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In Silico Photochemistry of Atmospheric Molecules in Aqueous Aerosols

Project description

Shedding more light on aerosol photochemistry

The chemistry of our atmosphere is more complex than it seems. While volatile organic compounds (VOCs) are known to react with sunlight to form secondary pollutants, recent discoveries reveal that aqueous aerosols – tiny water-containing particles in the air – play a significantly bigger role. These aerosols act as miniature chemical reactors, altering how VOCs interact with sunlight and potentially accelerating the formation of secondary organic aerosols, which contribute to air pollution and climate change. Despite its vast influence, the impact of photochemistry in aqueous aerosols is mostly ignored by current atmospheric models. The ERC-funded ISPAMIA project aims to fill that gap. Researchers will develop a global understanding of photochemical reactions in aqueous aerosols by exploiting recent breakthroughs in computational chemistry.

Objective

Our atmosphere is not only composed of simple di- or triatomic molecules, but also of volatile organic compounds (VOCs) that can undergo chemical or photochemical reactions following sunlight absorption to produce even more complex molecules responsible for the appearance of secondary pollutants. Yet, this ‘gas-phase’ picture of atmospheric chemistry has recently been challenged by the realization that aqueous aerosols – water microdroplets or other hygroscopic atmospheric aerosols with a water layer – act as true miniature chemical reactors and alter the sunlight-induced photochemical reactivity of VOCs. Aqueous aerosols are also suspected to catalyze the formation of secondary organic aerosols, strong contributors to radiative forcing and air pollution. Given that the total surface area of aerosols in the atmosphere is greater than the combined surface area of all bodies of water on Earth, the influence of aerosol photochemistry can be tremendous on the composition of our atmosphere. Still, the impact of aqueous aerosols on photochemical processes is completely neglected in most chemical models used by atmospheric modelers to predict the evolution and composition of the atmosphere, as well as inform political decisions on pollution management. This lack of knowledge is rooted in the challenge of performing photochemical experiments in aqueous aerosols and the absence of a theoretical framework to model such photochemical processes in complex environments.
This project, ISPAMIA, launches the field of in silico aerosol photochemistry and will develop a global understanding of photochemical reactions in aqueous aerosols by exploiting our recent breakthroughs in theoretical/computational chemistry. ISPAMIA goes beyond pure theoretical curiosity as it aims to calculate actual photochemical observables and determine simple rules that can be included in atmospheric models in collaboration with atmospheric scientists to achieve, ultimately, a direct social impact.

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HORIZON-ERC - HORIZON ERC Grants

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(opens in new window) ERC-2025-COG

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Host institution

UNIVERSITY OF BRISTOL
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 2 200 250,00
Address
BEACON HOUSE QUEENS ROAD
BS8 1QU BRISTOL
United Kingdom

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Region
South West (England) Gloucestershire, Wiltshire and Bristol/Bath area Bristol, City of
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 2 200 250,00

Beneficiaries (1)

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