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Opto-valleytronic moiré polaritons

Project description

Twisted 2D semiconductors hold great promise for photonic chips

Polaritons are quasiparticles arising from strong light-matter coupling between cavity photons and semiconductor excitons. In modern van der Waals heterostructures based on twisted transition metal dichalcogenide (TMD) semiconductors, excitons are subject to a modulated in-plane potential due to moiré interference effects. In the regime of strong light-matter coupling to cavity photons, they form respective moiré polaritons with distinct spin-valley polarization and optical selection rules. The EU-funded 2DValley project aims at realizing and studying the regime of strong coupling between optical microcavities and TMD heterostructure systems with the ultimate goal to explore the potential of moiré polaritons for novel opto-valleytronic devices with applications in non-linear and non-reciprocal quantum photonics.

Objective

The emerging field of opto-valleytronics based on two-dimensional (2D) transition metal dichalcogenides (TMDs) has the potential to revolutionize quantum information processing by enabling all-optical quantum photonic circuits with nonlinear and non-reciprocal devices, such as optical switches and isolators. Such devices are inherently difficult to realize because photons generally do not interact and flow in both directions due to time-reversal symmetry. In this action, I propose to develop novel optical microcavities with embedded TMD heterostructures to achieve photon-photon interaction and directional light propagation. A small twist angle between TMD heterobilayers gives rise to hybrid moir excitons exhibiting a permanent dipole moment in addition to increased lifetimes and oscillator strengths. Strongly coupled to a microcavity, moir polaritons emerge with valley-contrasting dipolar optical selection rules. Moir polaritons exhibit optical nonlinearities induced by the moir potential. Based on all this, the overriding research objective of the project 2DValley is to develop and investigate novel opto-valleytronic devices utilizing valley-polarized moir polaritons. To achieve this goal, I will first develop gate-tunable moir polaritons by studying hybrid moir excitons in cryogenic optical spectroscopy and then embedding them into optical microcavities. I propose to lift the valley degeneracy of moir polaritons with an external magnetic field, providing control over the valley degree of freedom. Finally, I propose to replace the external magnetic field by an internal built-in magnetic field via 2D ferromagnets, which enables unprecedented intrinsic control of the valley degree of freedom by lifting valley degeneracy via magnetic proximity exchange interaction. Such nonlinear and non-reciprocal opto-valleytronic devices would have potential technological and societal impact by increasing information processing speed, volume, and security.

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Programme(s)

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Topic(s)

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Funding Scheme

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HORIZON-TMA-MSCA-PF-EF - HORIZON TMA MSCA Postdoctoral Fellowships - European Fellowships

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Call for proposal

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(opens in new window) HORIZON-MSCA-2021-PF-01

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Coordinator

LUDWIG-MAXIMILIANS-UNIVERSITAET MUENCHEN
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 173 847,36
Address
GESCHWISTER SCHOLL PLATZ 1
80539 MUNCHEN
Germany

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Region
Bayern Oberbayern München, Kreisfreie Stadt
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

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