An Artificial Leaf: a photo-electro-catalytic cell from earth-abundant materials for sustainable solar production of CO2-based chemicals and fuels

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A-LEAF Data Management plan

ALEAF Data Management plan and updates

A-LEAF Data Management plan - Update 12 months

A-LEAF Data Management plan and updates

A-LEAF Data Management plan - Update 24 months

A-LEAF Data Management plan and updates

A-LEAF Data Management plan - Update 36 months

A-LEAF Data Management plan and updates

A-LEAF Communication and Outreach plan - Update 24 months

A-LEAF Communication and Outreach plan and updates

A-LEAF Dissemination and Exploitation plan - Update 12 months

A-LEAF Dissemination and Exploitation plan and updates

A-LEAF Communication and Outreach plan

ALEAF Communication and Outreach plan and updates

A-LEAF Dissemination and Exploitation plan - Update 36 months

A-LEAF Dissemination and Exploitation plan and updates

A-LEAF Dissemination and Exploitation plan

ALEAF Dissemination and Exploitation plan and updates

A-LEAF Dissemination and Exploitation plan - Update 24 months

A-LEAF Dissemination and Exploitation plan and updates

A-LEAF Communication and Outreach plan - Update 12 months

A-LEAF Communication and Outreach plan and updates

A-LEAF Communication and Outreach plan - Update 36 months

A-LEAF Communication and Outreach plan and updates

RP2
RP3: Final report

RP3 Final report

RP1
Project management book

Web-Page and logo

WebPage and logo

Publicaciones

Atomic‐Scale Studies of Fe 3 O 4 (001) and TiO 2 (110) Surfaces Following Immersion in CO 2 ‐Acidified Water

Autores: Francesca Mirabella, Jan Balajka, Jiri Pavelec, Markus Göbel, Florian Kraushofer, Michael Schmid, Gareth S. Parkinson, Ulrike Diebold
Publicado en: ChemPhysChem, Edición 21/16, 2020, Página(s) 1788-1796, ISSN 1439-4235
Editor: John Wiley & Sons Ltd.
DOI: 10.1002/cphc.202000471

Volcano Trend in Electrocatalytic CO 2 Reduction Activity over Atomically Dispersed Metal Sites on Nitrogen-Doped Carbon

Autores: Jingkun Li, Paulina Pršlja, Tatsuya Shinagawa, Antonio José Martín Fernández, Frank Krumeich, Kateryna Artyushkova, Plamen Atanassov, Andrea Zitolo, Yecheng Zhou, Rodrigo García-Muelas, Núria López, Javier Pérez-Ramírez, Frédéric Jaouen
Publicado en: ACS Catalysis, Edición 9/11, 2019, Página(s) 10426-10439, ISSN 2155-5435
Editor: American Chemical Society
DOI: 10.1021/acscatal.9b02594

Non-redox doping boosts oxygen evolution electrocatalysis on hematite

Autores: Huu Chuong Nguyën, Felipe Andrés Garcés-Pineda, Mabel de Fez-Febré, José Ramón Galán-Mascarós, Núria López
Publicado en: Chemical Science, Edición 11/9, 2020, Página(s) 2464-2471, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/c9sc05669f

Spectroelectrochemical study of water oxidation on nickel and iron oxyhydroxide electrocatalysts

Autores: Laia Francàs, Sacha Corby, Shababa Selim, Dongho Lee, Camilo A. Mesa, Robert Godin, Ernest Pastor, Ifan E. L. Stephens, Kyoung-Shin Choi, James R. Durrant
Publicado en: Nature Communications, Edición 10/1, 2019, ISSN 2041-1723
Editor: Nature Publishing Group
DOI: 10.1038/s41467-019-13061-0

Versatile Nature of Oxygen Vacancies in Bismuth Vanadate Bulk and (001) Surface

Autores: Franziska Simone Hegner, Daniel Forrer, José Ramón Galán-Mascarós, Núria López, Annabella Selloni
Publicado en: The Journal of Physical Chemistry Letters, Edición 10/21, 2019, Página(s) 6672-6678, ISSN 1948-7185
Editor: American Chemical Society
DOI: 10.1021/acs.jpclett.9b02552

Water oxidation kinetics of nanoporous BiVO 4 photoanodes functionalised with nickel/iron oxyhydroxide electrocatalysts

Autores: Laia Francàs, Shababa Selim, Sacha Corby, Dongho Lee, Camilo A. Mesa, Ernest Pastor, Kyoung-Shin Choi, James R. Durrant
Publicado en: Chemical Science, Edición 12/21, 2021, Página(s) 7442-7452, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/d0sc06429g

Sputtered Nickel Oxide Thin Films on n-Si(100)/SiO 2 Surfaces for Photo-Electrochemical Oxygen Evolution Reaction (OER): Impact of Deposition Temperature on OER Performance and on Composition before and after OER

Autores: M. Fingerle, S. Tengeler, W. Calvet, W. Jaegermann, T. Mayer
Publicado en: Journal of The Electrochemical Society, Edición 167/13, 2020, Página(s) 136514, ISSN 1945-7111
Editor: The Electrochemical Society
DOI: 10.1149/1945-7111/abbcdf

Cobalt Amide Imidate Imidazolate Frameworks as Highly Active Oxygen Evolution Model Materials

Autores: Alberto Bucci, Suvendu Sekhar Mondal, Vlad Martin-Diaconescu, Alexandr Shafir, Julio Lloret-Fillol
Publicado en: ACS Applied Energy Materials, Edición 2/12, 2019, Página(s) 8930-8938, ISSN 2574-0962
Editor: ACS publications
DOI: 10.1021/acsaem.9b01977

Impact of the Synthesis Route on the Water Oxidation Kinetics of Hematite Photoanodes

Autores: Camilo A. Mesa, Ludmilla Steier, Benjamin Moss, Laia Francàs, James E. Thorne, Michael Grätzel, James R. Durrant
Publicado en: The Journal of Physical Chemistry Letters, Edición 11/17, 2020, Página(s) 7285-7290, ISSN 1948-7185
Editor: American Chemical Society
DOI: 10.1021/acs.jpclett.0c02004

The effect of nanoparticulate PdO co-catalysts on the faradaic and light conversion efficiency of WO 3 photoanodes for water oxidation

Autores: Anna A. Wilson, Sacha Corby, Laia Francàs, James R. Durrant, Andreas Kafizas
Publicado en: Physical Chemistry Chemical Physics, Edición 23/2, 2021, Página(s) 1285-1291, ISSN 1463-9076
Editor: Royal Society of Chemistry
DOI: 10.1039/d0cp06124g

Push‐Pull Electronic Effects in Surface‐Active Sites Enhance Electrocatalytic Oxygen Evolution on Transition Metal Oxides

Autores: Felipe Andrés Garcés‐Pineda, Huu Chuong Nguyën, Marta Blasco‐Ahicart, Miguel García‐Tecedor, Mabel Fez Febré, Peng‐Yi Tang, Jordi Arbiol, Sixto Giménez, José Ramón Galán‐Mascarós, Núria López
Publicado en: ChemSusChem, Edición 14/6, 2021, Página(s) 1595-1601, ISSN 1864-5631
Editor: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/cssc.202002782

Adsorption processes on a Pd monolayer-modified Pt(111) electrode

Autores: Xiaoting Chen, Laura P. Granda-Marulanda, Ian T. McCrum, Marc T. M. Koper
Publicado en: Chemical Science, Edición 11/6, 2020, Página(s) 1703-1713, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/c9sc05307g

Emergence of Potential-Controlled Cu-Nanocuboids and Graphene-Covered Cu-Nanocuboids under Operando CO 2 Electroreduction

Autores: Thanh Hai Phan, Karla Banjac, Fernando P. Cometto, Federico Dattila, Rodrigo García-Muelas, Stefan J. Raaijman, Chunmiao Ye, Marc T. M. Koper, Núria López, Magalí Lingenfelder
Publicado en: Nano Letters, Edición 21/5, 2021, Página(s) 2059-2065, ISSN 1530-6984
Editor: American Chemical Society
DOI: 10.1021/acs.nanolett.0c04703

Efficient Oxygen Evolution Electrocatalyst by Incorporation of Nickel into Nanoscale Dicobalt Boride

Autores: Jona Schuch, Sebastian Klemenz, Patrick Schuldt, Anne‐Marie Zieschang, Stephanie Dolique, Paula Connor, Bernhard Kaiser, Ulrike I. Kramm, Barbara Albert, Wolfram Jaegermann
Publicado en: ChemCatChem, Edición 13/7, 2021, Página(s) 1772-1780, ISSN 1867-3880
Editor: Wiley - VCH Verlag GmbH & CO. KGaA
DOI: 10.1002/cctc.202002030

An integrated photoanode based on non-critical raw materials for robust solar water splitting

Autores: Drialys Cardenas-Morcoso, Miguel García-Tecedor, Tsvetelina Merdzhanova, Vladimir Smirnov, Friedhelm Finger, Bernhard Kaiser, Wolfram Jaegermann, Sixto Gimenez
Publicado en: Materials Advances, Edición 1/5, 2020, Página(s) 1202-1211, ISSN 2633-5409
Editor: Royal Society of Chemistry
DOI: 10.1039/d0ma00355g

Influence of Van der Waals Interactions on the Solvation Energies of Adsorbates at Pt‐Based Electrocatalysts

Autores: Laura P. Granda‐Marulanda, Santiago Builes, Marc T. M. Koper, Federico Calle‐Vallejo
Publicado en: ChemPhysChem, Edición 20/22, 2019, Página(s) 2968-2972, ISSN 1439-4235
Editor: John Wiley & Sons Ltd.
DOI: 10.1002/cphc.201900512

Self-limited growth of an oxyhydroxide phase at the Fe 3 O 4 (001) surface in liquid and ambient pressure water

Autores: Florian Kraushofer, Francesca Mirabella, Jian Xu, Jiří Pavelec, Jan Balajka, Matthias Müllner, Nikolaus Resch, Zdeněk Jakub, Jan Hulva, Matthias Meier, Michael Schmid, Ulrike Diebold, Gareth S. Parkinson
Publicado en: The Journal of Chemical Physics, Edición 151/15, 2019, Página(s) 154702, ISSN 0021-9606
Editor: American Institute of Physics
DOI: 10.1063/1.5116652

Determining the role of oxygen vacancies in the photoelectrocatalytic performance of WO 3 for water oxidation

Autores: Sacha Corby, Laia Francàs, Andreas Kafizas, James R. Durrant
Publicado en: Chemical Science, Edición 11/11, 2020, Página(s) 2907-2914, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/c9sc06325k

Electrochemical Reduction of Carbon Dioxide to 1‐Butanol on Oxide‐Derived Copper

Autores: Louisa Rui Lin Ting, Rodrigo García‐Muelas, Antonio J. Martín, Florentine L. P. Veenstra, Stuart Tze‐Jin Chen, Yujie Peng, Edwin Yu Xuan Per, Sergio Pablo‐García, Núria López, Javier Pérez‐Ramírez, Boon Siang Yeo
Publicado en: Angewandte Chemie, Edición 132/47, 2020, Página(s) 21258-21265, ISSN 0044-8249
Editor: John Wiley & Sons Ltd.
DOI: 10.1002/ange.202008289

Sulfur-Modified Copper Catalysts for the Electrochemical Reduction of Carbon Dioxide to Formate

Autores: Tatsuya Shinagawa, Gastón O. Larrazábal, Antonio J. Martín, Frank Krumeich, Javier Pérez-Ramírez
Publicado en: ACS Catalysis, Edición 8/2, 2018, Página(s) 837-844, ISSN 2155-5435
Editor: American Chemical Society
DOI: 10.1021/acscatal.7b03161

Water Interaction with Sputter-Deposited Nickel Oxide on n-Si Photoanode: Cryo Photoelectron Spectroscopy on Adsorbed Water in the Frozen Electrolyte Approach

Autores: Mathias Fingerle, Sven Tengeler, Wolfram Calvet, Thomas Mayer, Wolfram Jaegermann
Publicado en: Journal of The Electrochemical Society, Edición 165/4, 2018, Página(s) H3148-H3153, ISSN 0013-4651
Editor: Electrochemical Society, Inc.
DOI: 10.1149/2.0191804jes

The Impact of Different Si Surface Terminations in the (001) n-Si/NiOx Heterojunction on the Oxygen Evolution Reaction (OER) by XPS and Electrochemical Methods

Autores: Sven Tengeler, Mathias Fingerle, Wolfram Calvet, Céline Steinert, Bernhard Kaiser, Thomas Mayer, Wolfram Jaegermann
Publicado en: Journal of The Electrochemical Society, Edición 165/4, 2018, Página(s) H3122-H3130, ISSN 0013-4651
Editor: Electrochemical Society, Inc.
DOI: 10.1149/2.0151804jes

Effect of Saturating the Electrolyte with Oxygen on the Activity for the Oxygen Evolution Reaction

Autores: Amanda C. Garcia, Marc T. M. Koper
Publicado en: ACS Catalysis, Edición 8/10, 2018, Página(s) 9359-9363, ISSN 2155-5435
Editor: American Chemical Society
DOI: 10.1021/acscatal.8b01447

Nitride‐Derived Copper Modified with Indium as a Selective and Highly Stable Catalyst for the Electroreduction of Carbon Dioxide

Autores: Florentine LP Veenstra, Antonio J Martín, Javier Pérez-Ramírez
Publicado en: ChemSusChem, 2019, ISSN 1864-5631
Editor: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/cssc.201901309

Origin of the Selective Electroreduction of Carbon Dioxide to Formate by Chalcogen Modified Copper

Autores: Rodrigo García-Muelas, Federico Dattila, Tatsuya Shinagawa, Antonio J. Martín, Javier Pérez-Ramírez, Núria López
Publicado en: The Journal of Physical Chemistry Letters, Edición 9/24, 2018, Página(s) 7153-7159, ISSN 1948-7185
Editor: American Chemical Society
DOI: 10.1021/acs.jpclett.8b03212

Unraveling Charge Transfer in CoFe Prussian Blue Modified BiVO 4 Photoanodes

Autores: Benjamin Moss, Franziska Simone Hegner, Sacha Corby, Shababa Selim, Laia Francàs, Núria López, Sixto Giménez, José-Ramón Galán-Mascarós, James Robert Durrant
Publicado en: ACS Energy Letters, Edición 4/1, 2018, Página(s) 337-342, ISSN 2380-8195
Editor: American Chemical Society
DOI: 10.1021/acsenergylett.8b02225

Microfabricated electrodes unravel the role of interfaces in multicomponent copper-based CO2 reduction catalysts

Autores: Gastón O. Larrazábal, Tatsuya Shinagawa, Antonio J. Martín, Javier Pérez-Ramírez
Publicado en: Nature Communications, Edición 9/1, 2018, ISSN 2041-1723
Editor: Nature Publishing Group
DOI: 10.1038/s41467-018-03980-9

The Impact of Different Si Surface Terminations in the (100) p-Si | n + -Si | Cu Junction with Respect to the Photo Electrochemical Performance

Autores: Céline Steinert, Sven Tengeler, Bernhard Kaiser, Wolfram Jaegermann
Publicado en: Journal of The Electrochemical Society, Edición 166/5, 2019, Página(s) H3208-H3214, ISSN 0013-4651
Editor: Electrochemical Society, Inc.
DOI: 10.1149/2.0291905jes

Oxygen Isotope Labeling Experiments Reveal Different Reaction Sites for the Oxygen Evolution Reaction on Nickel and Nickel Iron Oxides

Autores: Seunghwa Lee, Karla Banjac, Magalí Lingenfelder, Xile Hu
Publicado en: Angewandte Chemie International Edition, Edición 58/30, 2019, Página(s) 10295-10299, ISSN 1433-7851
Editor: John Wiley & Sons Ltd.
DOI: 10.1002/anie.201903200

Building Blocks for High Performance in Electrocatalytic CO 2 Reduction: Materials, Optimization Strategies, and Device Engineering

Autores: Gastón O. Larrazábal, Antonio J. Martín, Javier Pérez-Ramírez
Publicado en: The Journal of Physical Chemistry Letters, Edición 8/16, 2017, Página(s) 3933-3944, ISSN 1948-7185
Editor: American Chemical Society
DOI: 10.1021/acs.jpclett.7b01380

The role of oxygen vacancies in water splitting photoanodes

Autores: Roser Fernández-Climent, Sixto Giménez, Miguel García-Tecedor
Publicado en: Sustainable Energy & Fuels, Edición 4/12, 2020, Página(s) 5916-5926, ISSN 2398-4902
Editor: Royal Society of Chemistry
DOI: 10.1039/d0se01305f

A Semiempirical Method to Detect and Correct DFT-Based Gas-Phase Errors and Its Application in Electrocatalysis

Autores: Laura P. Granda-Marulanda, Alejandra Rendón-Calle, Santiago Builes, Francesc Illas, Marc T. M. Koper, Federico Calle-Vallejo
Publicado en: ACS Catalysis, Edición 10/12, 2020, Página(s) 6900-6907, ISSN 2155-5435
Editor: American Chemical Society
DOI: 10.1021/acscatal.0c01075

Heading to Distributed Electrocatalytic Conversion of Small Abundant Molecules into Fuels, Chemicals, and Fertilizers

Autores: Antonio José Martín, Javier Pérez-Ramírez
Publicado en: Joule, Edición 3/11, 2019, Página(s) 2602-2621, ISSN 2542-4351
Editor: Elsevier
DOI: 10.1016/j.joule.2019.09.007

Laser-Microstructured Copper Reveals Selectivity Patterns in the Electrocatalytic Reduction of CO2

Autores: Florentine L.P. Veenstra, Norbert Ackerl, Antonio J. Martín, Javier Pérez-Ramírez
Publicado en: Chem, Edición 6/7, 2020, Página(s) 1707-1722, ISSN 2451-9294
Editor: Elsevier
DOI: 10.1016/j.chempr.2020.04.001

Charge accumulation kinetics in multi-redox molecular catalysts immobilised on TiO 2

Autores: Carlota Bozal-Ginesta, Camilo A. Mesa, Annika Eisenschmidt, Laia Francàs, Ravi B. Shankar, Daniel Antón-García, Julien Warnan, Janina Willkomm, Anna Reynal, Erwin Reisner, James R. Durrant
Publicado en: Chemical Science, Edición 12/3, 2021, Página(s) 946-959, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/d0sc04344c

Active and Selective Ensembles in Oxide-Derived Copper Catalysts for CO 2 Reduction

Autores: Federico Dattila, Rodrigo Garcı́a-Muelas, Núria López
Publicado en: ACS Energy Letters, Edición 5/10, 2020, Página(s) 3176-3184, ISSN 2380-8195
Editor: ACS publications
DOI: 10.1021/acsenergylett.0c01777

Separating bulk and surface processes in NiO x electrocatalysts for water oxidation

Autores: Sacha Corby, Miguel-García Tecedor, Sven Tengeler, Céline Steinert, Benjamin Moss, Camilo A. Mesa, Hany F. Heiba, Anna A. Wilson, Bernhard Kaiser, Wolfram Jaegermann, Laia Francàs, Sixto Gimenez, James R. Durrant
Publicado en: Sustainable Energy & Fuels, Edición 4/10, 2020, Página(s) 5024-5030, ISSN 2398-4902
Editor: Royal Society of Chemistry
DOI: 10.1039/d0se00977f

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