Cement-based materials, properties, evolution, barrier functions

Resultado final

Manuscript for peer-reviewed publication on results generated within WP3
Detailed WP1 description of scientific work: compilation of partner descriptions with update of Appendix_B
Draft of the 4th and final project workshop proceedings

Draft of the 4th and final project Workshop proceedings

Planning on interaction with socio-political stakeholders
Report (with update) on basis for application to Safety Case

Report (with update) on Basis for application to Safety Case. This Report will be updated in Project month 36 and 48

Report on WP1 established experimental boundary conditions, experimental methods
State-of-art report related to WP2 topics (updated)
Planned dissemination of final results
Detailed WP3 description of scientific work: compilation of partner descriptions with update of Appendix_B
Final results and interpretation of the modelling by incorporating results from WP1&WP2 experiments

Final results and interpretation of the modelling by incorporating results from WP&WP2 experiments

Report on interaction with non-scientific stakeholder
Manuscript for peer-reviewed publication on results generated in WP1
Manuscript for peer-reviewed publication on results generated within WP2
State-of-art report related to WP2 topics (initial)
Draft of the 3rd Annual Project Workshop Proceedings
List of mobility measures and summary of the works undertaken
Report/Documentation of exchange of data between experimental and modelling WPs (with updating)

This deliverable will be updated in month 26, 38 and 48

State-of-art report related to WP1 topics (updated)
Consolidated plan for Upscaling Modelling Task
Agreement and documentation of systems to be studied (WP1)

Agreement and documentation of systems to be studied

Periodic management and activity reports

Periodic Management and activity Report. This deliverable will be updated in Project month 36 and 48

Draft of the 2nd Annual Project Workshop Proceedings
Preliminary results and interpretation of the modelling by incorporating results from WP1&WP2 experiments
Agreement and documentation of systems to be studied (WP2)

Agreement and documentation of systems to be studied

State-of-art report related to WP1 topics (initial)
Draft of the 1st Annual project Workshop Proceedings

Draft of the 1st Annual Workshop Proceedings

Review and definition of modelling approach to be followed in the project: scale of analysis, physico-chemical processes, software, HPC resources
Report on the Upscaling Modelling Task
Report on new data (sorption, speciation, solubility) for radionuclide retention generated in WP2 (with updating)

Report on new data (sorption, speciation, solubility) for radionuclide Retention generated in WP2 (with updating)

Report on the relevance of the outcome of Cebama for the Safety Case (Manuscript for peer-reviewed publication)
Detailed WP2 description of scientific work: compilation of partner descriptions with update of Appendix B
Minutes from 2nd Annual Workshop
Report on WP1 selected experimental materials to be used, including both new laboratory and aged in-situ samples
Communication Action Plan
Description of and results from the modelling of external lab and/or field experiments and industrial analogues

Description of and results from the modelling of external lab and/or field experiments and industrial analogues.

Final project reporting, dissemination, communication, training & education, ethical/socio-political/broader stakeholder involvement

Final project reporting, dissemination, communication, Training & education, ethical/socio-political/broader stakeholder involvement

Final Report (EUR)

Final Report (EUR). Lead beneficiaries for this deliverable are KIT and AMPHOS21

Preparation of a generic poster presenting the project
Press release
Set up project webpage and blog

Publicaciones

Sorpce radia na vybrané cementové materiály/ Sorption of radium on cementitious materials (in Czech)

Autores: Jana Kittnerová
Publicado en: 2017
Editor: CTU in Prague, Faculty of Nuclear Sciences and Physical Engineering, Department of Nuclear Chemistry

Kinetics of low-pH cementitious materials in deep underground repository

Autores: Schmidt, Luisa
Publicado en: Master’s Thesis at the Technical University of Munich, Department of Civil, Geo, and Environmental Engineering, Chair of Material Science and Testing, Edición 1st of May, 2018, 2018
Editor: Technical University of Munich

Coupled thermo-hydro-chemical-mechanical models of the bentonite barrier in a HLW repository

Autores: Mon A.
Publicado en: Edición September 2017, 2017
Editor: UDC

Chemical behaviour of bentonite in the near field of the KBS-3V concept

Autores: Itälä Aku
Publicado en: Edición 2018-11-20, 2018, ISBN 978-951-38-8670-7
Editor: VTT Technical Research Centre of Finland

Comparison of experimental and modelled pore solutions of low-pH Ordinary Portland Cement based mix designs

Autores: Vehmas, T, Leivo, M & Holt, Erika
Publicado en: XXIII Nordic Concrete Research Symposium,, Edición 21 - 23 August 2017, Aalborg, Denmark, 2017, Página(s) 11-14
Editor: Nordic Concrete Federation

Cementitious leachates interaction with MX-80 bentonite in geological nuclear waste repository environment

Autores: Vehmas T., Itälä, A., Heikola, T., Leivo, M., Holt E., Vuorio, M
Publicado en: 7th International conference on clays in natural and engineered barriers for radioactive waste confinement, Edición 24th-27th of September 2017, 2017
Editor: Congrex Switzerland Ltd

Reactive Transport Modeling and Changes in Porosity at Reactive Interfaces in a HLW repository in Clay

Autores: J. Samper, A Mon, L Montenegro, A Naves & J Fernández
Publicado en: Book of Abstracts - Eos Trans. American Geophysical Union GU, Fall Meeting, 2016
Editor: American Geophysical Union

Coupled THCM numerical models of heating and hydration tests to study the interactions of OPC concrete with compacted FEBEX bentonite

Autores: J. Samper, A. Mon, L. Montenegro, A. Naves, J Fernández, J. Cuevas, R. Fernández, M.J. Turrero, E. Torres
Publicado en: Book of Abstracts - VII International Conference on Clays in Natural and Engineered Barriers for Radioactive Waste Confinement, Edición 24-27 September 2017, 2017, Página(s) 17-19
Editor: Clay Conference 2017

Long-term non-isothermal geochemical evolution of compacted bentonite, concrete and corrosion products in a HLW repository in clay

Autores: A. Mon, J. Samper, L. Montenegro, A. Naves, J Fernández
Publicado en: Book of Abstracts - VII International Conference on Clays in Natural and Engineered Barriers for Radioactive Waste Confinement, Edición 24-27 September 2017, 2017
Editor: Clay Conference 2017

Formation of magnesium sheet silicates as a consequence of the alkaline perturbation of a bentonite barrier

Autores: Fernández, R., González-Santamaría, D.1, Angulo, M., Torres, E.2, Ruiz, A.I., Turrero, M.J. and Cuevas, J.
Publicado en: The 7th International Conference on Clays in Natural and Engineered Barriers for radioactive waste confinement, Edición 24-27 September 2017, 2017
Editor: Book of abstracts

Concrete-bentonite interaction: comparing long-term laboratory tests (HB) and in situ experiments (FEBEX-DP)

Autores: E. Torres, J. Cuevas, R. Fernández, A.I. Ruiz, A. Ortega, M. Angulo, M.C. Alonso, J.L. García-Calvo, M.J. Turrero
Publicado en: The 7th International Conference on Clays in Natural and Engineered Barriers for radioactive waste confinement, 2017
Editor: Book of abstracts

Stable isotopes applied to the study of the concrete/bentonite interaction in the FEBEX in situ Test

Autores: E. Torres, M.J. Turrero, A. Garralón, J. Cuevas, R. Fernández, A. Ortega, A.I. Ruiz
Publicado en: The 7th International Conference on Clays in Natural and Engineered Barriers for radioactive waste confinement., 2017
Editor: Book of abstracts

SurfacE Reactivity Interface Experiments studying microscale concrete-bentonite interaction

Autores: Daniel González-Santamaría, Raúl Fernández, Ana Isabel Ruiz, María Angulo, Almudena Ortega, Enrique Rodríguez, Jaime Cuevas
Publicado en: 16th INTERNATIONAL CLAY CONFERENCE, clay from the oceans to the space, Edición 17-21 July 2017, 2017
Editor: Book of abstracts

An extended membrane polarization model for spectral induced polarization of low-pH cement and concrete

Autores: A. Hördt, M. Bücker, P. Leroy, S. Huisman, E. Zimmermann, S. Gaboreau, F. Claret, H. Stebner
Publicado en: European Geosciences Union General Assembly 2018, 2018
Editor: Book of abstracts

EVOLUTION OF MINERALOGY AND RADIONUCLIDE DIFFUSION ON PORTLANDTYPE CEMENTITIOUS MATERIALS DUE GEOCHEMICAL AND THERMAL EFFECTS

Autores: Tomáš ROSENDORF, Radek ČERVINKA, Dušan VOPÁLKA, Petr VEČERNÍK
Publicado en: RadChem - 18th Radiochemical Conference, 2018
Editor: Book of abstracts

Taking profit from molecular sensitivity on the macro scale: Application of PET for investigating transport processes in barrier material

Autores: Johannes Kulenkampff
Publicado en: European Geosciences Union General Assembly 2018, Edición 8- 13 April 2018, 2018
Editor: Proceedings

Experiments on a cement-clay interface and the impact on physical properties: The Dutch context

Autores: D. Bykov, A. Sabău, Y. Yigittop, J. L. Kloosterman, R. J. M. Konings, J. C. L. Meeussen
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 31
Editor: PSI-EMPA-UBERN

Kinetic parameters for assessing the pH –evolution of low pH concrete

Autores: Vehmas T., Leivo M., Holt E.
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 27
Editor: PSI-EMPA-UBERN

Impact of temperature on microstructure and transport properties of OPC paste / argilite interface

Autores: P. Lalan, A. Dauzères, L. De Windt, D. Bartier, J. Sammaljärvi, I. Techer, V. Detilleux
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 37
Editor: PSI-EMPA-UBERN

Cemtex project: Understand the physico-chemical evolution of cementitious material in clayey environment at 70°C

Autores: P. Lalan, A. Dauzères, L. De Windt, D. Bartier, J. Sammaljärvi, I. Techer
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 38
Editor: PSI-EMPA-UBERN

Changes in diffusion properties of cement paste induced by leaching and carbonation accounting for the effects of limestone fillers and water/powder ratio

Autores: Phung, Q. T., Maes, N., Jacops, E., Jacques, D., De Schutter, G.
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 98
Editor: PSI-EMPA-UBERN

Interaction processes at the concrete-bentonite interface after 13 years exposure of febex-plug. Part I Concrete alteration

Autores: MC Alonso, J.L. García-Calvo, J. Cuevas, M.J. Turrero, R. Fernández,E. Torres, A.I. Ruiz
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 29
Editor: PSI-EMPA-UBERN

Interaction processes at the concrete-bentonite interface after 13 years of FEBEX-Plug operation. Part II: Bentonite contact

Autores: Cuevas, J., Ruiz, A.I. Fernández, R.Torres, E., Alonso, M.C., García-Calvo, J.L. Aparicio, A., Turrero, M.J.
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 32
Editor: PSI-EMPA-UBERN

Uptake and retention of safety relevant radionuclides in cementitious systems.

Autores: Lange, S., Deissmann, G., Bosbach, D.
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 68
Editor: PSI-EMPA-UBERN

Solubility, hydrolysis and sorption of beryllium in cementitious systems

Autores: GAONA, X., BÖTTLE, M., RABUNG, Th., ALTMAIER, M.
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 57
Editor: PSI-EMPA-UBERN

Predicting long term interactions between concrete and boom clay with a reactive transport model

Autores: Meeussen, J. C. L., Koenen, M., Griffioen, J.
Publicado en: Book of abstracts - 4th International Workshop on Mechanisms and Modelling of Waste/Cement Interactions, 2016, Página(s) 41
Editor: PSI-EMPA-UBERN

Coupling thermodynamic modelling of cement hydration with moisture transfer. Application to low-pH cement systems.

Autores: A. Idiart, M. Laviña, J. Olmeda
Publicado en: International Symposium On Concrete Modelling, CONMOD2018, Edición August 2018, 2018
Editor: RILEM

Reactive transport modelling of cement hydration and degradation. Application to USFD experiments

Autores: M. Laviña, J. Olmeda, A. Idiart
Publicado en: Book of abstracts - 5th International Workshop on Mechanisms and Modelling of Waste / Cement Interactions, CEM2019, Edición March 2019, 2019
Editor: KIT

Molybdenum adsorption onto cement pure phases. The role of C-S-H and AFm phases

Autores: M. López-García, J. Olmeda, M. Grivé, P. Henoqc
Publicado en: Book of Abstracts - 5th International Workshop on Mechanisms and Modelling of Waste / Cement Interactions, Edición 25-27 March 2019, 2019
Editor: KIT

Molybdenum retention onto cement pastes and cement hydrate pure phases 1

Autores: M. López-García, M. Grivé, J. Olmeda, P. Henocq
Publicado en: 6th International Conference on the Chemistry and Migration Behaviour of Actinides and Fission Products in the Geosphere, Edición 10-15 September 2017, 2017
Editor: Amphos 21

Benchmark of reactive transport models within CEBAMA: application to a concrete / clay interface

Autores: A Idiart, M Laviña, V Montoya, G Kosakowski, B Cochepin, I Munier, J Samper, A Mon, L Montenegro, J Meeussen, G Deissmann, S Rohmen, J Poonoosamy
Publicado en: 9th European Commission Conference EURATOM Res. Training Radioactive Waste Management, EURADWASTE 2019, Edición June 2019, 2019
Editor: EURADWASTE

Pore-scale reactive transport modeling of degradation processes in cementitious systems: Concept development based on the Lattice-Boltzmann approach

Autores: S. Rohmen, A. Idiart, G. Deissmann, D. Bosbach
Publicado en: 9th International Conference on Porous Media & Annual Meeting, Interpore 2017, Edición May 2017, 2017
Editor: Interpore

Reactive transport processes at a low-pH concrete / clay interface: a benchmark modelling study

Autores: A Idiart, M Laviña, E Coene, V Montoya, G Kosakowski, B Cochepin, I Munier, J Samper, A Mon, J Meeussen, G Deissmann, S Rohmen, J Poonoosamy, D Vopálka
Publicado en: International Symposium On Cement-based Materials for Nuclear Wastes, NUWCEM 2018, Edición 24-26 October 2018, 2018
Editor: SFEN

Coupled thermo-hydro-chemical-mechanical model of shotcrete-bentonite interaction in FEBEX in situ test

Autores: Samper J., Mon A., Montenegro L.
Publicado en: Book of abstracts - 5th International Workshop on Mechanisms and Modelling of Waste / Cement Interactions, CEM2019, Edición March 2019, 2019
Editor: KIT

Coupled themo-hyodro-chemical-mechanical model of laboratory mortar-bentonite interaction tests

Autores: Samper, J., Mon A., Montenegro L.
Publicado en: Book of abstracts - 5th International Workshop on Mechanisms and Modelling of Waste / Cement Interactions, CEM2019, Edición March 2019, 2019
Editor: KIT

Reactive transport numerical predictions of the interactions of the bentonite with the concrete plug of the FEBEX in situ test

Autores: Samper, J., A. Mon, L. Montenegro
Publicado en: Book of Abstracts - VII International Conference on Clays in Natural and Engineered Barriers for Radioactive Waste Confinement, Edición 24-27 September 2017, 2017, Página(s) 514-515
Editor: Clay Conference 2017

Non-isothermal reactive transport model of the geochemical interactions of compacted bentonite, concrete and corrosion products in a radioactive waste repository in clay

Autores: Fernández, J., J. Samper, A. Mon, L. Montenegro
Publicado en: 45th IAH Congress. Groundwater and life, Edición 9-14 September 2018, 2018
Editor: IAH Congress

Non-isothermal benchmark of interactions of concrete, bentonite and clay

Autores: Mon A., Kosakowski G., Samper J., Montenegro L.
Publicado en: Book of Abstracts. International Workshop Subsurface Environmental Simulation Benchmarking Workshop V, A Coruña,, Edición October 2016, 2016, Página(s) 66-68, ISBN 978-84-617-5468-7
Editor: Tórculo

Ground wáter composition in the interaction with low-pH OPC-SF based concretes

Autores: M.C. Alonso, A. Fernandez and J.L. Garcia-Calvo
Publicado en: 3rd International Symposium on cement-based materials for nuclear wastes, Edición 2 years, 2019, Página(s) 48
Editor: CEA and SFEN

Thermodynamic and crystallographic model for anion uptake by hydrated calcium aluminate (AFm): an example of molybdenum

Autores: Nicolas C. M. Marty, Sylvain Grangeon, Erik Elkaïm, Christophe Tournassat, Clémence Fauchet, Francis Claret
Publicado en: Scientific Reports, Edición 8/1, 2018, ISSN 2045-2322
Editor: Nature Publishing Group
DOI: 10.1038/s41598-018-26211-z

Deciphering mineralogical changes and carbonation development during hydration and ageing of a consolidated ternary blended cement paste

Autores: Francis Claret, Sylvain Grangeon, Annick Loschetter, Christophe Tournassat, Wout De Nolf, Nicholas Harker, Faiza Boulahya, Stéphane Gaboreau, Yannick Linard, Xavier Bourbon, Alejandro Fernandez-Martinez, Jonathan Wright
Publicado en: IUCrJ, Edición 5/2, 2018, Página(s) 150-157, ISSN 2052-2525
Editor: International Union of Crystallography (IUCr)
DOI: 10.1107/s205225251701836x

Exploring the electrical potential inside cylinders beyond the Debye-Hückel approximation: a computer code to solve the Poisson-Boltzmann equation for multivalent electrolytes

Autores: Philippe Leroy, Alexis Maineult
Publicado en: Geophysical Journal International, 2018, ISSN 0956-540X
Editor: Geological Society by Blackwell Scientific
DOI: 10.1093/gji/ggy124

Modeling the evolution of complex conductivity during calcite precipitation on glass beads

Autores: Philippe Leroy, Shuai Li, Damien Jougnot, André Revil, Yuxin Wu
Publicado en: Geophysical Journal International, 2017, Página(s) ggx001, ISSN 0956-540X
Editor: Geological Society by Blackwell Scientific
DOI: 10.1093/gji/ggx001

Long-term non-isothermal reactive transport model of compacted bentonite, concrete and corrosion products in a HLW repository in clay

Autores: Alba Mon, Javier Samper, Luis Montenegro, Acacia Naves, Jesús Fernández
Publicado en: Journal of Contaminant Hydrology, Edición 197, 2017, Página(s) 1-16, ISSN 0169-7722
Editor: Elsevier BV
DOI: 10.1016/j.jconhyd.2016.12.006

Low-pH cement mortar-bentonite perturbations in a small-scale pilot laboratory experiment

Autores: D.E. González-Santamaría, M. Angulo, A.I. Ruiz, R. Fernández, A. Ortega, J. Cuevas
Publicado en: Clay Minerals, Edición 53/02, 2018, Página(s) 237-254, ISSN 0009-8558
Editor: Mineralogical Society
DOI: 10.1180/clm.2018.16

Characterisation of a high pH cement backfill for the geological disposal of nuclear waste: The Nirex Reference Vault Backfill

Autores: Vasconcelos, R.G.W.; Beaudoin, N.; Hamilton, A.; Hyatt, N.C.; Provis, J.L.; Corkhill, C.L.
Publicado en: Applied Geochemistry, 2018, ISSN 0883-2927
Editor: Pergamon Press Ltd.

PREPUBLICATION: Dissolution kinetics of hydrated calcium aluminates (AFm-Cl) as a function of pH and at room temperature

Autores: Marty, Nicolas C.M.1; Grangeon, Sylvain1; Lerouge, Catherine1; Warmont, Fabienne2; Rozenbaum, Olivier3; Conte, Thibaud1; Claret, Francis1
Publicado en: Mineralogical Magazine, 2016
Editor: Mineralogical Society
DOI: 10.1180/minmag.2016.080.161

Coupled THCM model of a heating and hydration concrete-bentonite column test

Autores: J. Samper, A. Mon, L. Montenegro, J. Cuevas, M.J. Turrero, A. Naves, R. Fernández, E. Torres
Publicado en: Applied Geochemistry, Edición 94, 2018, Página(s) 67-81, ISSN 0883-2927
Editor: Pergamon Press Ltd.
DOI: 10.1016/j.apgeochem.2018.05.007

Uptake of 226Ra in cementitious systems: A complementary solution chemistry and atomistic simulation study

Autores: Steve Lange, Piotr M. Kowalski, Milan Pšenička, Martina Klinkenberg, Stephan Rohmen, Dirk Bosbach, Guido Deissmann
Publicado en: Applied Geochemistry, Edición 96, 2018, Página(s) 204-216, ISSN 0883-2927
Editor: Pergamon Press Ltd.
DOI: 10.1016/j.apgeochem.2018.06.015

Authigenic Clay Minerals from Interface Reactions of Concrete-Clay Engineered Barriers: A New Perspective on Mg-Clays Formation in Alkaline Environments

Autores: Jaime Cuevas, Ana Ruiz, Raúl Fernández, Daniel González-Santamaría, María Angulo, Almudena Ortega, Elena Torres, María Turrero
Publicado en: Minerals, Edición 8/9, 2018, Página(s) 362, ISSN 2075-163X
Editor: MDPI
DOI: 10.3390/min8090362

Stable isotopes applied to the study of the concrete/bentonite interaction in the FEBEX in situ test

Autores: E. Torres, M.J. Turrero, A. Garralón, J. Cuevas, R. Fernández, A. Ortega, A.I. Ruíz
Publicado en: Applied Geochemistry, Edición 100, 2019, Página(s) 432-443, ISSN 0883-2927
Editor: Pergamon Press Ltd.
DOI: 10.1016/j.apgeochem.2018.12.017

Investigating the Potential Barrier Function of Nanostructured Materials Formed in Engineered Barrier Systems (EBS) Designed for Nuclear Waste Isolation

Autores: Jaime Cuevas, Ana Isabel Ruiz, Raúl Fernández
Publicado en: The Chemical Record, Edición 18/7-8, 2018, Página(s) 1065-1075
Editor: UAM-biblioteca peer rev unformatted
DOI: 10.1002/tcr.201700094

Geochemical conditions for the formation of Mg silicates phases in bentonite and implications for radioactive waste disposal

Autores: Fernández, Raúl; González-Santamaría, Daniel; Angulo, María; Torres, Elena; Ruiz, Ana Isabel; Turrero, María Jesús; Cuevas, Jaime
Publicado en: UAM_Biblioteca, 2018
Editor: UAM-biblioteca peer rev unformatted

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