
Publié dans: Optics Express, Numéro 26/2, 2018, Page(s) 1108, ISSN 1094-4087
Éditeur: Optical Society of America
DOI: 10.1364/oe.26.001108

Alignment and Imaging of the CS 2 Dimer Inside Helium Nanodroplets

Auteurs: James D. Pickering, Benjamin Shepperson, Bjarke A. K. Hübschmann, Frederik Thorning, Henrik Stapelfeldt
Publié dans: Physical Review Letters, Numéro 120/11, 2018, ISSN 0031-9007
Éditeur: American Physical Society
DOI: 10.1103/PhysRevLett.120.113202

Time–frequency representation of autoionization dynamics in helium

Auteurs: D Busto, L Barreau, M Isinger, M Turconi, C Alexandridi, A Harth, S Zhong, R J Squibb, D Kroon, S Plogmaker, M Miranda, Á Jiménez-Galán, L Argenti, C L Arnold, R Feifel, F Martín, M Gisselbrecht, A L’Huillier, P Salières
Publié dans: Journal of Physics B: Atomic, Molecular and Optical Physics, Numéro 51/4, 2018, Page(s) 044002, ISSN 0953-4075
Éditeur: Institute of Physics Publishing
DOI: 10.1088/1361-6455/aaa057

Note: Knife edge skimming for improved separation of molecular species by the deflector

Auteurs: Sebastian Trippel, Melby Johny, Thomas Kierspel, Jolijn Onvlee, Helen Bieker, Hong Ye, Terry Mullins, Lars Gumprecht, Karol Długołęcki, Jochen Küpper
Publié dans: Review of Scientific Instruments, Numéro 89/9, 2018, Page(s) 096110, ISSN 0034-6748
Éditeur: American Institute of Physics
DOI: 10.1063/1.5026145

High-order harmonic generation spectroscopy by recolliding electron caustics

Auteurs: D Faccialà, S Pabst, B D Bruner, A G Ciriolo, M Devetta, M Negro, P Prasannan Geetha, A Pusala, H Soifer, N Dudovich, S Stagira, C Vozzi
Publié dans: Journal of Physics B: Atomic, Molecular and Optical Physics, Numéro 51/13, 2018, Page(s) 134002, ISSN 0953-4075
Éditeur: Institute of Physics Publishing
DOI: 10.1088/1361-6455/aac351

Two-photon double ionization of neon using an intense attosecond pulse train

Auteurs: B. Manschwetus, L. Rading, F. Campi, S. Maclot, H. Coudert-Alteirac, J. Lahl, H. Wikmark, P. Rudawski, C. M. Heyl, B. Farkas, T. Mohamed, A. L'Huillier, P. Johnsson
Publié dans: Physical Review A, Numéro 93/6, 2016, ISSN 2469-9926
Éditeur: American Physical Society (APS)
DOI: 10.1103/PhysRevA.93.061402

Laser-induced dissociative ionization of H 2 from the near-infrared to the mid-infrared regime

Auteurs: Qingli Jing, Lars Bojer Madsen
Publié dans: Physical Review A, Numéro 94/6, 2016, ISSN 2469-9926
Éditeur: American Physical Society
DOI: 10.1103/PhysRevA.94.063402

Femtosecond laser induced Coulomb explosion imaging of aligned OCS oligomers inside helium nanodroplets

Auteurs: James D. Pickering, Benjamin Shepperson, Lars Christiansen, Henrik Stapelfeldt
Publié dans: The Journal of Chemical Physics, Numéro 149/15, 2018, Page(s) 154306, ISSN 0021-9606
Éditeur: American Institute of Physics
DOI: 10.1063/1.5049555

Multiple ionization of argon via multi-XUV-photon absorption induced by 20-GW high-order harmonic laser pulses

Auteurs: A. Nayak, I. Orfanos, I. Makos, M. Dumergue, S. Kühn, E. Skantzakis, B. Bodi, K. Varju, C. Kalpouzos, H. I. B. Banks, A. Emmanouilidou, D. Charalambidis, P. Tzallas
Publié dans: Physical Review A, Numéro 98/2, 2018, ISSN 2469-9926
Éditeur: PHYSICAL REVIEW A
DOI: 10.1103/physreva.98.023426

Generation of ultrashort pulses by four wave mixing in a gas-filled hollow core fiber

Auteurs: Anna G Ciriolo, Aditya Pusala, Matteo Negro, Michele Devetta, Davide Faccialà, Giacomo Mariani, Caterina Vozzi, Salvatore Stagira
Publié dans: Journal of Optics, Numéro 20/12, 2018, Page(s) 125503, ISSN 2040-8978
Éditeur: Institute of Physics Publishing
DOI: 10.1088/2040-8986/aaec41

Communication: Gas-phase structural isomer identification by Coulomb explosion of aligned molecules

Auteurs: Michael Burt, Kasra Amini, Jason W. L. Lee, Lars Christiansen, Rasmus R. Johansen, Yuki Kobayashi, James D. Pickering, Claire Vallance, Mark Brouard, Henrik Stapelfeldt
Publié dans: The Journal of Chemical Physics, Numéro 148/9, 2018, Page(s) 091102, ISSN 0021-9606
Éditeur: American Institute of Physics
DOI: 10.1063/1.5023441

Generalized perspective on chiral measurements without magnetic interactions

Auteurs: Andres F. Ordonez, Olga Smirnova
Publié dans: Physical Review A, Numéro 98/6, 2018, ISSN 2469-9926
Éditeur: PHYSICAL REVIEW A - American Physical Society
DOI: 10.1103/physreva.98.063428

XUV double-pulses with femtosecond to 650 ps separation from a multilayer-mirror-based split-and-delay unit at FLASH

Auteurs: Mario Sauppe, Dimitrios Rompotis, Benjamin Erk, Sadia Bari, Tobias Bischoff, Rebecca Boll, Cédric Bomme, Christoph Bostedt, Simon Dörner, Stefan Düsterer, Torsten Feigl, Leonie Flückiger, Tais Gorkhover, Katharina Kolatzki, Bruno Langbehn, Nils Monserud, Erland Müller, Jan P. Müller, Christopher Passow, Daniel Ramm, Daniel Rolles, Kaja Schubert, Lucas Schwob, Björn Senfftleben, Rolf Treusch
Publié dans: Journal of Synchrotron Radiation, Numéro 25/5, 2018, Page(s) 1517-1528, ISSN 1600-5775
Éditeur: JOURNAL OF SYNCHROTRON RADIATION
DOI: 10.1107/s1600577518006094

Coulomb explosion imaging of CH 3 I and CH 2 ClI photodissociation dynamics

Auteurs: Felix Allum, Michael Burt, Kasra Amini, Rebecca Boll, Hansjochen Köckert, Pavel K. Olshin, Sadia Bari, Cédric Bomme, Felix Brauße, Barbara Cunha de Miranda, Stefan Düsterer, Benjamin Erk, Marie Géléoc, Romain Geneaux, Alexander S. Gentleman, Gildas Goldsztejn, Renaud Guillemin, David M. P. Holland, Iyas Ismail, Per Johnsson, Loïc Journel, Jochen Küpper, Jan Lahl, Jason W. L. Lee, Sylvain M
Publié dans: The Journal of Chemical Physics, Numéro 149/20, 2018, Page(s) 204313, ISSN 0021-9606
Éditeur: American Institute of Physics
DOI: 10.1063/1.5041381

Extreme-ultraviolet refractive optics

Auteurs: L. Drescher, O. Kornilov, T. Witting, G. Reitsma, N. Monserud, A. Rouzée, J. Mikosch, M. J. J. Vrakking, B. Schütte
Publié dans: Nature, Numéro 564/7734, 2018, Page(s) 91-94, ISSN 0028-0836
Éditeur: Nature Publishing Group
DOI: 10.1038/s41586-018-0737-3

Propensity rules in photoelectron circular dichroism in chiral molecules. I. Chiral hydrogen

Auteurs: Andres F. Ordonez, Olga Smirnova
Publié dans: Physical Review A, Numéro 99/4, 2019, ISSN 2469-9926
Éditeur: PHYSICAL REVIEW A
DOI: 10.1103/physreva.99.043416

Propensity rules in photoelectron circular dichroism in chiral molecules. II. General picture

Auteurs: Andres F. Ordonez, Olga Smirnova
Publié dans: Physical Review A, Numéro 99/4, 2019, ISSN 2469-9926
Éditeur: PHYSICAL REVIEW A
DOI: 10.1103/physreva.99.043417

Spatial separation of pyrrole and pyrrole-water clusters

Auteurs: Melby Johny, Jolijn Onvlee, Thomas Kierspel, Helen Bieker, Sebastian Trippel, Jochen Küpper
Publié dans: Chemical Physics Letters, Numéro 721, 2019, Page(s) 149-152, ISSN 0009-2614
Éditeur: Elsevier BV
DOI: 10.1016/j.cplett.2019.01.052

024 TW ultrabroadband, CEP-stable multipass Ti:Sa amplifier

Auteurs: Mikayel Musheghyan, Fabian Lücking, Zhao Cheng, Harald Frei, Andreas Assion
Publié dans: Optics Letters, Numéro 44/6, 2019, Page(s) 1464, ISSN 0146-9592
Éditeur: Optical Society of America
DOI: 10.1364/ol.44.001464

Single-shot extreme-ultraviolet wavefront measurements of high-order harmonics

Auteurs: Hugo Dacasa, Hélène Coudert-Alteirac, Chen Guo, Emma Kueny, Filippo Campi, Jan Lahl, Jasper Peschel, Hampus Wikmark, Balázs Major, Erik Malm, Domenico Alj, Katalin Varjú, Cord L. Arnold, Guillaume Dovillaire, Per Johnsson, Anne L’Huillier, Sylvain Maclot, Piotr Rudawski, Philippe Zeitoun
Publié dans: Optics Express, Numéro 27/3, 2019, Page(s) 2656, ISSN 1094-4087
Éditeur: Optical Society of America
DOI: 10.1364/oe.27.002656

Spatiotemporal coupling of attosecond pulses

Auteurs: Hampus Wikmark, Chen Guo, Jan Vogelsang, Peter W. Smorenburg, Hélène Coudert-Alteirac, Jan Lahl, Jasper Peschel, Piotr Rudawski, Hugo Dacasa, Stefanos Carlström, Sylvain Maclot, Mette B. Gaarde, Per Johnsson, Cord L. Arnold, Anne L’Huillier
Publié dans: Proceedings of the National Academy of Sciences, Numéro 116/11, 2019, Page(s) 4779-4787, ISSN 0027-8424
Éditeur: National Academy of Sciences
DOI: 10.1073/pnas.1817626116

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