Electron beams enhancing analytical microscopy

Deliverables

Report on first year progress
Report on charge-carrier dynamics mapped using coincidence EELS-CL microscopy
Cross-project collaboration plan in coordination with the ONEM project

Crossproject collaboration plan in coordination with the ONEM project

Report on interim results

Logo, website, and social media accounts

Logo website and social media accounts

First summer school on novel concepts in EM
First Workshop on Electron Beam Spectroscopy for Nanophotonics

Kick-off meeting

Kickoff meeting

Publications

Nanoscale Modification of WS2 Trion Emission by Its Local Electromagnetic Environment

Author(s): Bonnet, N.; Lee, H. Y.; Shao, F. H.; Woo, S. Y.; Blazit, J. D.; Watanabe, K.; Taniguchi, T.; Zobelli, A.; Stephan, O.; Kociak, M.; Gradecak, S. and Tizei, L. H. G.
Published in: Nano Letters, Issue 21, 2021, Page(s) 10178-10185, ISSN 1530-6984
Publisher: American Chemical Society
DOI: 10.1021/acs.nanolett.1c02600

A fast push to photon pairs

Author(s): Nahid Talebi
Published in: Nature Physics, 2022, ISSN 1745-2473
Publisher: Nature Publishing Group
DOI: 10.1038/s41567-021-01410-0

Optical coherence transfer mediated by free electrons

Author(s): O. Kfir, V. Di Giulio, F. J. García de Abajo, and C. Ropers
Published in: Science Advances, 2021, ISSN 2375-2548
Publisher: American Association for the Advancement of Science
DOI: 10.1126/sciadv.abf6380

Charting the Exciton–Polariton Landscape of WSe2 Thin Flakes by Cathodoluminescence Spectroscopy

Author(s): Masoud Taleb,Fatemeh Davoodi,Florian K. Diekmann,Kai Rossnagel and Nahid Talebi
Published in: Advanced Photonics Research, 2021, ISSN 2699-9293
Publisher: Wiley-VCH GmbH
DOI: 10.1002/adpr.202100124

Optical Excitations with Electron Beams: Challenges and Opportunities

Author(s): F. J. García de Abajo and V. Di Giulio
Published in: ACS Photonics, 2021, ISSN 2330-4022
Publisher: American Chemical Society
DOI: 10.1021/acsphotonics.0c01950

Optical manipulation of matter waves

Author(s): KAMRAN AKBARI, VALERIO DI GIULIO AND F. JAVIER GARCÍA DE ABAJO
Published in: Science Advances, 2022, ISSN 2375-2548
Publisher: American Association for the Advancement of Science
DOI: 10.1126/sciadv.abq2659

Event driven 4D STEM acquisition with a Timepix3 detector: Microsecond dwell time and faster scans for high precision and low dose applications

Author(s): Jannis D., Hofer C., Gao, C., Xie X., Béché A., Pennycook, Tj., Verbeeck J.
Published in: Ultramicroscopy, 2022, ISSN 0304-3991
Publisher: Elsevier BV
DOI: 10.1016/j.ultramic.2021.113423

Modulation of Cathodoluminescence Emission by Interference with External Light

Author(s): V. Di Giulio, O. Kfir, C. Ropers, and F. J. García de Abajo
Published in: ACS Nano, 2021, ISSN 1936-0851
Publisher: American Chemical Society
DOI: 10.1021/acsnano.1c00549

Three-dimensional vectorial imaging of surface phonon polaritons

Author(s): Li, X. Y.; Haberfehlner, G.; Hohenester, U.; Stephan, O.; Kothleitner, G. and Kociak, M.
Published in: Science, Issue 371, 2021, Page(s) 1364-1367, ISSN 0036-8075
Publisher: American Association for the Advancement of Science
DOI: 10.1126/science.abg0330

Spontaneous and stimulated electron–photon interactions in nanoscale plasmonic near fields

Author(s): M. Liebtrau, M. Sivis, A. Feist, H. Lourenço-Martins, N. Pazos-Perez, R. A. Álvarez-Puebla, F. J. García de Abajo, A. Polman, and C. Ropers
Published in: Light: Science & Applications, 2021, ISSN 2095-5545
Publisher: Nature Publishing Group
DOI: 10.1038/s41377-021-00511-y

Employing Cathodoluminescence for Nanothermometry and Thermal Transport Measurements in Semiconductor Nanowires

Author(s): Kelly W. Mauser; Magdalena Solà-Garcia; Matthias Liebtrau; Benjamin Damilano; Pierre-Marie Coulon; Stéphane Vézian; Philip A. Shields; Sophie Meuret; Albert Polman
Published in: ACS Nano, 2021, ISSN 1936-0851
Publisher: American Chemical Society
DOI: 10.1021/acsnano.1c00850

Interaction of excitons with Cherenkov radiation in WSe2 beyond the non-recoil approximation

Author(s): F. Chahshouri, M. Taleb, F. K Diekmann, K. Rossnagel and N. Talebi
Published in: Journal of Physics D: Applied Physics, 2022, ISSN 0022-3727
Publisher: Institute of Physics Publishing
DOI: 10.1088/1361-6463/ac453a

Cathodoluminescence excitation spectroscopy: Nanoscale imaging of excitation pathways

Author(s): NADEZDA VARKENTINA, YVES AUAD, STEFFI Y. WOO, ALBERTO ZOBELLI, LAURA BOCHER, JEAN-DENIS BLAZIT, XIAOYAN LI, MARCEL TENCÉ, KENJI WATANABE, TAKASHI TANIGUCHI, ODILE STÉPHAN, MATHIEU KOCIAK , AND LUIZ H. G. TIZEI
Published in: Science Advances, Issue 8, 2022, ISSN 2375-2548
Publisher: American Association for the Advancement of Science
DOI: 10.1126/sciadv.abq4947

Can Copper Nanostructures Sustain High-Quality Plasmons?

Author(s): Mkhitaryan, V.; March, K.; Tseng, E. N.; Li, X. Y.; Scarabelli, L.; Liz-Marzan, L. M.; Chen, S. Y.; Tizei, L. H. G.; Stephan, O.; Song, J. M.; Kociak, M.; de Abajo, F. J. G. and Gloter, A.
Published in: Nano Letters, 2021, ISSN 1530-6984
Publisher: American Chemical Society
DOI: 10.1021/acs.nanolett.0c04667

μeV electron spectromicroscopy using free-space light

Author(s): Yves Auad, Eduardo J. C. Dias, Marcel Tencé, Jean-Denis Blazit, Xiaoyan Li, Luiz Fernando Zagonel, Odile Stéphan, Luiz H. G. Tizei, F. Javier García de Abajo, & Mathieu Kociak
Published in: Nature Communications, 2023, ISSN 2041-1723
Publisher: Nature Publishing Group
DOI: 10.1038/s41467-023-39979-0

Modulation of Cathodoluminescence by Surface Plasmons in Silver Nanowires

Author(s): Amelia C. Y. Liu, Timothy J. Davis, Toon Coenen, Sangeetha Hari, Lenard M. Voortman, Zhou Xu, Gangcheng Yuan, Patrycja M. Ballard, Alison M. Funston, Joanne Etheridge
Published in: Small, 2023, ISSN 1613-6829
Publisher: Wiley
DOI: 10.1002/smll.202207747

Cavity-mediated electron-photon pairs

Author(s): Armin Feist, Guanhao Huang, Germaine Arend, Yujia Yang, Jan-Wilke Henke, Arslan Sajid Raja, F. Jasmin Kappert, Rui Ning Wang, Hugo Lourenço-Martins, Zheru Qiu, Junqiu Liu, Ofer Kfir, Tobias J. Kippenberg, and Claus Ropers
Published in: Science, 2022, ISSN 0036-8075
Publisher: American Association for the Advancement of Science
DOI: 10.1126/science.abo5037

Complete Excitation of Discrete Quantum Systems by Single Free Electrons

Author(s): García de Abajo, F. Javier; Dias, Eduardo J. C.; Di Giulio, Valerio
Published in: Physical Review Letters, Issue 14, 2022, ISSN 1079-7114
Publisher: American Physical Society
DOI: 10.5281/zenodo.6638381

Author(s): Rudolf Haindl, Armin Feist, Till Domröse, Marcel Möller, John H. Gaida, Sergey V. Yalunin & Claus Ropers
Published in: Nature Physics, 2023, ISSN 1745-2473
Publisher: Nature Publishing Group
DOI: 10.1038/s41567-023-02067-7

Optical-cavity mode squeezing by free electrons

Author(s): Valerio Di Giulio and F. Javier García de Abajo
Published in: Nanophotonics, 2023, ISSN 2192-8614
Publisher: De Gruyter
DOI: 10.1515/nanoph-2022-0481

Attosecond electron microscopy by free-electron homodyne detection

Author(s): JH Gaida, H Lourenço-Martins, M Sivis, T Rittmann, A Feist, F de Abajo, C Ropers
Published in: Nature Communications, 2023, ISSN 2041-1723
Publisher: Nature Publishing Group
DOI: 10.48550/arxiv.2305.03005

Photon Statistics of Incoherent Cathodoluminescence with Continuous and Pulsed Electron Beams

Author(s): Magdalena Solà-Garcia, Kelly W. Mauser, Matthias Liebtrau, Toon Coenen, Silke Christiansen, Sophie Meuret and Albert Polman
Published in: ACS Photonics, 2021, ISSN 2330-4022
Publisher: American Chemical Society
DOI: 10.1021/acsphotonics.0c01939

Unveiling the Coupling of Single Metallic Nanoparticles to Whispering-Gallery Microcavities

Author(s): Auad, Y.; Hamon, C.; Tence, M.; Lourenco-Martins, H.; Mkhitaryan, V.; Stephan, O.; de Abajo, F. J. G.; Tizei, L. H. G. and Kociak, M.
Published in: Nano Letters, Issue 22, 2021, Page(s) 319-327, ISSN 1530-6984
Publisher: American Chemical Society
DOI: 10.1021/acs.nanolett.1c03826

Theory of Atomic-Scale Vibrational Mapping and Isotope Identification with Electron Beams

Author(s): A. Konečná, F. Iyikanat, and F. J. García de Abajo
Published in: ACS Nano, 2021, ISSN 1936-0851
Publisher: American Chemical Society
DOI: 10.1021/acsnano.1c01071

Inelastic electron scattering at a single-beam structured light wave

Author(s): Sven Ebel, Nahid Talebi
Published in: Communications Physics, Issue 6, 2023, ISSN 2399-3650
Publisher: Nature Portfolio
DOI: 10.1038/s42005-023-01300-2

Spatiotemporal Electron Beam Focusing through Parallel Interactions with Shaped Optical Fields

Author(s): F. Javier García de Abajo and Claus Ropers
Published in: Physical Review Letters, 2023, ISSN 1079-7114
Publisher: American Physical Society
DOI: 10.1103/physrevlett.130.246901

Integrated photonics enables continuous-beam electron phase modulation

Author(s): Jan-Wilke Henke, Arslan Sajid Raja, Armin Feist, Guanhao Huang, Germaine Arend, Yujia Yang, F. Jasmin Kappert, Rui Ning Wang, Marcel Möller, Jiahe Pan, Junqiu Liu, Ofer Kfir, Claus Ropers and Tobias J. Kippenberg
Published in: Nature, 2021, ISSN 0028-0836
Publisher: Nature Publishing Group
DOI: 10.1038/s41586-021-04197-5

Coincidence Detection of EELS and EDX Spectral Events in the Electron Microscope

Author(s): Daen Jannis; Knut Müller-Caspary; Armand Béché; Jo Verbeeck
Published in: Applied Sciences, 2021, ISSN 2076-3417
Publisher: MDPI
DOI: 10.3390/app11199058

Optical Modulation of Electron Beams in Free Space

Author(s): F. J. García de Abajo and A. Konečná
Published in: Physical Review Letters, 2021, ISSN 0031-9007
Publisher: American Physical Society
DOI: 10.1103/physrevlett.126.123901

Inelastic Scattering of Electron Beams by Nonreciprocal Nanotructures

Author(s): R. Yu, A. Konečná, and F. J. García de Abajo
Published in: Physical Review Letters, 2021, ISSN 0031-9007
Publisher: American Physical Society
DOI: 10.1103/physrevlett.127.157404

Plasmon–Exciton Interactions in Nanometer-Thick Gold-WSe2 Multilayer Structures: Implications for Photodetectors, Sensors, and Light-Emitting Devices

Author(s): Fatemeh Davoodi and Nahid Talebi
Published in: ACS Applied Nano Materials, 2021, ISSN 2574-0970
Publisher: American Chemical Society
DOI: 10.1021/acsanm.1c00889

Tailored high-contrast attosecond electron pulses for coherent excitation and scattering

Author(s): Yalunin, S. V., Feist, A. and Ropers, C.
Published in: Physical Review Research, 2021, ISSN 2643-1564
Publisher: American Physical Society
DOI: 10.1103/physrevresearch.3.l032036

Time-resolved cathodoluminescence in an ultrafast transmission electron microscope

Author(s): Meuret, S.; Tizei, L. H. G.; Houdellier, F.; Weber, S.; Auad, Y.; Tence, M.; Chang, H. C.; Kociak, M. and Arbouet, A.
Published in: Applied Physics Letters, 2021, ISSN 0003-6951
Publisher: American Institute of Physics
DOI: 10.1063/5.0057861

Phase-locked photon–electron interaction without a laser

Author(s): Masoud Taleb, Mario Hentschel, Kai Rossnagel, Harald Giessen, Nahid Talebi
Published in: Nature Physics, 2023, ISSN 1745-2481
Publisher: Nature Portfolio
DOI: 10.1038/s41567-023-01954-3

Multi-plasmon effects and plasmon satellites in photoemission from nanostructures

Author(s): P. A. D. Gonçalves and F. Javier García de Abajo
Published in: Nanoscale, 2023, ISSN 2040-3372
Publisher: Royal Society of Chemistry
DOI: 10.1039/d3nr01223a

Spin–orbit interactions in plasmonic crystals probed by site-selective cathodoluminescence spectroscopy

Author(s): Masoud Taleb; Mohsen Samadi; Fatemeh Davoodi; Maximilian Black; Janek Buhl; Hannes Lüder; Martina Gerken; Nahid Talebi
Published in: Nanophotonics, Issue 6, 2023, Page(s) 1877-1889, ISSN 2192-8614
Publisher: 2023
DOI: 10.1515/nanoph-2023-0065

Lorentz Microscopy of Optical Fields

Author(s): John Gaida, Hugo Lourenço-Martins, Sergey Yalunin, Armin Feist, Murat Sivis, Thorsten Hohage, Javier García de Abajo, and Claus Ropers
Published in: Nature Communications, 2023, ISSN 2041-1723
Publisher: Nature Publishing Group
DOI: 10.21203/rs.3.rs-2150760/v1

Tailoring the Band Structure of Plexcitonic Crystals by Strong Coupling

Author(s): Fatemeh Davoodi, Masoud Taleb, Florian K. Diekmann, Toon Coenen, Kai Rossnagel, and Nahid Talebi
Published in: ACS Photonics, 2022, ISSN 2330-4022
Publisher: American Chemical Society
DOI: 10.1021/acsphotonics.2c00586

Mapping optical Bloch modes of a plasmonic square lattice in real and reciprocal spaces using cathodoluminescence spectroscopy

Author(s): Paul H. Bittorf, Fatemeh Davoodi, Masoud Taleb, and Nahid Talebi
Published in: Optics Express, 2021, ISSN 1094-4087
Publisher: Optical Society of America
DOI: 10.1364/oe.437984

Revealing Nanoscale Confinement Effects on Hyperbolic Phonon Polaritons with an Electron Beam

Author(s): A. Konečná, J. Li, J. H. Edgar, F. J. García de Abajo, and J. A. Hachtel
Published in: Small, 2021, ISSN 1613-6810
Publisher: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/smll.202103404

Tailoring near-field-mediated photon electron interactions with light polarization

Author(s): Fatemeh Chahshouri, Nahid Talebi
Published in: New Journal of Physics, 2023, ISSN 1367-2630
Publisher: Institute of Physics Publishing
DOI: 10.1088/1367-2630/acb4b7

Optical polarization analogue in free electron beams

Author(s): Lourenco-Martins, H.; Gerard, D. and Kociak, M.
Published in: Nature Physics, 2021, ISSN 1745-2473
Publisher: Nature Publishing Group
DOI: 10.1038/s41567-021-01163-w

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