Objective Compounds of transition metals with 4d valence electrons (“4d metals”) play eminent roles in many areas of condensed matter physics ranging from unconventional superconductivity to oxide electronics, but fundamental questions about the interplay between the spin-orbit coupling and electronic correlations at the atomic scale remain unanswered. Momentum-resolved spectroscopies of collective electronic excitations yield detailed insight into the magnitude and spatial range of the electronic correlations, and have thus decisively shaped the conceptual understanding of quantum many-body phenomena in 3d-electron systems. We will devise and build a novel resonant inelastic x-ray scattering (RIXS) instrument capable of determining the dispersion relations of electronic collective modes in 4d-metal compounds with full momentum-space coverage, high energy resolution, and monolayer sensitivity. Data from this instrument will yield comprehensive information about the interaction parameters specifying the electronic Hamiltonians of 4d-electron materials, unique insight into the spin-orbital composition of their excited-state wavefunctions, and definitive tests of proposals to realize Kitaev models with spin-liquid states that are potentially relevant in topological quantum computation. The element-specificity of RIXS will also allow us to determine the microscopic exchange interactions in complex materials with both 3d and 4d valence electrons, and its high sensitivity will enable experiments on operational device structures comprising only a few monolayers. We will thus be able to tightly integrate momentum-resolved spectroscopy with state-of-the-art, monolayer-by-monolayer deposition methods of 4d metal-oxide films and heterostructures. The results will fuel a feedback loop comprising synthesis, characterization, and modeling, which will greatly advance our ability to design materials and devices whose functionality derives from the collective organization of electrons. Fields of science natural sciencesphysical sciencescondensed matter physicsnatural scienceschemical sciencesinorganic chemistrytransition metalsnatural sciencesphysical scienceselectromagnetism and electronicssuperconductivitynatural sciencesphysical sciencestheoretical physicsparticle physicsphotonsnatural sciencesphysical sciencesopticsspectroscopy Programme(s) H2020-EU.1.1. - EXCELLENT SCIENCE - European Research Council (ERC) Main Programme Topic(s) ERC-ADG-2014 - ERC Advanced Grant Call for proposal ERC-2014-ADG See other projects for this call Funding Scheme ERC-ADG - Advanced Grant Host institution MAX-PLANCK-GESELLSCHAFT ZUR FORDERUNG DER WISSENSCHAFTEN EV Net EU contribution € 3 176 850,00 Address HOFGARTENSTRASSE 8 80539 Munchen Germany See on map Region Bayern Oberbayern München, Kreisfreie Stadt Activity type Research Organisations Links Contact the organisation Opens in new window Website Opens in new window Participation in EU R&I programmes Opens in new window HORIZON collaboration network Opens in new window Total cost € 3 176 850,00 Beneficiaries (1) Sort alphabetically Sort by Net EU contribution Expand all Collapse all MAX-PLANCK-GESELLSCHAFT ZUR FORDERUNG DER WISSENSCHAFTEN EV Germany Net EU contribution € 3 176 850,00 Address HOFGARTENSTRASSE 8 80539 Munchen See on map Region Bayern Oberbayern München, Kreisfreie Stadt Activity type Research Organisations Links Contact the organisation Opens in new window Website Opens in new window Participation in EU R&I programmes Opens in new window HORIZON collaboration network Opens in new window Total cost € 3 176 850,00