Objective
To address climate change and achieve carbon neutrality, innovative technologies are needed to convert CO2 into fuels and chemicals. Among the several strategies, the direct conversion of CO2 and green H2 into fuel-range hydrocarbons (C5+) presents a sustainable alternative to fossil-based processes, ensuring energy security, especially in hard-to-electrify sectors such as shipping and aviation. In general, this tandem process through the RWGS-FT pathway demands at least two different types of active sites in a catalytic system for the formation of primary intermediate CO and subsequent consumption through C-C coupling and chain growth. Although Fe, Co, and Ru-based nanomaterials are well studied for this process, they have critical limitations, including low CO formation, limited C5+ selectivity, and insufficient activity under mild conditions.
The core of this proposal is to construct single-atom sites (Fe or Co) within doped/co-doped carbon that combines the advantages of single-metal dispersion for *CO formation and stabilization and dynamic aggregation and carburization under reaction conditions for obtaining high C5+ selectivity. Therefore, this research will focus on tailoring the coordination environment at the atomic scale for achieving C5+ selectivity beyond the ASF limit (48%).
This work will adopt a multidisciplinary approach, integrating a simple catalyst synthesis strategy with advanced characterization and in-situ/operando spectroscopy studies. Special attention will be given to probe dynamic structural and electronic changes under reaction conditions. By establishing a structure-activity relationship, fundamental insights into how a single site and its structural evolution affect the catalytic performance will be achieved.
The expected outcome of this project is to develop a robust and scalable single-atom catalyst for CO2 valorization, contributing to the EU's Green Deal goal and enhancing researchers’ skills in both catalysis and leadership.
Fields of science (EuroSciVoc)
CORDIS classifies projects with EuroSciVoc, a multilingual taxonomy of fields of science, through a semi-automatic process based on NLP techniques. See: The European Science Vocabulary.
CORDIS classifies projects with EuroSciVoc, a multilingual taxonomy of fields of science, through a semi-automatic process based on NLP techniques. See: The European Science Vocabulary.
- natural sciences chemical sciences organic chemistry hydrocarbons
- natural sciences chemical sciences catalysis
- engineering and technology nanotechnology nano-materials
- engineering and technology environmental engineering energy and fuels
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Keywords
Project’s keywords as indicated by the project coordinator. Not to be confused with the EuroSciVoc taxonomy (Fields of science)
Project’s keywords as indicated by the project coordinator. Not to be confused with the EuroSciVoc taxonomy (Fields of science)
Programme(s)
Multi-annual funding programmes that define the EU’s priorities for research and innovation.
Multi-annual funding programmes that define the EU’s priorities for research and innovation.
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HORIZON.1.2 - Marie Skłodowska-Curie Actions (MSCA)
MAIN PROGRAMME
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Topic(s)
Calls for proposals are divided into topics. A topic defines a specific subject or area for which applicants can submit proposals. The description of a topic comprises its specific scope and the expected impact of the funded project.
Calls for proposals are divided into topics. A topic defines a specific subject or area for which applicants can submit proposals. The description of a topic comprises its specific scope and the expected impact of the funded project.
Funding Scheme
Funding scheme (or “Type of Action”) inside a programme with common features. It specifies: the scope of what is funded; the reimbursement rate; specific evaluation criteria to qualify for funding; and the use of simplified forms of costs like lump sums.
Funding scheme (or “Type of Action”) inside a programme with common features. It specifies: the scope of what is funded; the reimbursement rate; specific evaluation criteria to qualify for funding; and the use of simplified forms of costs like lump sums.
HORIZON-TMA-MSCA-PF-EF - HORIZON TMA MSCA Postdoctoral Fellowships - European Fellowships
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Call for proposal
Procedure for inviting applicants to submit project proposals, with the aim of receiving EU funding.
Procedure for inviting applicants to submit project proposals, with the aim of receiving EU funding.
(opens in new window) HORIZON-MSCA-2025-PF
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Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.
CF10 3AT CARDIFF
United Kingdom
The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.