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A holistic approach to bridge the gap between microsecond computer simulations and millisecond biological events

Project description

Smart data-driven techniques to model how biological molecules function

Biological motors, such as the V1Vo-ATPase, are molecular machines found in living cells that convert chemical energy into mechanical work with remarkable efficiency. However, understanding the atomic-level picture of their millisecond transitions between functional states is challenging owing to computational limitations. The ERC-funded MilliInMicro project proposes a holistic approach to bridge microsecond simulations with millisecond-scale biological processes. Researchers will use data-driven methods to determine key reaction coordinates with advanced algorithms for mapping free-energy pathways. They will also accelerate the process of exploring these pathways using advanced methods that map complex energy landscapes much faster than existing techniques. Project findings could illuminate the effects of disease-causing mutations and guide the design of artificial cells.

Objective

Complete understanding of how complex biological objects operate and fulfill their cellular role requires at its core a detailed picture of the millisecond (ms) conformational transitions between functional states. Computational investigation of such ms–events is thwarted by our difficulty—and often impossibility—to identify and sample efficiently the relevant degrees of freedom at play, as well as the current limitation of all-atom molecular dynamics to the microsecond (μs) timescale on common computer architectures. Guided by concrete biological questions that experiment alone has hitherto proven unable to address, we propose a holistic approach to bridge affordable μs–computer simulations and ms–biological processes without the aid of a special-purpose supercomputer. To meet this grand theoretical challenge, we will associate two powerful developments to make the quantum leap, and open a breadth of applications, scaling up to very large biological objects, so far inaccessible to μs–timescale computer simulations. First, we will determine the reaction coordinate in an unprecedented combination of data- driven discovery of collective variables and advanced algorithms to find the minimum free-energy pathway that connects the end states of the conformational transition. Second, we will accelerate sampling along this pathway by associating ergodic schemes to a novel approach that maps complex free-energy landscapes significantly faster than its competitors. We will apply this methodology to a V1Vo–ATPase, a complete ATP–driven biological motor that converts over the ms–timescale the chemical energy of ATP hydrolysis into mechanical work, with minimalist dissipation. Beyond illuminating the allosteric pathways that underlie the conformational transition, atomic-level description of the rotary-catalysis milestones will shed new light on the effects of pathological mutations altering ATP activity, while helping engineer artificial cells with accelerated ATP turnover.

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(opens in new window) ERC-2022-ADG

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Host institution

CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 2 134 529,00
Address
RUE MICHEL ANGE 3
75794 PARIS
France

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Region
Ile-de-France Ile-de-France Paris
Activity type
Research Organisations
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 2 134 529,00

Beneficiaries (1)

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