Novel photo-assisted systems for direct Solar-driven redUctioN of CO2 to energy rich CHEMicals

Livrables

Report on the prediction of the behaviour of the materials from T2.1-2 for theoretical/rational design composites

Will be completed soon by ULEI

LCA and LCC of ethylene production from different PEC configurations, and at different TRL

Application of LCA this to analyze the whole life cycle of different configurations of ethylene production by PC and PEC and to understand and evaluate the various environmental impacts of the production processes. Similarly to LCA, specific guidelines for LCC will be proposed by IFPEN again. LCC is a methodology framework that generally aim to examine technological feasibility and economic profitability of a process, product or service, by combining results from classical Techno-Economic Assessment (TEA) with the monetarization of environmental impacts / flows.

Report on the understanding of the physiochemical properties of the as-prepared materials

After elaboration of most performing composites for CO2 reduction reaction pysicochemical evidences are necessary to explain their optimal behavior and disseminate these materials beyond the stateoftheart in top Q1 articles

Report on the identification of the optimal synthetic methods, combination ans proportions of materials

After screening several synthetic methods proportions of best of both SCs and M NPs selection will be made The goal is to find the best compromise in term of intimate interfacial contact between the different components for rationally design the multiphase materials

Report on system performance under simulated sunlight irradiation and optimisation roadmap

A final report summarising the solar to fuels performance of all systems studied throughout the project will be issued. The main correlations between components and assemblies towards performance and stability will be identify. These conclusions will allow us to define strengths, weaknesses and a roadmap for future development.

Report on social acceptance study and impacts on energy security

The aim of D7.3 is to present an overview of the anticipated social opposition, which will include a guideline on how planning and usage actions related to this technology can increase the likelihood of social acceptance. In order to do so, surveys and qualitative interviews will be carried out with relevant stakeholder groups. The analysis of the collected data will be conducted through known frameworks for other renewable energy technologies, why the only critical element is the selection of respondents and the validation of the collected data. D.7.3 will moreover focus on the impact on energy security for energy consumers after implementation of the technology. The analysis of this part will depend on the information gathered on the expected efficiency, as the entire project is aiming at a contribution to a stable energy supply. The technology will therefore be assessed in terms of availability and efficiency, and further analyzed follow standard principles of energy security.

Roadmap for upscaling towards TW scale

A detailed plan for upscaling the system will be reported. The remaining challenges and the milestones over the relevant time period will be discussed in detail.

Project website in English

Website with specific sections that will all be available in English. A written report with the main contents from the website will be produced.

Publications

Defect engineering over anisotropic brookite toward substrate-specific photo-oxidation of alcohols

Auteurs: S. M. Hossein Hejazi, Mahdi Shahrezaei, Piotr Błoński, Mattia Allieta, Polina M. Sheverdyaeva, Paolo Moras, Zdeněk Baďura, Sergii Kalytchuk, Elmira Mohammadi, Radek Zbořil, Štěpán Kment, Michal Otyepka, Alberto Naldoni, Paolo Fornasiero
Publié dans: Chem Catalysis, 2022, ISSN 2667-1093
Éditeur: Elsevier
DOI: 10.1016/j.checat.2022.03.015

Cooperative Effects Drive Water Oxidation Catalysis in Cobalt Electrocatalysts through the Destabilization of Intermediates

Auteurs: Benjamin Moss; Katrine Louise Svane; David Nieto-Castro; Reshma R. Rao; Soren B. Scott; Cindy Tseng; Michael Sachs; Anuj Pennathur; Caiwu Liang; Louise I. Oldham; Eva Mazzolini; Lole Jurado; Gopinathan Sankar; Stephen Parry; Veronica Celorrio; Jahan M. Dawlaty; Jan Rossmeisl; J. R. Galán-Mascarós; Ifan E. L. Stephens; James R. Durrant
Publié dans: Journal of the American Chemical Society, Numéro 2, 2024, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.3c11651

The role of crystal facets and disorder on photo-electrosynthesis

Auteurs: Ernest Pastor; Laura Montañés; Ana Gutiérrez-Blanco; Franziska S. Hegner; Camilo A. Mesa; Núria López; Sixto Giménez
Publié dans: Nanoscale, Numéro 4, 2022, ISSN 2040-3364
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d2nr03609f

Design of dye-sensitized TiO2 materials for photocatalytic hydrogen production: light and shadow

Auteurs: Lorenzo Zani, Michele Melchionna, Tiziano Montini, Paolo Fornasiero
Publié dans: JPhys Energy, 2021, ISSN 2515-7655
Éditeur: IOP Publishing
DOI: 10.1088/2515-7655/abe04b

Challenges and prospects of plasmonic metasurfaces for photothermal catalysis

Auteurs: Luca Mascaretti; Andrea Schirato; Paolo Fornasiero; Alexandra Boltasseva; Vladimir M. Shalaev; Alessandro Alabastri; Alberto Naldoni
Publié dans: Nanophotonics, Numéro 5, 2022, ISSN 2192-8614
Éditeur: De Gruyter
DOI: 10.1515/nanoph-2022-0073

Electrocatalytic CO$_2$ Reduction: Role of the Cross-Talk at Organic-Inorganic Interfaces

Auteurs: Melchionna, Michele; Fornasiero, Paolo; Prato, Maurizio; Bonchio, Marcella
Publié dans: Energy & Environmental Science, Numéro 5, 2022, ISSN 1754-5692
Éditeur: Royal Society of Chemistry
DOI: 10.48550/arxiv.2212.04410

Effect of Band Bending in Photoactive MOF-Based Heterojunctions

Auteurs: Giulia E. M. Schukraft; Benjamin Moss; Andreas G. Kafizas; Camille Petit
Publié dans: ACS Applied Materials & Interfaces, Numéro 5, 2022, ISSN 1944-8244
Éditeur: American Chemical Society
DOI: 10.1021/acsami.2c00335

Morphology and Light‐Dependent Spatial Distribution of Spin Defects in Carbon Nitride

Auteurs: Arianna Actis; Michele Melchionna; Giacomo Filippini; Paolo Fornasiero; Maurizio Prato; Enrico Salvadori; Mario Chiesa
Publié dans: Angewandte Chemie, Numéro 2, 2022, ISSN 0044-8249
Éditeur: Wiley-VCH GmbH
DOI: 10.1002/ange.202210640

Well-defined Cu2O photocatalysts for solar fuels and chemicals

Auteurs: Sourav Rej; Matteo Bisetto; Alberto Naldoni; Paolo Fornasiero
Publié dans: Journal of Materials Chemistry A, 2021, ISSN 2050-7488
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0ta10181h

Plasmonic Au-based junctions onto TiO2, gC3N4, and TiO2-gC3N4 systems for photocatalytic hydrogen production: Fundamentals and challenges

Auteurs: Valérie Keller; Valérie Caps; Pablo Jiménez-Calvo; Pablo Jiménez-Calvo
Publié dans: Renewable and Sustainable Energy Reviews, Numéro 3, 2021, ISSN 1364-0321
Éditeur: Elsevier BV
DOI: 10.1016/j.rser.2021.111095

Facile Surfactant-Assisted Synthesis of BiVO4 Nanoparticulate Films for Solar Water Splitting

Auteurs: Laura Montañes; Camilo A. Mesa; Ana Gutiérrez-Blanco; Christian Robles; Beatriz Julián-López; Sixto Gimenez
Publié dans: Catalysts, Vol 11, Iss 1244, p 1244 (2021), 2021, ISSN 2073-4344
Éditeur: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/catal11101244

A Parametric Study of the Crystal Phases on Au/TiO2 Photocatalysts for CO2 Gas-Phase Reduction in the Presence of Water

Auteurs: Clément Marchal; Caroline Mary; Leila Hammoud; Qingyang Xi; Joumana Toufaily; Tayssir Hamieh; Luka Suhadolnik; Paolo Fornasiero; Christophe Colbeau-Justin; Valérie Caps; Thomas Cottineau; Valérie Keller
Publié dans: Catalysts, Numéro 3, 2022, ISSN 2073-4344
Éditeur: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/catal12121623

Proactive understanding of the multi-level stakeholder acceptance of a novel renewable energy technology: Chemical storage of solar energy

Auteurs: Maja Due Kadenic, Anne Gammelgaard Ballantyne, Trine Bjørn Olsen, Peter Enevoldsen, Allan Gross
Publié dans: Energy Research & Social Science, Numéro Volume 108, 2024, ISSN 2214-6296
Éditeur: Elsevier Limited
DOI: 10.1016/j.erss.2023.103370

Photodoping and Fast Charge Extraction in Ionic Carbon Nitride Photoanodes

Auteurs: Christiane Adler; Shababa Selim; Igor Krivtsov; Chunyu Li; Chunyu Li; Dariusz Mitoraj; Benjamin Dietzek; Benjamin Dietzek; James R. Durrant; Radim Beranek
Publié dans: Advanced functional materials, 2021, ISSN 1616-301X
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/adfm.202105369

Electrocatalytic CO2 reduction: role of the cross-talk at nano-carbon interfaces

Auteurs: Michele Melchionna; Paolo Fornasiero; Maurizio Prato; Maurizio Prato; Marcella Bonchio
Publié dans: Royal Society of Chemistry, 2021, ISSN 1754-5692
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d1ee00228g

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