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Ultrafast topological engineering of quantum materials

Project description

Exploring non-equilibrium topological phases in trivial materials

Topological materials can be insulating in bulk but have conductive surface states owing to symmetry-protected topological order. Comprising electronic states that are protected against perturbation, this class of materials shows high promise for use in dissipationless electronics and fault-tolerant quantum computers. Topological insulators could be switched from a non-conducting state to a conducting state using light pulses. Light pulses could also help stabilise non-equilibrium topological phases in trivial materials. However, real-time monitoring of ultrafast, non-equilibrium topological phase transitions is challenging. The ERC-funded UTOPIQ project will use tailored femtosecond pulses with peculiar symmetries to induce ultrafast electronic dynamics leading to topological phase transitions in 2D materials. The non-equilibrium electronic band structure of photoexcited 2D quantum materials will be measured using time-, angle- and polarisation-resolved spectroscopy.

Objective

Topological phases of matter emerge from the interplay between broken symmetries and many-body physics and exhibit many fascinating quantum phenomena. Ultrafast switching between different topological phases using light pulses holds the promise for disruptive optoelectronic functionalities, like dissipationless and fault-tolerant logical operations. However, the lack of proper observable being simultaneously sensitive to the local (in momentum-space) topology of the band structure and compatible with time-resolved measurements prevents the real-time monitoring of ultrafast non-equilibrium topological phase transitions.

I will address this fundamental challenge by introducing innovative control and measurement methodologies using tailored light pulses in time-, angle- and polarization-resolved extreme ultraviolet photoemission spectroscopy. This approach will enable to follow the ultrafast evolution of the electronic band structures local topology, in photoexcited quantum materials. This will represent a major advance in photoemission spectroscopy, by moving from band structure mapping to accessing the dynamical evolution of the Bloch wavefunction of solids.

I will use these novel time- and quantum-state-resolved dichroic observables to investigate the rich non-equilibrium physics underlying ultrafast topological phase transitions occurring on various timescales following impulsive optical excitation using shaped pump pulses: i) during the formation of hybrid light-matter (Floquet-Bloch) states, ii) upon the transient modification of electronic correlations, and iii) following the excitation of coherent phonon modes. UTOPIQ will deliver a dramatically improved understanding of the interplay between the non-equilibrium behaviour and non-trivial topology in photoexcited quantum materials, while further representing a decisive step towards the development of the field of ultrafast on demand topology.

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Programme(s)

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Topic(s)

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Funding Scheme

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HORIZON-ERC - HORIZON ERC Grants

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Call for proposal

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(opens in new window) ERC-2022-STG

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Host institution

CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 1 595 671,50
Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 1 754 304,00

Beneficiaries (2)

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