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Monomer sequence control in Polymers : Toward next-generation precision materials

Deliverables

8 publications from WP5 ESRs

8 publications from WP5 ESRs of which at least 3 of them will be jointly with WP2/3/4

Final report

Final report

12 Publications from WP3 ESRs

12 Publications from WP3 ESRs of which at least 4 will be jointly with WP2 and WP5

12 publications from WP2 ESRs

12 publications from WP2 ESRs of which at least 6 will be jointly with WP4 and WP5

Outreach activities

Outreach activities

Kick-off meeting

Kick off meeting

At least one patent application on a new technology developed in this project

At least one patent application on a new technology developed in this project

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Publications

PEGylated Precision Segments Based on Sequence-Defined Thiolactone Oligomers

Author(s): Sensu Celasun, Filip E. Du Prez, Hans G. Börner
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700688, ISSN 1022-1336
DOI: 10.1002/marc.201700688

Cooperative Folding of Linear Poly(dimethyl siloxane)s via Supramolecular Interactions

Author(s): Marcin L. Ślęczkowski, E. W. Meijer, Anja R. A. Palmans
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700566, ISSN 1022-1336
DOI: 10.1002/marc.201700566

Tailored Modification of Thioacrylates in a Versatile, Sequence-Defined Procedure

Author(s): Joshua O. Holloway, Suzan Aksakal, Filip E. Du Prez, C. Remzi Becer
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700500, ISSN 1022-1336
DOI: 10.1002/marc.201700500

Click and Click-Inspired Chemistry for the Design of Sequence-Controlled Polymers

Author(s): Steven Martens, Joshua O. Holloway, Filip. E. Du Prez
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700469, ISSN 1022-1336
DOI: 10.1002/marc.201700469

Translocation of Precision Polymers through Biological Nanopores

Author(s): Mordjane Boukhet, Niklas Felix König, Abdelaziz Al Ouahabi, Gerhard Baaken, Jean-François Lutz, Jan C. Behrends
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700680, ISSN 1022-1336
DOI: 10.1002/marc.201700680

Photocontrolled Synthesis of Abiotic Sequence-Defined Oligo(Phosphodiester)s

Author(s): Niklas Felix König, Sofia Telitel, Salomé Poyer, Laurence Charles, Jean-François Lutz
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700651, ISSN 1022-1336
DOI: 10.1002/marc.201700651

Sequence Controlled Polymers from a Novel β-Cyclodextrin Core

Author(s): Yamin Abdouni, Gökhan Yilmaz, C. Remzi Becer
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700501, ISSN 1022-1336
DOI: 10.1002/marc.201700501

Sequence and Architectural Control in Glycopolymer Synthesis

Author(s): Yamin Abdouni, Gokhan Yilmaz, C. Remzi Becer
Published in: Macromolecular Rapid Communication, 2017, Page(s) 229-256, ISSN 1022-1336
DOI: 10.1002/9783527806096.ch8

Negative mode MS/MS to read digital information encoded in sequence-defined oligo(urethane)s: A mechanistic study

Author(s): Jean-Arthur Amalian, Salomé Poyer, Benoit Eric Petit, Sofia Telitel, Valérie Monnier, Denise Karamessini, Didier Gigmes, Jean-François Lutz, Laurence Charles
Published in: International Journal of Mass Spectrometry, Issue 421, 2017, Page(s) 271-278, ISSN 1387-3806
DOI: 10.1016/j.ijms.2017.07.006

2D Sequence-Coded Oligourethane Barcodes for Plastic Materials Labeling

Author(s): Denise Karamessini, Salomé Poyer, Laurence Charles, Jean-François Lutz
Published in: Macromolecular Rapid Communications, Issue 38/24, 2017, Page(s) 1700426, ISSN 1022-1336
DOI: 10.1002/marc.201700426

Cleavable Binary Dyads: Simplifying Data Extraction and Increasing Storage Density in Digital Polymers

Author(s): Gianni Cavallo, Salomé Poyer, Jean-Arthur Amalian, Florent Dufour, Alexandre Burel, Christine Carapito, Laurence Charles, Jean-François Lutz
Published in: Angewandte Chemie International Edition, Issue 57/21, 2018, Page(s) 6266-6269, ISSN 1433-7851
DOI: 10.1002/anie.201803027

Digging into the Sequential Space of Thiolactone Precision Polymers: A Combinatorial Strategy to Identify Functional Domains

Author(s): Sensu Celasun, Dario Remmler, Timm Schwaar, Michael G. Weller, Filip Du Prez, Hans G. Börner
Published in: Angewandte Chemie International Edition, Issue 58/7, 2019, Page(s) 1960-1964, ISSN 1433-7851
DOI: 10.1002/anie.201810393

Thioester functional polymers

Author(s): Suzan Aksakal, Resat Aksakal, C. Remzi Becer
Published in: Polymer Chemistry, Issue 9/36, 2018, Page(s) 4507-4516, ISSN 1759-9954
DOI: 10.1039/c8py00872h

Abiotic Sequence-Coded Oligomers as Efficient In Vivo Taggants for the Identification of Implanted Materials

Author(s): Denise Karamessini, Teresa Simon-Yarza, Salomé Poyer, Evgeniia Konishcheva, Laurence Charles, Didier Letourneur, Jean-François Lutz
Published in: Angewandte Chemie International Edition, Issue 57/33, 2018, Page(s) 10574-10578, ISSN 1433-7851
DOI: 10.1002/anie.201804895

Elements of fractal geometry in the 1 H NMR spectrum of a copolymer intercalation-complex: identification of the underlying Cantor set

Author(s): John S. Shaw, Rajendran Vaiyapuri, Matthew P. Parker, Claire A. Murray, Kate J. C. Lim, Cong Pan, Marcus Knappert, Christine J. Cardin, Barnaby W. Greenland, Ricardo Grau-Crespo, Howard M. Colquhoun
Published in: Chemical Science, Issue 9/17, 2018, Page(s) 4052-4061, ISSN 2041-6520
DOI: 10.1039/c8sc00830b

Translocation of Sequence-Controlled Synthetic Polymers through Biological Nanopores

Author(s): Mordjane Boukhet, Niklas F. König, Abdelaziz Al Ouahabi, Gerhard Baaken, Jean-François Lutz, Jan C. Behrends
Published in: Biophysical Journal, Issue 114/3, 2018, Page(s) 182a, ISSN 0006-3495
DOI: 10.1016/j.bpj.2017.11.1013

Synthesis of Macromolecules Containing Phenylalanine and Aliphatic Building Blocks

Author(s): Delphine Chan-Seng, Jeroen Louwsma, Jean-François Lutz, Stéphane Joly
Published in: Macromolecular Rapid Communications, Issue 39/8, 2018, Page(s) 1700764, ISSN 1022-1336
DOI: 10.1002/marc.201700764

Poly(thioacrylate)s: expanding the monomer toolbox of functional polymers

Author(s): Suzan Aksakal, C. Remzi Becer
Published in: Polym. Chem., Issue 7/45, 2016, Page(s) 7011-7018, ISSN 1759-9954
DOI: 10.1039/C6PY01721E

Identification-Tagging of Methacrylate-Based Intraocular Implants Using Sequence Defined Polyurethane Barcodes

Author(s): Denise Karamessini, Benoit Eric Petit, Michel Bouquey, Laurence Charles, Jean-Fran?ois Lutz
Published in: Advanced Functional Materials, Issue 27/3, 2017, Page(s) 1604595, ISSN 1616-301X
DOI: 10.1002/adfm.201604595

Controlling the structure of sequence-defined poly(phosphodiester)s for optimal MS/MS reading of digital information

Author(s): Jean-Arthur Amalian, Abdelaziz Al Ouahabi, Gianni Cavallo, Niklas Felix K?nig, Salom? Poyer, Jean-Fran?ois Lutz, Laurence Charles
Published in: Journal of Mass Spectrometry, 2017, ISSN 1076-5174
DOI: 10.1002/jms.3947

MS/MS-Assisted Design of Sequence-Controlled Synthetic Polymers for Improved Reading of Encoded Information

Author(s): Laurence Charles, Gianni Cavallo, Val?rie Monnier, Laurence Oswald, Roza Szweda, Jean-Fran?ois Lutz
Published in: Journal of The American Society for Mass Spectrometry, Issue 28/6, 2017, Page(s) 1149-1159, ISSN 1044-0305
DOI: 10.1007/s13361-016-1543-5

A Simple Post-Polymerization Modification Method for Controlling Side-Chain Information in Digital Polymers

Author(s): Niklas Felix König, Abdelaziz Al Ouahabi, Salomé Poyer, Laurence Charles, Jean-François Lutz
Published in: Angewandte Chemie International Edition, Issue 56/25, 2017, Page(s) 7297-7301, ISSN 1433-7851
DOI: 10.1002/anie.201702384

Chemoselective Synthesis of Uniform Sequence-Coded Polyurethanes and Their Use as Molecular Tags

Author(s): Ufuk?Saim Gunay, Beno?t?Eric Petit, Denise Karamessini, Abdelaziz Al?Ouahabi, Jean-Arthur Amalian, Christophe Chendo, Michel Bouquey, Didier Gigmes, Laurence Charles, Jean-Fran?ois Lutz
Published in: Chem, Issue 1/1, 2016, Page(s) 114-126, ISSN 2451-9294
DOI: 10.1016/j.chempr.2016.06.006

Orthogonal Synthesis of ?Easy-to-Read? Information-Containing Polymers Using Phosphoramidite and Radical Coupling Steps

Author(s): Gianni Cavallo, Abdelaziz Al Ouahabi, Laurence Oswald, Laurence Charles, Jean-Fran?ois Lutz
Published in: Journal of the American Chemical Society, Issue 138/30, 2016, Page(s) 9417-9420, ISSN 0002-7863
DOI: 10.1021/jacs.6b06222

Coding in 2D: Using Intentional Dispersity to Enhance the Information Capacity of Sequence-Coded Polymer Barcodes

Author(s): Chlo? Laure, Denise Karamessini, Olgica Milenkovic, Laurence Charles, Jean-Fran?ois Lutz
Published in: Angewandte Chemie International Edition, Issue 55/36, 2016, Page(s) 10722-10725, ISSN 1433-7851
DOI: 10.1002/anie.201605279

Click and Click‐Inspired Chemistry for the Design of Sequence‐Controlled Polymers

Author(s): Steven Martens, Joshua O. Holloway, Filip E. Du Prez
Published in: Sequence‐Controlled Polymers, 2017, Page(s) 379-416
DOI: 10.1002/9783527806096.ch13