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Force-free microstructures host intrinsic dynamics of orbital phases in AV3Sb5 Kagome metals

Project description

Force-free setup reveals intrinsic electronic orders in AV3Sb5 Kagome superconductors

Electron correlations can result in competing orders and exotic quantum phenomena. The recently discovered AV3Sb5 Kagome superconductors exhibit such correlations and competing correlated orders. Due to robust entanglement, manipulating one order can modify another. Scientists predict that this can result in an orbital-loop current, yet demonstrating this hypothesis experimentally is highly challenging with conventional approaches due to their sensitivity to experimental conditions. The ERC-funded Free-Kagome project aims to investigate three clear pathways to revealing the intrinsic electronic orders of AV3Sb5 Kagome superconductors. These pathways are based on a unique force-free setup with a controllable coupling between the focused-ion-beam fabricated microstructure and its supporting frame, setting the stage ready for exploring quantum functionalities in Kagome metals.

Objective

Electron correlations significantly modify electron self-organization in quantum materials, resulting in a landscape of competing orders and exotic quantum phenomena. The recently discovered AV3Sb5 family Kagome superconductors is an intriguing example of competing correlated orders with robust entanglement, as manipulating one order can affect or modify another, akin to the unique electromagnetic responses of multi-ferroics. These strongly entangled orders have led to an exciting hypothesis of orbital loop current, a prime example of correlation-driven electronic instabilities. Nevertheless, it renders the inherent characteristics practically inaccessible through conventional means, as even slight variations in experimental conditions can significantly affect their physical properties.

Our research plan is to examine the novel electronic response of the hypothesized orbital loop current in AV3Sb5. We will research the intrinsic dynamics of orbital phases and their unique electronic response via 1) atomically engineering the Kagome nets with the comprehensive material database serves as the Kagome toolbox, 2) heat/electric quenching of charge order for effectively tuning the interlayer coupling in a Kagome glass state, 3) spatial control of chiral domains with optical polarization, representing three unambiguous routes for revealing the intrinsic electronic orders in AV3Sb5.

These goals are ambitious yet entirely realizable: Free-Kagome’s research approach is based on a unique force-free setup that features controllable mechanical and thermal coupling between the focused-ion-beam (FIB) fabricated microstructure and its supporting frame based on the extremely soft membrane springs with designed geometry.

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HORIZON-ERC - HORIZON ERC Grants

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Call for proposal

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(opens in new window) ERC-2024-STG

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Host institution

MAX-PLANCK-GESELLSCHAFT ZUR FORDERUNG DER WISSENSCHAFTEN EV
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 1 500 000,00
Address
HOFGARTENSTRASSE 8
80539 MUNCHEN
Germany

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Region
Bayern Oberbayern München, Kreisfreie Stadt
Activity type
Research Organisations
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 1 500 000,00

Beneficiaries (1)

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