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Engineering Metal-Organic Framework-Polymer Binder Interfaces for Carbon Capture

Project description

Metal-organic frameworks and binder composites development

To reduce CO2 emissions, large-scale carbon capture technologies are essential, often relying on porous metal-organic frameworks (MOFs). Typically available in small forms, MOFs need shaping with polymer binders to function effectively in adsorption systems. However, current design practices lack clear guidelines. Supported by the Marie Skłodowska-Curie Actions programme, the MOFBINDER project will develop a computational method to design MOF-binder composites with improved mechanical properties and controlled porosity. By combining parallel molecular simulations and machine learning applied to both simulated and existing data, the project aims to establish an efficient screening process. This work will also integrate with the process-informed design of tailor-made sorbent materials platform, which links material design, process optimisation, techno-economics, and life-cycle assessment.

Objective

Reducing CO2 emissions urgently requires the deployment of large-scale carbon capture technologies, many of which are being developed using innovative materials like porous metal-organic frameworks (MOFs). However, MOFs are typically synthesized as small crystals or powders, making them unsuitable for adsorption systems due to the high-pressure drops caused by fine particles. To address this issue, MOFs must be shaped into larger particles using polymer binders. While studies have explored MOF materials combined with binders, no clear guidelines exist, and the design process is often based on trial and error.

This project aims to develop a computational approach for designing MOF-binder composites with enhanced mechanical properties and controlled porosity. By utilizing parallel molecular simulations, we will predict the interface properties in a high-throughput manner. Machine learning techniques, drawing from both simulated and literature-mined data, will enable the development of a robust screening method. Additionally, our work will be integrated with the state-of-the-art Process-Informed design of tailor-made Sorbent Materials (PrISMa) platform, which connects material design, process optimization, techno-economics, and life-cycle assessment. This integration will allow for the evaluation and comparison of MOF formulations in terms of their greenhouse gas emissions throughout the lifecycle of the carbon capture plant, addressing one of the final steps in the deployment of carbon capture technologies.

To achieve these goals, the Researcher will receive training in high-throughput atomistic simulation workflows, materials informatics, and machine learning for material discovery, along with a holistic engineering approach through PrISMa. Moreover, this project offers the Researcher the opportunity to apply her expertise to the field of composite design, bridging fundamental science with industry-oriented perspectives actively pursued at IMDEA Materials Institute

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Topic(s)

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HORIZON-TMA-MSCA-PF-EF - HORIZON TMA MSCA Postdoctoral Fellowships - European Fellowships

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Call for proposal

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(opens in new window) HORIZON-MSCA-2024-PF-01

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Coordinator

FUNDACION IMDEA MATERIALES
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 194 074,56
Address
CALLE ERIC KANDEL 2 PARQUE CIENTIFICO Y TECNOLOGICO TECNOGETAFE
28906 Getafe
Spain

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Region
Comunidad de Madrid Comunidad de Madrid Madrid
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Research Organisations
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