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Atomic Quantum Emitters in 2D Frameworks

Project description

Engineering and probing atomic quantum systems in 2D materials at the space-time limit

The ability to create and control connected quantum states lies at the heart of quantum information technologies. Manipulating the electron spin associated with colour centres in 2D materials could eventually eliminate the need for keeping quantum technologies in cryogenic environments. However, developing the full potential of these atomic qubit systems is hampered by the lack of atomistic insight into their properties. The EU-funded AQE2D project aims to overcome this challenge by tapping into breakthrough developments in the synthetic control of 2D materials and ultrafast, single-atom probes. Atomically precise engineering of 2D materials and unprecedented insight into atomic quantum emitters could transform quantum sensing and quantum information.

Objective

The ability to create and control connected quantum states established the advent of quantum information technologies (Q-IT). Manipulation of the electron spin associated with colour centres in solid state crystals is one of the pillar technologies that could eventually push Q-IT beyond cryogenic environments. Exploitation of the full potential of these atomic qubit systems is, however, hampered by two key challenges: the lack of atomistic insights into their properties, and the ability to place them with the required fidelity and atomic spatial precision.

Here I propose to converge recent breakthrough developments in the synthetic control of two-dimensional (2D) materials and ultra-fast, single-atom resolving probes to overcome these challenges. Specifically, I will develop a platform for electro-optically addressable spin qubits (Atomic Quantum Emitters, AQEs) in 2D materials based on atomic dopants in transition metal dichalcogenide (TMD) monolayers and molecular spin systems in 2D covalent organic frameworks (2D-COFs). These systems will provide an ideal platform to generate AQEs by chemical design, to control the mesoscopic environment averting variability between emitters, to achieve atomically precise spatial placement, to identify and eliminate decoherence channels, and to develop high-fidelity scalable pumping schemes.

The proposed construction of a spin-polarized ultrafast THz scanning probe microscope with optical detection capabilities will enable the direct correlation of structural, electronic, magnetic, and optical properties of individual AQEs with simultaneous atomic spatial resolution and picosecond time resolution. This will open new frontiers in the spatio-temporal characterization and control of solid-state AQE systems.

The atomically precise engineering of 2D quantum materials and unprecedented microscopic insights into AQEs bear transformative potential for the field of quantum sensing, communication and information processing.

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Keywords

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Programme(s)

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Topic(s)

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Funding Scheme

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ERC-STG - Starting Grant

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Call for proposal

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(opens in new window) ERC-2020-STG

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Host institution

EIDGENOSSISCHE MATERIALPRUFUNGS- UND FORSCHUNGSANSTALT
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 2 139 400,00
Address
UEBERLANDSTRASSE 129
8600 Dubendorf
Switzerland

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Region
Schweiz/Suisse/Svizzera Zürich Zürich
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 2 139 400,00

Beneficiaries (1)

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