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Real-time nanoscale manipulation of structure and environment to understand light-harvesting regulation in photosynthesis

Project description

New approach to study light-harvesting complexes in plants

Plants rely on light-harvesting complexes (LHC) to fuel photosynthesis and safely vent excess energy as heat, shielding delicate tissues from light-induced stress. However, it is not clear what triggers the protective switch in LHCs due to limited experimental tools in the field. The ERC-funded MARIONETTE project aims to fill this knowledge gap by using a variety of novel methodologies and solutions to overcome previous limitations in the study of LHCs. Specifically, it will use single-molecule optical tweezers resolved in force and fluorescence, a novel ultrafast multipulse spectroscopic tool, and integrate ad hoc molecular dynamics simulations to advance and deepen our understanding.

Objective

Sunlight is a source of life for plants but also of photodamage. To harvest solar energy “safely”, plants have developed a nanoscale mechanism controlled by small proteins which bind pigments, called light-harvesting complexes (LHCs). At low light intensities, the LHCs harvest and transport solar energy to the sites of photochemistry. Under intense light, LHCs switch function to dissipate excess energy as heat. Through this photoprotective switch, the LHCs efficiently protect plants from photodamage.
Yet, how do plants activate the LHC photoprotective switch? Current models assume that the switch is driven by protein conformational changes of the LHCs, regulated by the environment through pH changes and interactions with protein and cofactors. However, no experimental tool implemented in the field of photosynthesis allows to identify the conformational changes responsible of photoprotection and to determine how the environment controls them – limiting our mechanistic understanding of light-harvesting regulation in plants.
I will tackle this challenge by:
1) Pioneering the study of LHC nanomechanics via single-molecule optical tweezers, resolved in force and fluorescence, to track LHC conformational changes at single-residue level and identify those driving the photoprotective switch.
2) Leveraging a novel ultrafast multipulse spectroscopic tool — just developed by my group — to rapidly control environmental changes and determine the intermediate steps in the photoprotective switch of the LHCs.
3) Integrating ad hoc molecular dynamics simulations to map how external physiological factors tune the conformational landscape of the LHCs.
By implementing a novel optical and computational toolkit, I will advance our understanding of how plants regulate light harvesting at the nanoscale, while establishing a new framework in photosynthesis and photobiology to determine how structure and environment control the function of photosensory proteins across all life domains.

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(opens in new window) ERC-2025-STG

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Host institution

FUNDACIO INSTITUT DE CIENCIES FOTONIQUES
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 2 174 716,00
Address
AVINGUDA CARL FRIEDRICH GAUSS 3
08860 Castelldefels
Spain

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Region
Este Cataluña Barcelona
Activity type
Research Organisations
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 2 174 716,00

Beneficiaries (1)

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