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High Energy Optical Soliton Dynamics for Efficient Sub-Femtosecond and Vacuum-Ultraviolet Pulse Generation

Objective

I will study a new regime of high-energy temporal optical soliton dynamics in gas and plasma filled large-bore hollow capillaries—something never previously attempted. Soliton dynamics are fundamental to many of the most fascinating and useful nonlinear processes occurring in conventional optical fibres. Currently the peak powers demonstrated are around 100 megawatts, in hollow-core photonic crystal fibres, with energies of tens of microjoules. I aim to achieve terawatt peak power, millijoule energy-scale, soliton dynamics, and thus combine high-field laser science with the physics of solitons.

I will transfer energy from millijoule pump solitons in the near-infrared to the vacuum ultraviolet (100 nm to 200 nm, 6 eV to 12 eV), through resonant dispersive-wave emission. The emitted radiation will be coherent, ultrafast, and tunable through control of the filling gas pressure and capillary bore radius. The predicted conversion efficiencies are up to 20%, leading to VUV energies of over 400 microjoules in pulse durations of just 400 attoseconds (a single-cycle), with corresponding terawatt peak power; making this low-cost and table-top VUV source brighter than synchrotron sources. This will have wide impact: the VUV region, poorly served by current sources, is of great importance to many ultrafast spectroscopy techniques because many materials have electronic resonances there.

Through soliton self-compression I will also compress 10 femtosecond, millijoule-scale, near-infrared, pump pulses to both single-cycle and even sub-cycle waveforms, achieving sub-femtosecond durations and terawatt peak powers. These will be the shortest isolated optical pulses ever generated in the near-infrared spectral region. I will use them to drive high-energy isolated attosecond pulse generation in the XUV through HHG.

Finally, I will combine these VUV and XUV sources, in a single experiment, to perform proof-of-concept attosecond resolved VUV–XUV pump-probe spectroscopy experiments.

Fields of science (EuroSciVoc)

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Programme(s)

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Topic(s)

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Funding Scheme

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ERC-STG - Starting Grant

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Call for proposal

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(opens in new window) ERC-2015-STG

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Host institution

HERIOT-WATT UNIVERSITY
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 1 723 190,99
Address
RICCARTON
EH14 4AS Edinburgh
United Kingdom

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Region
Scotland Eastern Scotland Edinburgh
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 1 723 190,99

Beneficiaries (1)

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