Deliverables
Pump-probe experiment with femtosecond and attosecond time resolution on large molecules will be conducted. The experimental results will be compared with theoretical models, focusing on the kinetic energy release obtained in attosecond XUV-IR pump-probe spectroscopy. The dominant ionization and dissociative pathways will be theoretically identified.
Nonadiabatic strong-field ionization dynamicsNonadiabatic effects in the strong-field ionization of hydrocarbons molecules will be investigated using HHG.
Supervisory Board of the networkThe Supervisory Board of the network will meet for the first time during the kickoff meeting JanuaryFebruary 2015 The Supervisory Board will be composed by the will be composed of the scientistsincharge of the beneficiaries and partner organizations the WP Coordinators Prof Nora Berrah and a representative of the ESRs elected by the young fellows The SB will agree on common guidelines regarding the individual training of the fellows and it will provide the guidelines for the drafting of the CDPs of the individual ESRsDuring this first meeting a training for unbiased selection and dissemination of common best practises to supervisors will be provided kickoff meeting
Structural and dynamical effects in HHGThe interplay between structural and dynamical effects in high-order harmonic generation (HHG) spectroscopy will be elucidated. Advanced alignment techniques will be investigated for the implementation of high-order HHG-based tomography of nonplanar molecules. From the theoretical side, a simulation code for HHG-based spectroscopy of multi-electron dynamics will be developed, considering also the extended harmonic cut-off achieved using mid-IR systems as driving pulses.
High-repetition rate photoelectron spectroscopyAcquisition of photoelectron/photoion pump-probe data with full energy, angular and temporal resolution using the developed high repetition rate (200 kHz) attosecond source . The network will be involved in the development of new apparatuses and technologies for the generation of ultrashort XUV pulses including novel schemes for the stabilisation of the CEP of high-energy, high-repetition rate laser systems operating up to 10 kHz, the demonstration of thin-disk laser pump delivering up to E=200 mJ energy.
Dissemination and outreach activities planA plan for the outreach activities of the ESRs will be drafted This will be based on the activities to be performed in secondary schools using the Photonics Explorer Kit Additional outreach activities for example the participation to specific event such as the Researchers night will be also considered
Time-resolved dynamics in conformer selected beamsConformer selection will be accomplished and time-resolved dynamics in different conformers will be characterized by pump-probe experiment with attosecond and femtosecond resolution.
Influence of the environment on ultrafast eletronic/nuclear dynamics1) Experimental evidences of electronic relaxation mechanism (for example Interatomic Coulombic Decay) induced by intense XUV light pulses in atomic clusters/dimers will be obtained. 2) The influence of the helium environment on the rotational, vibrational and electronic dynamics of embedded molecules will be characterized
Demonstration of coherent control schemes using XUV FELsThe consortium will demonstrate new schemes for the generation of multi-color coherent XUV radiation exploiting FELs. Using this approach, the network will investigated coherent control schemes in the XUV spectral range. In particular, the combination of multi-color coherent XUV radiation will be used to control the photoionization process and electronic dynamics in inner-valence shells in atoms and, eventually also in molecules. Finally we will also investigate novel approaches for the generation of attosecond pulse trains using XUV FELs.
Improved HHG tomography of linear moleculesHHG tomography strongly depends on the quality of alignment of molecules in cold gas jets. We will investigate strategies for a reliable reconstruction of molecular orbitals by HHG in simple linear molecules, even in presence of degraded alignment conditions.
Attosecond XUV-pump-XUV-probe on moleculesThe ultrafast autoionization dynamics of small molecules such as H2/D2 (hydrogen and deuterium) will be characterized exploiting high-energy low repetition rate laser systems.
Dynamical structure by HHGDynamical structure information in simple molecules using XUV light generated by HHG will be obtained
The Webpage of the network will be designed during the first four months The webpage will be used to advertise the network activities the open positions until the recruitment of all ESRs and to disseminate the videoclips virtual lab tours and video tutorials and to communicate the list of speakers of the webinars At the same time the LinkedIn group of the network will be created and maintained
Publications
Author(s):
Daniela Rupp, Nils Monserud, Bruno Langbehn, Mario Sauppe, Julian Zimmermann, Yevheniy Ovcharenko, Thomas Möller, Fabio Frassetto, Luca Poletto, Andrea Trabattoni, Francesca Calegari, Mauro Nisoli, Katharina Sander, Christian Peltz, Marc J. Vrakking, Thomas Fennel, Arnaud Rouzée
Published in:
Nature Communications, Issue 8/1, 2017, Page(s) Article number: 493, ISSN 2041-1723
Publisher:
Nature Publishing Group
DOI:
10.1038/s41467-017-00287-z
Author(s):
A. Golinelli, X. Chen, E. Gontier, B. Bussière, O. Tcherbakoff, M. Natile, P. d’Oliveira, P.-M. Paul, J.-F. Hergott
Published in:
Optics Letters, Issue 42/12, 2017, Page(s) 2326, ISSN 0146-9592
Publisher:
Optical Society of America
DOI:
10.1364/OL.42.002326
Author(s):
Michael Burt, Rebecca Boll, Jason W. L. Lee, Kasra Amini, Hansjochen Köckert, Claire Vallance, Alexander S. Gentleman, Stuart R. Mackenzie, Sadia Bari, Cédric Bomme, Stefan Düsterer, Benjamin Erk, Bastian Manschwetus, Erland Müller, Dimitrios Rompotis, Evgeny Savelyev, Nora Schirmel, Simone Techert, Rolf Treusch, Jochen Küpper, Sebastian Trippel, Joss Wiese, Henrik Stapelfeldt, Barbara Cunha
Published in:
Physical Review A, Issue 96/4, 2017, ISSN 2469-9926
Publisher:
PHYSICAL REVIEW A
DOI:
10.1103/PhysRevA.96.043415
Author(s):
Anna Ciriolo, Matteo Negro, Michele Devetta, Eugenio Cinquanta, Davide Faccialà, Aditya Pusala, Sandro De Silvestri, Salvatore Stagira, Caterina Vozzi
Published in:
Applied Sciences, Issue 7/3, 2017, Page(s) 265, ISSN 2076-3417
Publisher:
Applied Sciences
DOI:
10.3390/app7030265
Author(s):
Coudert-Alteirac, Hélène; Dacasa, Hugo; Campi, Filippo; Kueny, Emma; Farkas, Balázs; Brunner, Fabian; Maclot, Sylvain; Manschwetus, Bastian; Wikmark, Hampus; Lahl, Jan; Rading, Linnea; Peschel, Jasper; Major, Balázs; Varjú, Katalin; Dovillaire, Guillaume; Zeitoun, Philippe; Johnsson, Per; L'Huillier, Anne; Rudawski, Piotr
Published in:
Applied Sciences, Issue 7/11, 1159, 2018, ISSN 2076-3417
Publisher:
Applied Sciences
DOI:
10.3204/PUBDB-2017-11919
Author(s):
Linnea Rading, Jan Lahl, Sylvain Maclot, Filippo Campi, Hélène Coudert-Alteirac, Bart Oostenrijk, Jasper Peschel, Hampus Wikmark, Piotr Rudawski, Mathieu Gisselbrecht, Per Johnsson
Published in:
Applied Sciences, Issue 8/6, 2018, Page(s) 998, ISSN 2076-3417
Publisher:
Applied Sciences
DOI:
10.3390/app8060998
Author(s):
S. Beaulieu, A. Comby, D. Descamps, B. Fabre, G. A. Garcia, R. Géneaux, A. G. Harvey, F. Légaré, Z. Mašín, L. Nahon, A. F. Ordonez, S. Petit, B. Pons, Y. Mairesse, O. Smirnova, V. Blanchet
Published in:
Nature Physics, Issue 14/5, 2018, Page(s) 484-489, ISSN 1745-2473
Publisher:
Nature Publishing Group
DOI:
10.1038/s41567-017-0038-z
Author(s):
Qingli Jing, Roger Y. Bello, Fernando Martín, Alicia Palacios, Lars Bojer Madsen
Published in:
Physical Review A, Issue 97/4, 2018, ISSN 2469-9926
Publisher:
PHYSICAL REVIEW A
DOI:
10.1103/PhysRevA.97.043426
Author(s):
Erik Mårsell, Emil Boström, Anne Harth, Arthur Losquin, Chen Guo, Yu-Chen Cheng, Eleonora Lorek, Sebastian Lehmann, Gustav Nylund, Martin Stankovski, Cord L. Arnold, Miguel Miranda, Kimberly A. Dick, Johan Mauritsson, Claudio Verdozzi, Anne L’Huillier, Anders Mikkelsen
Published in:
Nano Letters, Issue 18/2, 2018, Page(s) 907-915, ISSN 1530-6984
Publisher:
American Chemical Society
DOI:
10.1021/acs.nanolett.7b04267
Author(s):
Chen Guo, Anne Harth, Stefanos Carlström, Yu-Chen Cheng, Sara Mikaelsson, Erik Mårsell, Christoph Heyl, Miguel Miranda, Mathieu Gisselbrecht, Mette B Gaarde, Kenneth J Schafer, Anders Mikkelsen, Johan Mauritsson, Cord L Arnold, Anne L’Huillier
Published in:
Journal of Physics B: Atomic, Molecular and Optical Physics, Issue 51/3, 2018, Page(s) 034006, ISSN 0953-4075
Publisher:
Institute of Physics Publishing
DOI:
10.1088/1361-6455/aa9953
Author(s):
Felix Brauße, Gildas Goldsztejn, Kasra Amini, Rebecca Boll, Sadia Bari, Cédric Bomme, Mark Brouard, Michael Burt, Barbara Cunha de Miranda, Stefan Düsterer, Benjamin Erk, Marie Géléoc, Romain Geneaux, Alexander S. Gentleman, Renaud Guillemin, Iyas Ismail, Per Johnsson, Loïc Journel, Thomas Kierspel, Hansjochen Köckert, Jochen Küpper, Pascal Lablanquie, Jan Lahl, Jason W. L. Lee, Stuart R.
Published in:
Physical Review A, Issue 97/4, 2018, Page(s) 043429, ISSN 2469-9934
Publisher:
American Physical Society
DOI:
10.1103/PhysRevA.97.043429
Author(s):
Anne Harth, Chen Guo, Yu-Chen Cheng, Arthur Losquin, Miguel Miranda, Sara Mikaelsson, Christoph M Heyl, Oliver Prochnow, Jan Ahrens, Uwe Morgner, Anne L’Huillier, Cord L Arnold
Published in:
Journal of Optics, Issue 20/1, 2018, Page(s) 014007, ISSN 2040-8978
Publisher:
Institute of Physics Publishing
DOI:
10.1088/2040-8986/aa9b04
Author(s):
Stephan Prinz, Maximilian Schnitzenbaumer, Dionysios Potamianos, Marcel Schultze, Sebastian Stark, Matthias Häfner, Catherine Y. Teisset, Christoph Wandt, Knut Michel, Reinhard Kienberger, Birgitta Bernhardt, Thomas Metzger
Published in:
Optics Express, Issue 26/2, 2018, Page(s) 1108, ISSN 1094-4087
Publisher:
Optical Society of America
DOI:
10.1364/oe.26.001108
Author(s):
James D. Pickering, Benjamin Shepperson, Bjarke A. K. Hübschmann, Frederik Thorning, Henrik Stapelfeldt
Published in:
Physical Review Letters, Issue 120/11, 2018, ISSN 0031-9007
Publisher:
American Physical Society
DOI:
10.1103/PhysRevLett.120.113202
Author(s):
D Busto, L Barreau, M Isinger, M Turconi, C Alexandridi, A Harth, S Zhong, R J Squibb, D Kroon, S Plogmaker, M Miranda, Á Jiménez-Galán, L Argenti, C L Arnold, R Feifel, F Martín, M Gisselbrecht, A L’Huillier, P Salières
Published in:
Journal of Physics B: Atomic, Molecular and Optical Physics, Issue 51/4, 2018, Page(s) 044002, ISSN 0953-4075
Publisher:
Institute of Physics Publishing
DOI:
10.1088/1361-6455/aaa057
Author(s):
Sebastian Trippel, Melby Johny, Thomas Kierspel, Jolijn Onvlee, Helen Bieker, Hong Ye, Terry Mullins, Lars Gumprecht, Karol Długołęcki, Jochen Küpper
Published in:
Review of Scientific Instruments, Issue 89/9, 2018, Page(s) 096110, ISSN 0034-6748
Publisher:
American Institute of Physics
DOI:
10.1063/1.5026145
Author(s):
D Faccialà, S Pabst, B D Bruner, A G Ciriolo, M Devetta, M Negro, P Prasannan Geetha, A Pusala, H Soifer, N Dudovich, S Stagira, C Vozzi
Published in:
Journal of Physics B: Atomic, Molecular and Optical Physics, Issue 51/13, 2018, Page(s) 134002, ISSN 0953-4075
Publisher:
Institute of Physics Publishing
DOI:
10.1088/1361-6455/aac351
Author(s):
B. Manschwetus, L. Rading, F. Campi, S. Maclot, H. Coudert-Alteirac, J. Lahl, H. Wikmark, P. Rudawski, C. M. Heyl, B. Farkas, T. Mohamed, A. L'Huillier, P. Johnsson
Published in:
Physical Review A, Issue 93/6, 2016, ISSN 2469-9926
Publisher:
American Physical Society (APS)
DOI:
10.1103/PhysRevA.93.061402
Author(s):
Qingli Jing, Lars Bojer Madsen
Published in:
Physical Review A, Issue 94/6, 2016, ISSN 2469-9926
Publisher:
American Physical Society
DOI:
10.1103/PhysRevA.94.063402
Author(s):
James D. Pickering, Benjamin Shepperson, Lars Christiansen, Henrik Stapelfeldt
Published in:
The Journal of Chemical Physics, Issue 149/15, 2018, Page(s) 154306, ISSN 0021-9606
Publisher:
American Institute of Physics
DOI:
10.1063/1.5049555
Author(s):
A. Nayak, I. Orfanos, I. Makos, M. Dumergue, S. Kühn, E. Skantzakis, B. Bodi, K. Varju, C. Kalpouzos, H. I. B. Banks, A. Emmanouilidou, D. Charalambidis, P. Tzallas
Published in:
Physical Review A, Issue 98/2, 2018, ISSN 2469-9926
Publisher:
PHYSICAL REVIEW A
DOI:
10.1103/physreva.98.023426
Author(s):
Anna G Ciriolo, Aditya Pusala, Matteo Negro, Michele Devetta, Davide Faccialà, Giacomo Mariani, Caterina Vozzi, Salvatore Stagira
Published in:
Journal of Optics, Issue 20/12, 2018, Page(s) 125503, ISSN 2040-8978
Publisher:
Institute of Physics Publishing
DOI:
10.1088/2040-8986/aaec41
Author(s):
Michael Burt, Kasra Amini, Jason W. L. Lee, Lars Christiansen, Rasmus R. Johansen, Yuki Kobayashi, James D. Pickering, Claire Vallance, Mark Brouard, Henrik Stapelfeldt
Published in:
The Journal of Chemical Physics, Issue 148/9, 2018, Page(s) 091102, ISSN 0021-9606
Publisher:
American Institute of Physics
DOI:
10.1063/1.5023441
Author(s):
Andres F. Ordonez, Olga Smirnova
Published in:
Physical Review A, Issue 98/6, 2018, ISSN 2469-9926
Publisher:
PHYSICAL REVIEW A - American Physical Society
DOI:
10.1103/physreva.98.063428
Author(s):
Mario Sauppe, Dimitrios Rompotis, Benjamin Erk, Sadia Bari, Tobias Bischoff, Rebecca Boll, Cédric Bomme, Christoph Bostedt, Simon Dörner, Stefan Düsterer, Torsten Feigl, Leonie Flückiger, Tais Gorkhover, Katharina Kolatzki, Bruno Langbehn, Nils Monserud, Erland Müller, Jan P. Müller, Christopher Passow, Daniel Ramm, Daniel Rolles, Kaja Schubert, Lucas Schwob, Björn Senfftleben, Rolf Treusch
Published in:
Journal of Synchrotron Radiation, Issue 25/5, 2018, Page(s) 1517-1528, ISSN 1600-5775
Publisher:
JOURNAL OF SYNCHROTRON RADIATION
DOI:
10.1107/s1600577518006094
Author(s):
Felix Allum, Michael Burt, Kasra Amini, Rebecca Boll, Hansjochen Köckert, Pavel K. Olshin, Sadia Bari, Cédric Bomme, Felix Brauße, Barbara Cunha de Miranda, Stefan Düsterer, Benjamin Erk, Marie Géléoc, Romain Geneaux, Alexander S. Gentleman, Gildas Goldsztejn, Renaud Guillemin, David M. P. Holland, Iyas Ismail, Per Johnsson, Loïc Journel, Jochen Küpper, Jan Lahl, Jason W. L. Lee, Sylvain M
Published in:
The Journal of Chemical Physics, Issue 149/20, 2018, Page(s) 204313, ISSN 0021-9606
Publisher:
American Institute of Physics
DOI:
10.1063/1.5041381
Author(s):
L. Drescher, O. Kornilov, T. Witting, G. Reitsma, N. Monserud, A. Rouzée, J. Mikosch, M. J. J. Vrakking, B. Schütte
Published in:
Nature, Issue 564/7734, 2018, Page(s) 91-94, ISSN 0028-0836
Publisher:
Nature Publishing Group
DOI:
10.1038/s41586-018-0737-3
Author(s):
Andres F. Ordonez, Olga Smirnova
Published in:
Physical Review A, Issue 99/4, 2019, ISSN 2469-9926
Publisher:
PHYSICAL REVIEW A
DOI:
10.1103/physreva.99.043416
Author(s):
Andres F. Ordonez, Olga Smirnova
Published in:
Physical Review A, Issue 99/4, 2019, ISSN 2469-9926
Publisher:
PHYSICAL REVIEW A
DOI:
10.1103/physreva.99.043417
Author(s):
Melby Johny, Jolijn Onvlee, Thomas Kierspel, Helen Bieker, Sebastian Trippel, Jochen Küpper
Published in:
Chemical Physics Letters, Issue 721, 2019, Page(s) 149-152, ISSN 0009-2614
Publisher:
Elsevier BV
DOI:
10.1016/j.cplett.2019.01.052
Author(s):
Mikayel Musheghyan, Fabian Lücking, Zhao Cheng, Harald Frei, Andreas Assion
Published in:
Optics Letters, Issue 44/6, 2019, Page(s) 1464, ISSN 0146-9592
Publisher:
Optical Society of America
DOI:
10.1364/ol.44.001464
Author(s):
Hugo Dacasa, Hélène Coudert-Alteirac, Chen Guo, Emma Kueny, Filippo Campi, Jan Lahl, Jasper Peschel, Hampus Wikmark, Balázs Major, Erik Malm, Domenico Alj, Katalin Varjú, Cord L. Arnold, Guillaume Dovillaire, Per Johnsson, Anne L’Huillier, Sylvain Maclot, Piotr Rudawski, Philippe Zeitoun
Published in:
Optics Express, Issue 27/3, 2019, Page(s) 2656, ISSN 1094-4087
Publisher:
Optical Society of America
DOI:
10.1364/oe.27.002656
Author(s):
Hampus Wikmark, Chen Guo, Jan Vogelsang, Peter W. Smorenburg, Hélène Coudert-Alteirac, Jan Lahl, Jasper Peschel, Piotr Rudawski, Hugo Dacasa, Stefanos Carlström, Sylvain Maclot, Mette B. Gaarde, Per Johnsson, Cord L. Arnold, Anne L’Huillier
Published in:
Proceedings of the National Academy of Sciences, Issue 116/11, 2019, Page(s) 4779-4787, ISSN 0027-8424
Publisher:
National Academy of Sciences
DOI:
10.1073/pnas.1817626116
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