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Functionality Rotation-Mediated Solvent Separations in Nanochannel Membranes

Project description

Improving solvent separation selectivity without reducing efficiency

Solvent separation is essential in many industries including the pharmaceutical, chemical and energy sectors whereby separating or purifying solvent mixtures is a critical step in production. Traditional methods such as distillation are energy-intensive and costly. Nanochannel membranes with 1 nm channels offer a more energy-efficient alternative. However, improving membrane selectivity often reduces permeability – a trade-off that limits their effectiveness. With the support of the Marie Skłodowska-Curie Actions programme, the FREEMEN project will design membranes with rotatable functionalities that help selectivity without compromising permeability. MXene materials and fast-rotating ammonium ions will be used for their development. The proposed solution could advance membrane design, offering a new mechanism for efficient 1 nm mass transport.

Objective

Nanochannel membranes with 1-nm/sub-1-nm channels provide an energy-efficient and sustainable way of solvent separations for global process-based industries that operate on solvent mixtures. Channel modifications by binding selective functionalities are a widely adopted strategy to improve membrane selectivity, but it often compromises target solvents permeability, presenting a persistent and undesired trade-off dilemma. This is largely due to the relatively fixed position of the functionalities, whose steric hindrance unavoidably retards molecular transport at this scale.

In contrast to previous designs, this project aims to develop a novel nanochannel membrane featuring rotatable functionalities. It takes advantage of functionality dynamics - rotations - to facilitate target solvent transport while blocking competing solvent, effectively overcoming the trade-off. The demonstration and verification of this idea are based on 3 steps, including (1) development of a prototype membranes using a 2D layered MXene assembly as backbone and ammonium ions (NH4+) as functionalities due to their intrinsic ultrafast rotation in solvents (e.g. water); (2) evaluation of the solvent separation performance (e.g. water-ethanol) of such membranes against MXene membranes functionalised by slow-rotating ions or no ion (pristine); (3) elucidation of the relation between functionality rotation and solvent transport/separation by coupling experimental results, key characterizations, and computational modelling.

Project success will advance the state-of-the-art in practical, conceptual, and mechanistic aspects. A high-performance solvent separation membrane that breaks trade-off will be fabricated. A new nanochannel membrane design principle involving functionality dynamics will be established. Most importantly, a functionality rotation-mediated transport mechanism will be proposed as a new perspective to understand 1-nm/sub-1-nm mass transport in future membranes.

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Topic(s)

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Funding Scheme

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HORIZON-TMA-MSCA-PF-EF - HORIZON TMA MSCA Postdoctoral Fellowships - European Fellowships

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Call for proposal

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(opens in new window) HORIZON-MSCA-2024-PF-01

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Coordinator

THE UNIVERSITY OF EDINBURGH
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 260 347,92
Address
OLD COLLEGE, SOUTH BRIDGE
EH8 9YL Edinburgh
United Kingdom

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Region
Scotland Eastern Scotland Edinburgh
Activity type
Higher or Secondary Education Establishments
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Total cost

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