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Tandem Catalysts Design towards Efficient Selective Capture and Conversion of CO2

Project description

A single process to capture and convert carbon dioxide into valuable resources

Conventional methods to capture and recycle carbon dioxide require separate, energy-intensive steps for gas compression and material regeneration. Supported by the Marie Skłodowska-Curie Actions programme, the TCatSCC project will develop a new approach to bypass these high costs. The proposed approach merges gas capture and chemical conversion into a single, seamless process using bifunctional metal-organic frameworks. These specially engineered crystalline materials feature built-in adsorption sites and catalytic species, enabling energy-efficient carbon dioxide hydrogenation at low temperatures and pressures. Researchers will combine advanced synthesis methods with real-time microscopic tracking to uncover how these materials function. This catalysis technique aims to deliver scalable, cost-effective technologies that convert greenhouse gases into valuable resources.

Objective

This proposal will develop bifunctional metal-organic frameworks (MOFs) catalysts that integrate carbon dioxide (CO2) selective capture and conversion (CO2-SCC) into a single process, avoiding high energy penalties for CO2 compression and sorbent regeneration, kinetic mismatches, and costs of conventional, separate steps. By combining engineered adsorption sites with catalytic species, the catalysts will enable low-temperature, low-pressure hydrogenation with exceptional energy efficiency. An interdisciplinary approach – spanning advanced synthesis, state-of-the-art characterization, and operando mechanistic studies – will deliver fundamental insights into thermally catalyzed CO2-SCC and guide the rational design of future materials. The outcomes will advance scalable, cost-effective CO2 valorization technologies, directly supporting EU Green Deal targets, fostering innovation in sustainable catalysis, and strengthening Europe’s leadership in climate-neutral technologies.

Fields of science (EuroSciVoc)

Programme(s)

Topic(s)

Funding Scheme

HORIZON-TMA-MSCA-PF-EF - HORIZON TMA MSCA Postdoctoral Fellowships - European Fellowships

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Call for proposal

(opens in new window) HORIZON-MSCA-2025-PF

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Coordinator

KATHOLIEKE UNIVERSITEIT LEUVEN
Net EU contribution
€ 200 400,00
Address
OUDE MARKT 13
3000 Leuven
Belgium
Region
Vlaams Gewest Prov. Vlaams-Brabant Arr. Leuven
Activity type
Higher or Secondary Education Establishments
Links
Total cost
No data