Deliverables Documents, reports (12) Attosecond dynamics in small and large molecules Pump-probe experiment with femtosecond and attosecond time resolution on large molecules will be conducted. The experimental results will be compared with theoretical models, focusing on the kinetic energy release obtained in attosecond XUV-IR pump-probe spectroscopy. The dominant ionization and dissociative pathways will be theoretically identified. Nonadiabatic strong-field ionization dynamics Nonadiabatic effects in the strong-field ionization of hydrocarbons molecules will be investigated using HHG. Supervisory Board of the network The Supervisory Board of the network will meet for the first time during the kickoff meeting JanuaryFebruary 2015 The Supervisory Board will be composed by the will be composed of the scientistsincharge of the beneficiaries and partner organizations the WP Coordinators Prof Nora Berrah and a representative of the ESRs elected by the young fellows The SB will agree on common guidelines regarding the individual training of the fellows and it will provide the guidelines for the drafting of the CDPs of the individual ESRsDuring this first meeting a training for unbiased selection and dissemination of common best practises to supervisors will be provided kickoff meeting Structural and dynamical effects in HHG The interplay between structural and dynamical effects in high-order harmonic generation (HHG) spectroscopy will be elucidated. Advanced alignment techniques will be investigated for the implementation of high-order HHG-based tomography of nonplanar molecules. From the theoretical side, a simulation code for HHG-based spectroscopy of multi-electron dynamics will be developed, considering also the extended harmonic cut-off achieved using mid-IR systems as driving pulses. High-repetition rate photoelectron spectroscopy Acquisition of photoelectron/photoion pump-probe data with full energy, angular and temporal resolution using the developed high repetition rate (200 kHz) attosecond source . The network will be involved in the development of new apparatuses and technologies for the generation of ultrashort XUV pulses including novel schemes for the stabilisation of the CEP of high-energy, high-repetition rate laser systems operating up to 10 kHz, the demonstration of thin-disk laser pump delivering up to E=200 mJ energy. Dissemination and outreach activities plan A plan for the outreach activities of the ESRs will be drafted This will be based on the activities to be performed in secondary schools using the Photonics Explorer Kit Additional outreach activities for example the participation to specific event such as the Researchers night will be also considered Time-resolved dynamics in conformer selected beams Conformer selection will be accomplished and time-resolved dynamics in different conformers will be characterized by pump-probe experiment with attosecond and femtosecond resolution. Influence of the environment on ultrafast eletronic/nuclear dynamics 1) Experimental evidences of electronic relaxation mechanism (for example Interatomic Coulombic Decay) induced by intense XUV light pulses in atomic clusters/dimers will be obtained. 2) The influence of the helium environment on the rotational, vibrational and electronic dynamics of embedded molecules will be characterized Demonstration of coherent control schemes using XUV FELs The consortium will demonstrate new schemes for the generation of multi-color coherent XUV radiation exploiting FELs. Using this approach, the network will investigated coherent control schemes in the XUV spectral range. In particular, the combination of multi-color coherent XUV radiation will be used to control the photoionization process and electronic dynamics in inner-valence shells in atoms and, eventually also in molecules. Finally we will also investigate novel approaches for the generation of attosecond pulse trains using XUV FELs. Improved HHG tomography of linear molecules HHG tomography strongly depends on the quality of alignment of molecules in cold gas jets. We will investigate strategies for a reliable reconstruction of molecular orbitals by HHG in simple linear molecules, even in presence of degraded alignment conditions. Attosecond XUV-pump-XUV-probe on molecules The ultrafast autoionization dynamics of small molecules such as H2/D2 (hydrogen and deuterium) will be characterized exploiting high-energy low repetition rate laser systems. Dynamical structure by HHG Dynamical structure information in simple molecules using XUV light generated by HHG will be obtained Websites, patent fillings, videos etc. (1) Website design and development, and Social Media presence The Webpage of the network will be designed during the first four months The webpage will be used to advertise the network activities the open positions until the recruitment of all ESRs and to disseminate the videoclips virtual lab tours and video tutorials and to communicate the list of speakers of the webinars At the same time the LinkedIn group of the network will be created and maintained Publications Peer reviewed articles (33) Coherent diffractive imaging of single helium nanodroplets with a high harmonic generation source Author(s): Daniela Rupp, Nils Monserud, Bruno Langbehn, Mario Sauppe, Julian Zimmermann, Yevheniy Ovcharenko, Thomas Möller, Fabio Frassetto, Luca Poletto, Andrea Trabattoni, Francesca Calegari, Mauro Nisoli, Katharina Sander, Christian Peltz, Marc J. Vrakking, Thomas Fennel, Arnaud Rouzée Published in: Nature Communications, 8/1, 2017, Page(s) Article number: 493, ISSN 2041-1723 Publisher: Nature Publishing Group DOI: 10.1038/s41467-017-00287-z Original Ti:Sa 10 kHz front-end design delivering 17 fs, 170 mrad CEP stabilized pulses up to 5 W Author(s): A. Golinelli, X. Chen, E. Gontier, B. Bussière, O. Tcherbakoff, M. Natile, P. d’Oliveira, P.-M. Paul, J.-F. Hergott Published in: Optics Letters, 42/12, 2017, Page(s) 2326, ISSN 0146-9592 Publisher: Optical Society of America DOI: 10.1364/OL.42.002326 Coulomb-explosion imaging of concurrent CH 2 BrI photodissociation dynamics Author(s): Michael Burt, Rebecca Boll, Jason W. L. Lee, Kasra Amini, Hansjochen Köckert, Claire Vallance, Alexander S. Gentleman, Stuart R. Mackenzie, Sadia Bari, Cédric Bomme, Stefan Düsterer, Benjamin Erk, Bastian Manschwetus, Erland Müller, Dimitrios Rompotis, Evgeny Savelyev, Nora Schirmel, Simone Techert, Rolf Treusch, Jochen Küpper, Sebastian Trippel, Joss Wiese, Henrik Stapelfeldt, Barbara Cunha Published in: Physical Review A, 96/4, 2017, ISSN 2469-9926 Publisher: PHYSICAL REVIEW A DOI: 10.1103/PhysRevA.96.043415 Optical Parametric Amplification Techniques for the Generation of High-Energy Few-Optical-Cycles IR Pulses for Strong Field Applications Author(s): Anna Ciriolo, Matteo Negro, Michele Devetta, Eugenio Cinquanta, Davide Faccialà, Aditya Pusala, Sandro De Silvestri, Salvatore Stagira, Caterina Vozzi Published in: Applied Sciences, 7/3, 2017, Page(s) 265, ISSN 2076-3417 Publisher: Applied Sciences DOI: 10.3390/app7030265 Micro-focusing of broadband high-order harmonic radiation by a double toroidal mirror Author(s): Coudert-Alteirac, Hélène; Dacasa, Hugo; Campi, Filippo; Kueny, Emma; Farkas, Balázs; Brunner, Fabian; Maclot, Sylvain; Manschwetus, Bastian; Wikmark, Hampus; Lahl, Jan; Rading, Linnea; Peschel, Jasper; Major, Balázs; Varjú, Katalin; Dovillaire, Guillaume; Zeitoun, Philippe; Johnsson, Per; L'Huillier, Anne; Rudawski, Piotr Published in: Applied Sciences, 7/11, 1159, 2018, ISSN 2076-3417 Publisher: Applied Sciences DOI: 10.3204/PUBDB-2017-11919 A Versatile Velocity Map Ion-Electron Covariance Imaging Spectrometer for High-Intensity XUV Experiments Author(s): Linnea Rading, Jan Lahl, Sylvain Maclot, Filippo Campi, Hélène Coudert-Alteirac, Bart Oostenrijk, Jasper Peschel, Hampus Wikmark, Piotr Rudawski, Mathieu Gisselbrecht, Per Johnsson Published in: Applied Sciences, 8/6, 2018, Page(s) 998, ISSN 2076-3417 Publisher: Applied Sciences DOI: 10.3390/app8060998 Photoexcitation circular dichroism in chiral molecules Author(s): S. Beaulieu, A. Comby, D. Descamps, B. Fabre, G. A. Garcia, R. Géneaux, A. G. Harvey, F. Légaré, Z. Mašín, L. Nahon, A. F. Ordonez, S. Petit, B. Pons, Y. Mairesse, O. Smirnova, V. Blanchet Published in: Nature Physics, 14/5, 2018, Page(s) 484-489, ISSN 1745-2473 Publisher: Nature Publishing Group DOI: 10.1038/s41567-017-0038-z Monte Carlo wave-packet approach to trace nuclear dynamics in molecular excited states by XUV-pump–IR-probe spectroscopy Author(s): Qingli Jing, Roger Y. Bello, Fernando Martín, Alicia Palacios, Lars Bojer Madsen Published in: Physical Review A, 97/4, 2018, ISSN 2469-9926 Publisher: PHYSICAL REVIEW A DOI: 10.1103/PhysRevA.97.043426 Spatial Control of Multiphoton Electron Excitations in InAs Nanowires by Varying Crystal Phase and Light Polarization Author(s): Erik Mårsell, Emil Boström, Anne Harth, Arthur Losquin, Chen Guo, Yu-Chen Cheng, Eleonora Lorek, Sebastian Lehmann, Gustav Nylund, Martin Stankovski, Cord L. Arnold, Miguel Miranda, Kimberly A. Dick, Johan Mauritsson, Claudio Verdozzi, Anne L’Huillier, Anders Mikkelsen Published in: Nano Letters, 18/2, 2018, Page(s) 907-915, ISSN 1530-6984 Publisher: American Chemical Society DOI: 10.1021/acs.nanolett.7b04267 Phase control of attosecond pulses in a train Author(s): Chen Guo, Anne Harth, Stefanos Carlström, Yu-Chen Cheng, Sara Mikaelsson, Erik Mårsell, Christoph Heyl, Miguel Miranda, Mathieu Gisselbrecht, Mette B Gaarde, Kenneth J Schafer, Anders Mikkelsen, Johan Mauritsson, Cord L Arnold, Anne L’Huillier Published in: Journal of Physics B: Atomic, Molecular and Optical Physics, 51/3, 2018, Page(s) 034006, ISSN 0953-4075 Publisher: Institute of Physics Publishing DOI: 10.1088/1361-6455/aa9953 Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom Author(s): Felix Brauße, Gildas Goldsztejn, Kasra Amini, Rebecca Boll, Sadia Bari, Cédric Bomme, Mark Brouard, Michael Burt, Barbara Cunha de Miranda, Stefan Düsterer, Benjamin Erk, Marie Géléoc, Romain Geneaux, Alexander S. Gentleman, Renaud Guillemin, Iyas Ismail, Per Johnsson, Loïc Journel, Thomas Kierspel, Hansjochen Köckert, Jochen Küpper, Pascal Lablanquie, Jan Lahl, Jason W. L. Lee, Stuart R. Published in: Physical Review A, 97/4, 2018, Page(s) 043429, ISSN 2469-9934 Publisher: American Physical Society DOI: 10.1103/PhysRevA.97.043429 Compact 200 kHz HHG source driven by a few-cycle OPCPA Author(s): Anne Harth, Chen Guo, Yu-Chen Cheng, Arthur Losquin, Miguel Miranda, Sara Mikaelsson, Christoph M Heyl, Oliver Prochnow, Jan Ahrens, Uwe Morgner, Anne L’Huillier, Cord L Arnold Published in: Journal of Optics, 20/1, 2018, Page(s) 014007, ISSN 2040-8978 Publisher: Institute of Physics Publishing DOI: 10.1088/2040-8986/aa9b04 Thin-disk pumped optical parametric chirped pulse amplifier delivering CEP-stable multi-mJ few-cycle pulses at 6 kHz Author(s): Stephan Prinz, Maximilian Schnitzenbaumer, Dionysios Potamianos, Marcel Schultze, Sebastian Stark, Matthias Häfner, Catherine Y. Teisset, Christoph Wandt, Knut Michel, Reinhard Kienberger, Birgitta Bernhardt, Thomas Metzger Published in: Optics Express, 26/2, 2018, Page(s) 1108, ISSN 1094-4087 Publisher: Optical Society of America DOI: 10.1364/oe.26.001108 Alignment and Imaging of the CS 2 Dimer Inside Helium Nanodroplets Author(s): James D. Pickering, Benjamin Shepperson, Bjarke A. K. Hübschmann, Frederik Thorning, Henrik Stapelfeldt Published in: Physical Review Letters, 120/11, 2018, ISSN 0031-9007 Publisher: American Physical Society DOI: 10.1103/PhysRevLett.120.113202 Time–frequency representation of autoionization dynamics in helium Author(s): D Busto, L Barreau, M Isinger, M Turconi, C Alexandridi, A Harth, S Zhong, R J Squibb, D Kroon, S Plogmaker, M Miranda, Á Jiménez-Galán, L Argenti, C L Arnold, R Feifel, F Martín, M Gisselbrecht, A L’Huillier, P Salières Published in: Journal of Physics B: Atomic, Molecular and Optical Physics, 51/4, 2018, Page(s) 044002, ISSN 0953-4075 Publisher: Institute of Physics Publishing DOI: 10.1088/1361-6455/aaa057 Note: Knife edge skimming for improved separation of molecular species by the deflector Author(s): Sebastian Trippel, Melby Johny, Thomas Kierspel, Jolijn Onvlee, Helen Bieker, Hong Ye, Terry Mullins, Lars Gumprecht, Karol Długołęcki, Jochen Küpper Published in: Review of Scientific Instruments, 89/9, 2018, Page(s) 096110, ISSN 0034-6748 Publisher: American Institute of Physics DOI: 10.1063/1.5026145 High-order harmonic generation spectroscopy by recolliding electron caustics Author(s): D Faccialà, S Pabst, B D Bruner, A G Ciriolo, M Devetta, M Negro, P Prasannan Geetha, A Pusala, H Soifer, N Dudovich, S Stagira, C Vozzi Published in: Journal of Physics B: Atomic, Molecular and Optical Physics, 51/13, 2018, Page(s) 134002, ISSN 0953-4075 Publisher: Institute of Physics Publishing DOI: 10.1088/1361-6455/aac351 Two-photon double ionization of neon using an intense attosecond pulse train Author(s): B. Manschwetus, L. Rading, F. Campi, S. Maclot, H. Coudert-Alteirac, J. Lahl, H. Wikmark, P. Rudawski, C. M. Heyl, B. Farkas, T. Mohamed, A. L'Huillier, P. Johnsson Published in: Physical Review A, 93/6, 2016, ISSN 2469-9926 Publisher: American Physical Society (APS) DOI: 10.1103/PhysRevA.93.061402 Laser-induced dissociative ionization of H 2 from the near-infrared to the mid-infrared regime Author(s): Qingli Jing, Lars Bojer Madsen Published in: Physical Review A, 94/6, 2016, ISSN 2469-9926 Publisher: American Physical Society DOI: 10.1103/PhysRevA.94.063402 Femtosecond laser induced Coulomb explosion imaging of aligned OCS oligomers inside helium nanodroplets Author(s): James D. Pickering, Benjamin Shepperson, Lars Christiansen, Henrik Stapelfeldt Published in: The Journal of Chemical Physics, 149/15, 2018, Page(s) 154306, ISSN 0021-9606 Publisher: American Institute of Physics DOI: 10.1063/1.5049555 Multiple ionization of argon via multi-XUV-photon absorption induced by 20-GW high-order harmonic laser pulses Author(s): A. Nayak, I. Orfanos, I. Makos, M. Dumergue, S. Kühn, E. Skantzakis, B. Bodi, K. Varju, C. Kalpouzos, H. I. B. Banks, A. Emmanouilidou, D. Charalambidis, P. Tzallas Published in: Physical Review A, 98/2, 2018, ISSN 2469-9926 Publisher: PHYSICAL REVIEW A DOI: 10.1103/physreva.98.023426 Generation of ultrashort pulses by four wave mixing in a gas-filled hollow core fiber Author(s): Anna G Ciriolo, Aditya Pusala, Matteo Negro, Michele Devetta, Davide Faccialà, Giacomo Mariani, Caterina Vozzi, Salvatore Stagira Published in: Journal of Optics, 20/12, 2018, Page(s) 125503, ISSN 2040-8978 Publisher: Institute of Physics Publishing DOI: 10.1088/2040-8986/aaec41 Communication: Gas-phase structural isomer identification by Coulomb explosion of aligned molecules Author(s): Michael Burt, Kasra Amini, Jason W. L. Lee, Lars Christiansen, Rasmus R. Johansen, Yuki Kobayashi, James D. Pickering, Claire Vallance, Mark Brouard, Henrik Stapelfeldt Published in: The Journal of Chemical Physics, 148/9, 2018, Page(s) 091102, ISSN 0021-9606 Publisher: American Institute of Physics DOI: 10.1063/1.5023441 Generalized perspective on chiral measurements without magnetic interactions Author(s): Andres F. Ordonez, Olga Smirnova Published in: Physical Review A, 98/6, 2018, ISSN 2469-9926 Publisher: PHYSICAL REVIEW A - American Physical Society DOI: 10.1103/physreva.98.063428 XUV double-pulses with femtosecond to 650 ps separation from a multilayer-mirror-based split-and-delay unit at FLASH Author(s): Mario Sauppe, Dimitrios Rompotis, Benjamin Erk, Sadia Bari, Tobias Bischoff, Rebecca Boll, Cédric Bomme, Christoph Bostedt, Simon Dörner, Stefan Düsterer, Torsten Feigl, Leonie Flückiger, Tais Gorkhover, Katharina Kolatzki, Bruno Langbehn, Nils Monserud, Erland Müller, Jan P. Müller, Christopher Passow, Daniel Ramm, Daniel Rolles, Kaja Schubert, Lucas Schwob, Björn Senfftleben, Rolf Treusch Published in: Journal of Synchrotron Radiation, 25/5, 2018, Page(s) 1517-1528, ISSN 1600-5775 Publisher: JOURNAL OF SYNCHROTRON RADIATION DOI: 10.1107/s1600577518006094 Coulomb explosion imaging of CH 3 I and CH 2 ClI photodissociation dynamics Author(s): Felix Allum, Michael Burt, Kasra Amini, Rebecca Boll, Hansjochen Köckert, Pavel K. Olshin, Sadia Bari, Cédric Bomme, Felix Brauße, Barbara Cunha de Miranda, Stefan Düsterer, Benjamin Erk, Marie Géléoc, Romain Geneaux, Alexander S. Gentleman, Gildas Goldsztejn, Renaud Guillemin, David M. P. Holland, Iyas Ismail, Per Johnsson, Loïc Journel, Jochen Küpper, Jan Lahl, Jason W. L. Lee, Sylvain M Published in: The Journal of Chemical Physics, 149/20, 2018, Page(s) 204313, ISSN 0021-9606 Publisher: American Institute of Physics DOI: 10.1063/1.5041381 Extreme-ultraviolet refractive optics Author(s): L. Drescher, O. Kornilov, T. Witting, G. Reitsma, N. Monserud, A. Rouzée, J. Mikosch, M. J. J. Vrakking, B. Schütte Published in: Nature, 564/7734, 2018, Page(s) 91-94, ISSN 0028-0836 Publisher: Nature Publishing Group DOI: 10.1038/s41586-018-0737-3 Propensity rules in photoelectron circular dichroism in chiral molecules. I. Chiral hydrogen Author(s): Andres F. Ordonez, Olga Smirnova Published in: Physical Review A, 99/4, 2019, ISSN 2469-9926 Publisher: PHYSICAL REVIEW A DOI: 10.1103/physreva.99.043416 Propensity rules in photoelectron circular dichroism in chiral molecules. II. General picture Author(s): Andres F. Ordonez, Olga Smirnova Published in: Physical Review A, 99/4, 2019, ISSN 2469-9926 Publisher: PHYSICAL REVIEW A DOI: 10.1103/physreva.99.043417 Spatial separation of pyrrole and pyrrole-water clusters Author(s): Melby Johny, Jolijn Onvlee, Thomas Kierspel, Helen Bieker, Sebastian Trippel, Jochen Küpper Published in: Chemical Physics Letters, 721, 2019, Page(s) 149-152, ISSN 0009-2614 Publisher: Elsevier BV DOI: 10.1016/j.cplett.2019.01.052 024 TW ultrabroadband, CEP-stable multipass Ti:Sa amplifier Author(s): Mikayel Musheghyan, Fabian Lücking, Zhao Cheng, Harald Frei, Andreas Assion Published in: Optics Letters, 44/6, 2019, Page(s) 1464, ISSN 0146-9592 Publisher: Optical Society of America DOI: 10.1364/ol.44.001464 Single-shot extreme-ultraviolet wavefront measurements of high-order harmonics Author(s): Hugo Dacasa, Hélène Coudert-Alteirac, Chen Guo, Emma Kueny, Filippo Campi, Jan Lahl, Jasper Peschel, Hampus Wikmark, Balázs Major, Erik Malm, Domenico Alj, Katalin Varjú, Cord L. Arnold, Guillaume Dovillaire, Per Johnsson, Anne L’Huillier, Sylvain Maclot, Piotr Rudawski, Philippe Zeitoun Published in: Optics Express, 27/3, 2019, Page(s) 2656, ISSN 1094-4087 Publisher: Optical Society of America DOI: 10.1364/oe.27.002656 Spatiotemporal coupling of attosecond pulses Author(s): Hampus Wikmark, Chen Guo, Jan Vogelsang, Peter W. Smorenburg, Hélène Coudert-Alteirac, Jan Lahl, Jasper Peschel, Piotr Rudawski, Hugo Dacasa, Stefanos Carlström, Sylvain Maclot, Mette B. Gaarde, Per Johnsson, Cord L. Arnold, Anne L’Huillier Published in: Proceedings of the National Academy of Sciences, 116/11, 2019, Page(s) 4779-4787, ISSN 0027-8424 Publisher: National Academy of Sciences DOI: 10.1073/pnas.1817626116 Searching for OpenAIRE data... There was an error trying to search data from OpenAIRE No results available
