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Chiral phononics: Controlling electronic phases with phonon angular momentum

Project description

Controlling the functional properties of solids with phonon angular momentum

Even in solids, molecules or crystals are constantly vibrating around fixed positions. Ultrashort pulses of electromagnetic radiation can modify the crystal structure of solids by resonantly driving coherent phonons (packets of vibrational mechanical energy) that exchange energy and momentum with electrons. Chiral phonons have generally been viewed as a way to dissipate electronic angular momentum rather than a way to control the properties of solids. The ERC-funded CHIRALPHONONICS project aims to investigate how phonon angular momentum can be coherently generated to control functional properties such as topological and ferroic order. Microscopic modelling with first-principles calculations could lead to novel design principles for out-of-equilibrium quantum materials.

Objective

This projects aims to establish a new paradigm in the ultrafast control of solids, by using the angular momentum of chiral lattice vibrations (chiral phonons) to manipulate, induce, and switch electronic phases.

The properties of solids are fundamentally determined by the crystal-lattice geometry. Developments of ultrashort terahertz and mid-IR pulses in the past decade have made it possible to dynamically modify the crystal structure by resonantly driving coherent phonons. These phonons exchange energy and momentum with the electrons, modifying interactions that are dependent on the distance between the atoms.

Chiral phonons, in turn, have mostly been regarded as a dissipation channel for electronic angular momentum and only recently been used for ultrafast control of solids, following seminal theoretical predictions of me and my colleagues. The reason for this is rooted in two challenges: the lack of feasible protocols to coherently excite chiral phonons across the Brillouin zone and the complexity of angular momentum coupling processes out of the equilibrium.

CHIRALPHONONICS will address these challenges by bridging the gap between phonon angular momentum theory and ultrafast dynamical simulations. My team and I will investigate how phonon angular momentum can be coherently generated coupled to electronic, spin, and orbital degrees of freedom that are connected to functional properties, including topological and ferroic order. We will combine microscopic modeling with first-principles calculations to create effective ab-initio informed models that allow us to both predict novel fundamental coupling mechanisms as well as realize quantitative materials implementations.

This research will lead to new functionalities in solids and design principles for quantum materials out of the equilibrium. Pioneering the field of ultrafast chiral phononics will open an avenue towards technologies based on phonon angular momentum switching of electronic states.

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Keywords

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Programme(s)

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Topic(s)

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Funding Scheme

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HORIZON-ERC - HORIZON ERC Grants

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Call for proposal

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(opens in new window) ERC-2024-STG

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Host institution

TECHNISCHE UNIVERSITEIT EINDHOVEN
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 1 500 000,00
Address
GROENE LOPER 3
5612 AE Eindhoven
Netherlands

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Region
Zuid-Nederland Noord-Brabant Zuidoost-Noord-Brabant
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 1 500 000,00

Beneficiaries (1)

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