CORDIS - EU research results
CORDIS

SmArt Designed Full Printed Flexible RObust Efficient Organic HaLide PerOvskite solar cells

Deliverables

Development of a public/private website. Project logo, public and private portal

A website uniquely dedicated to the APOLO project will be designed and launched acting as central source for project information, description, objectives, updates, latest developments as well as links to relevant pages, dissemination activities and other events valuable to the APOLO project and its stakeholders. Means of verification: online installation of public and private website in the domain www.n-track.eu. Indicator: uptime - objective 99,9% of time.

Workshop about standardization issues related to Perovskites based PV technologies (in connection with OE-A and EU Platform PV

Event organized around standards in PV and PSC with OEA Organic Electronic Association Photonics 21 EU Platform PV in association with standardization committees as CENELEC or CEN Means of verification organisation of event targeting experts in standardisation in the PV sector Indicator number of participants objective 20

Summer School on PSC technology

The school will expect the participation of graduate and postdocs students that also can present their research in PSC technology through oral and poster sessions gathering senior and junior researchers to foster information trespassing and motivate young researchers in the field Means of verification organisation of training event targeting students Indicator number of participants objective 15

Development, characterization and performance of antisoiling coating formulations

Public report of antisoiling layer formulation and application methodology This deliverable will present the different formulations developed and applied based on both grafting or coating methodologies and the results obtained in terms of antisoiling and antistatic capacities as the effect over previous layers and over the cell morphology Means of verification antisoiling performance will be experimentally verified in WP2 determining optical and antistatic properties and in WP5 on fabricated cells using antisoiling coatings Indicator transmittance contact angle and surface resistance of antisoiling coating KPI6 objective transmittance 93 contact angle 110o surface resistance reduction 102 Ohm from SoA PV glass and 10 less of soiling deposition

Green solvents definition for APOLO cells

Public report of perovskites Green Solvent Engineering results It will present the results obtained in each step Hansen solvent parameters of perovskites precursors green solvent selection dissolution studies and perovskite formation step studies It will also present an optimal ink formulation for perovskite formation Means of verification perovskite formation using selected green solvents will be monitorized via structural characterization Besides in WP4 cells with greensolvent perovskites will be developed and their performance tested LCA study in WP6 will evaluate the impact reduction Indicator PSC performance KPI1 CMR Carcinogenic Mutagenic or Toxic for Reproduction solvent category and environmental impact objective performance of PSC using selected green solvent over threshold 22 No CMR categories 1A 1B or 2 solvents used Environmental impact reduction of 10 minimum

Final recommendations to relevant standardization groups and implementation to the IEC standard roadmap

The specificities of Perovskites PV technologies regarding existing standards in other PV technologies thin film PV or cSilicon PV or to completely different applications mechanical bending gas barrier measurements for packaging etc will be highlighted The resulting recommendations for future standards adapted to Perovskites PV particularly regarding aging electrical measurements component and recycling will be communicated to standardization groups TC119 or other groups existing working groups in OEA etc in order to be implemented to the IEC standard roadmap Means of verification final report on recommendations will be communicate to standardization groups Indicator guide line for APOLO technologies standardization objective guide line defined

Open Day Workshop I

An Open Day workshop dedicated to dissemination activities will support further engagement and creation of Open Innovation community related to APOLO project results Means of verification organisation of dissemination event targeting industries to present projects results Indicator number of participants objective 50

Open Day Workshop II

An Open Day workshop dedicated to dissemination and exploitation activities will support further engagement with mapped stakeholders and possible endusers of APOLO project results Means of verification organisation of dissemination event targeting industries to present projects results Indicator number of participants objective 50

Optimized optical design of photonic structures for transparent and opaque substrates

"This deliverable will present the optimum set of geometrical parameters of the photonic micro-structures that will be patterned on both types of PSC substrates, taking only into account the optical performance of the devices by focusing on the maximization of their generated photocurrent for a range of different thicknesses (~250-500 nm) of the absorber layer. Means of verification: the modeled benefits of implementing the optimized photonic structures in the cells will be experimentally verified in WP4 by comparing the fabricated cells with reference devices (MS2). Indicator: absorber layer thickness (KPI#4) – objective: cells between 250-500 nm thick with good performance."

Micro-structured substrates for LT, with the optimized parameters indicated by the modelling tasks (WP3), uniformly patterned over large-areas (>10 cm2)

This deliverable will show the fabrication of transparent and opaque flexible substrates containing an area of 10 cm2 uniformly patterned by a longrange ordered hexagonal array of microcavities with the dimensions determined in WP3 Such photonic structure will be patterned via a scalable and lowcost softlithography method that combines a colloidal lithography technique to fabricate the stamps with a hotembossing process to imprint on the substrates Means of verification the benefits of the implementation of optimized LT structures will be experimentally verified in WP4 by comparing the fabricated cells with reference devices Indicator PSC performance KPI1 objective PSC cells with efficiency 22

Intermediate report about advanced characterization and protocols for optimal optoelectronic

In this deliverable the results of the characterization of PSCs devices developed in WP2 and WP4 with advanced techniques will be presented Means of verification there will be an interaction loop between the results of characterization and the material development tasks to guarantee the performance targets Indicator performance of PSC KPI1 objective Characterization of PSC with at least 20 in efficiency in rigid substrates and 15 in flexible substrates

Report about advanced characterization and protocols for optimal optoelectronic measurements

In this deliverable a micro and macroscale characterization of perovskite layers and complete devices will be performed The outcome of the analysis will be used for solar cell improvement High accuracy measurements of electrical device parameters will also be presented Means of verification there will be a interaction loop between the results of characterization and the material development tasks to guarantee the performance targets Indicator performance of PSC KPI1 objective PSC with more than 23 in efficiency in rigid substrates

Improved Charge Transport Materials, Perovskite Absorber and Passivation Strategy

The deliverable will present the advances made by partners towards the development of improved charge transport materials perovskite absorber and passivation strategies The report will be disseminated among the partners and will include published data relevant to the APOLO project Means of verification the advances in the development of transport and absorber layers will be experimentally verified in WP2 measuring the optoelectronic properties and in WP5 with stability test of the fabricated PSC Indicator PSC performance KPI1 2 and 3 and stability of the PSC KPI5 objective PSC with more than 23 in efficiency in rigid substrates and less than 10 of losses in efficiency after 1000h of accelerated aging

Opto-electronic model of optimal LT-enhanced PSCs, with at least 22% efficiency, on transparent and opaque substrates

"This deliverable will complement the work presented in D3.1 by determining the optimum sets of parameters of both the photonic elements and the PSC layer structure that maximize the device efficiency with a minimum Perovskite absorber thickness, now considering the full optical and electrical performance of the cells.This will guide the following experimental development of highly flexible PSC cells with efficiency >22%. Means of verification: the modeled benefits of implementing the optimized opto-electronic structures in the cells will be experimentally verified in WP4 by comparing the fabricated cells with reference devices. Indicator: PSc performance (KPI#1) – objective: PSC cells with efficiency >22%. "

Publications

Modified P3HT materials as hole transport layers for flexible perovskite solar cells

Author(s): Francesca De Rossi, Giacomo Renno, Babak Taheri, Narges Yaghoobi Nia, Viktoria Ilieva, Andrea Fin, Aldo Di Carlo, Matteo Bonomo, Claudia Barolo, Francesca Brunetti
Published in: Journal of Power Sources, Issue 494, 2021, Page(s) 229735, ISSN 0378-7753
Publisher: Elsevier BV
DOI: 10.1016/j.jpowsour.2021.229735

Design of wave-optical structured substrates for ultra-thin perovskite solar cells

Author(s): Sirazul Haque, Miguel Alexandre, Manuel J. Mendes, Hugo Águas, Elvira Fortunato, Rodrigo Martins
Published in: Applied Materials Today, Issue 20, 2020, Page(s) 100720, ISSN 2352-9407
Publisher: Elsevier
DOI: 10.1016/j.apmt.2020.100720

Attributes of High-Performance Electron Transport Layers for Perovskite Solar Cells on Flexible PET versus on Glass

Author(s): Dkhili, M., Lucarelli, G., De Rossi, F., Taheri, B., Hammedi, K., Ezzaouia, H., Brunetti, F., Brown, T.M.
Published in: ACS Applied Energy Materials, Issue 25740962, 2022, Page(s) 4096–4107, ISSN 2574-0962
Publisher: American Chemical Society
DOI: 10.1021/acsaem.1c03311

Simple and effective deposition method for solar cell perovskite films using a sheet of paper

Author(s): Zarabinia, N., Lucarelli, G., Rasuli, R., De Rossi, F., Taheri, B., Javanbakht, H., Brunetti, F., Brown, T.M.
Published in: iScience, Issue 25890042, 2022, Page(s) art. no. 103712, ISSN 2589-0042
Publisher: Elsevier Inc.
DOI: 10.1016/j.isci.2021.103712

Light-Stable Methylammonium-Free Inverted Flexible Perovskite Solar Modules on PET Exceeding 10.5% on a 15.7 cm2Active Area

Author(s): Castriotta, L.A., Fuentes Pineda, R., Babu, V., Spinelli, P., Taheri, B., Matteocci, F., Brunetti, F., Wojciechowski, K., Di Carlo, A.
Published in: ACS Applied Materials and Interfaces, Issue 19448244, 2021, Page(s) 29576-29584, ISSN 1944-8244
Publisher: American Chemical Society
DOI: 10.1021/acsami.1c05506

Toward Understanding the Short-Circuit Current Loss in Perovskite Solar Cells with 2D Passivation Layers

Author(s): Jan Herterich,Clemens Baretzky,Moritz Unmüssig,Clément Maheu,Nico Glissmann,Jeremias Gutekunst,Georgios Loukeris,Thomas Mayer,Markus Kohlstädt,Jan P. Hofmann,Uli Würfel
Published in: Solar RRL, Issue 2367198X, 2022, Page(s) 2200195, ISSN 2367-198X
Publisher: Wiley
DOI: 10.1002/solr.202200195

Thermosetting Polyurethane Resins as Low-Cost, Easily Scalable, and Effective Oxygen and Moisture Barriers for Perovskite Solar Cells

Author(s): Matteo Bonomo, Babak Taheri, Luca Bonandini, Sergio Castro-Hermosa, Thomas M. Brown, Marco Zanetti, Alberto Menozzi, Claudia Barolo, Francesca Brunetti
Published in: ACS Applied Materials & Interfaces, Issue 12/49, 2020, Page(s) 54862-54875, ISSN 1944-8244
Publisher: American Chemical Society
DOI: 10.1021/acsami.0c17652

Fill Factor Assessment in Hole Selective Layer Free Carbon Electrode-Based Perovskite Solar Cells with 15.5% Certified Power Conversion Efficiency

Author(s): Salma Zouhair, Bin Luo, Dmitry Bogachuk, David Martineau, Lukas Wagner, Adil Chahboun, Stefan W. Glunz, Andreas Hinsch
Published in: Solar RRL, Issue 2367198X, 2022, Page(s) 2100745, ISSN 2367-198X
Publisher: Wiley
DOI: 10.1002/solr.202100745

Perovskite Photovoltaics on Roll-To-Roll Coated Ultra-thin Glass as Flexible High-Efficiency Indoor Power Generators

Author(s): Sergio Castro-Hermosa, Giulia Lucarelli, Michiel Top, Matthias Fahland, John Fahlteich, Thomas M. Brown
Published in: Cell Reports Physical Science, Issue 1/5, 2020, Page(s) 100045, ISSN 2666-3864
Publisher: Elsevier
DOI: 10.1016/j.xcrp.2020.100045

Double-Mesoscopic Hole-Transport-Material-Free Perovskite Solar Cells: Overcoming Charge-Transport Limitation by Sputtered Ultrathin Al 2 O 3 Isolating Layer

Author(s): Gayathri Mathiazhagan, Lukas Wagner, Shankar Bogati, Kübra Yasaroglu Ünal, Dmitry Bogachuk, Thomas Kroyer, Simone Mastroianni, Andreas Hinsch
Published in: ACS Applied Nano Materials, Issue 3/3, 2020, Page(s) 2463-2471, ISSN 2574-0970
Publisher: American Chemical Society
DOI: 10.1021/acsanm.9b02563

Photonic-Structured Perovskite Solar Cells: Detailed Optoelectronic Analysis

Author(s): Haque, S., Alexandre, M., Baretzky, C., Rossi, D., De Rossi, F., Vicente, A.T., Brunetti, F., Águas, H., Ferreira, R.A.S., Fortunato, E., Auf Der Maur, M., Würfel, U., Martins, R., Mendes, M.J.
Published in: ACS Photonics, Issue 23304022, 2022, Page(s) 2408-2421, ISSN 2330-4022
Publisher: American Chemical Society
DOI: 10.1021/acsphotonics.2c00446

Laser-Scribing Optimization for Sprayed SnO2-Based Perovskite Solar Modules on Flexible Plastic Substrates

Author(s): Taheri, B., De Rossi, F., Lucarelli, G., Castriotta, L.A., Di Carlo, A., Brown, T.M., Brunetti, F.
Published in: ACS Applied Energy Materials, Issue 25740962, 2021, Page(s) 4507-4518, ISSN 2574-0962
Publisher: American Chemical Society
DOI: 10.1021/acsaem.1c00140

Neutron irradiated perovskite films and solar cells on PET substrates

Author(s): De Rossi, F., Taheri, B., Bonomo, M., Gupta, V., Renno, G., Yaghoobi Nia, N., Rech, P., Frost, C., Cazzaniga, C., Quagliotto, P., Di Carlo, A., Barolo, C., Ottavi, M., Brunetti, F.
Published in: Nano Energy, Issue 22112855, 2022, ISSN 2211-2855
Publisher: Elsevier BV
DOI: 10.1016/j.nanoen.2021.106879

Quantifying Performance of Permeation Barrier—Encapsulation Systems for Flexible and Glass‐Based Electronics and Their Application to Perovskite Solar Cells

Author(s): Sergio Castro‐Hermosa, Michiel Top, Janardan Dagar, John Fahlteich, Thomas M. Brown
Published in: Advanced Electronic Materials, Issue 5/10, 2019, Page(s) 1800978, ISSN 2199-160X
Publisher: Wiley
DOI: 10.1002/aelm.201800978

Optimum Luminescent Down-Shifting Properties for High Efficiency and Stable Perovskite Solar Cells

Author(s): Miguel Alexandre, Manuel Chapa, Sirazul Haque, Manuel J. Mendes, Hugo Águas, Elvira Fortunato, Rodrigo Martins
Published in: ACS Applied Energy Materials, Issue 2/4, 2019, Page(s) 2930-2938, ISSN 2574-0962
Publisher: American Chemical Society
DOI: 10.1021/acsaem.9b00271

Low-Temperature Solution-Processed Thin SnO 2 /Al 2 O 3 Double Electron Transport Layers Toward 20% Efficient Perovskite Solar Cells

Author(s): Janardan Dagar, Sergio Castro-Hermosa, Giulia Lucarelli, Andrea Zampetti, Franco Cacialli, Thomas M. Brown
Published in: IEEE Journal of Photovoltaics, Issue 9/5, 2019, Page(s) 1309-1315, ISSN 2156-3381
Publisher: IEEE Electron Devices Society
DOI: 10.1109/jphotov.2019.2928466

Photonic-structured TiO2 for high-efficiency, flexible and stable Perovskite solar cells

Author(s): Sirazul Haque, Manuel J. Mendes, Olalla Sanchez-Sobrado, Hugo Águas, Elvira Fortunato, Rodrigo Martins
Published in: Nano Energy, Issue 59, 2019, Page(s) 91-101, ISSN 2211-2855
Publisher: Elsevier BV
DOI: 10.1016/j.nanoen.2019.02.023

Development of Highly Bendable Transparent Window Electrodes Based on MoOx, SnO2, and Au Dielectric/Metal/Dielectric Stacks: Application to Indium Tin Oxide (ITO)-Free Perovskite Solar Cells

Author(s): Giulia Lucarelli, Thomas M. Brown
Published in: Frontiers in Materials, Issue 6, 2019, Page(s) 1-11, ISSN 2296-8016
Publisher: Frontiers-Media
DOI: 10.3389/fmats.2019.00310

Consensus statement for stability assessment and reporting for perovskite photovoltaics based on ISOS procedures

Author(s): Mark V. Khenkin, Eugene A. Katz, Antonio Abate, Giorgio Bardizza, Joseph J. Berry, Christoph Brabec, Francesca Brunetti, Vladimir Bulović, Quinn Burlingame, Aldo Di Carlo, Rongrong Cheacharoen, Yi-Bing Cheng, Alexander Colsmann, Stephane Cros, Konrad Domanski, Michał Dusza, Christopher J. Fell, Stephen R. Forrest, Yulia Galagan, Diego Di Girolamo, Michael Grätzel, Anders Hagfeldt, Elizabeth von
Published in: Nature Energy, Issue 5/1, 2020, Page(s) 35-49, ISSN 2058-7546
Publisher: Springer Nature Limited
DOI: 10.1038/s41560-019-0529-5

Automated Scalable Spray Coating of SnO 2 for the Fabrication of Low‐Temperature Perovskite Solar Cells and Modules

Author(s): Babak Taheri, Emanuele Calabrò, Fabio Matteocci, Diego Di Girolamo, Giorgio Cardone, Andrea Liscio, Aldo Di Carlo, Francesca Brunetti
Published in: Energy Technology, Issue 8/5, 2020, Page(s) 1901284, ISSN 2194-4288
Publisher: Wiley
DOI: 10.1002/ente.201901284

Revealing fundamentals of charge extraction in photovoltaic devices through potentiostatic photoluminescence imaging

Author(s): Lukas Wagner, Patrick Schygulla, Jan Philipp Herterich, Mohamed Elshamy, Dmitry Bogachuk, Salma Zouhair, Simone Mastroianni, Uli Würfel, Yuhang Liu, Shaik M. Zakeeruddin, Michael Grätzel, Andreas Hinsch, Stefan W. Glunz
Published in: Matter, Issue 15488411, 2022, Page(s) 2352-2364, ISSN 1548-8411
Publisher: Elsevier
DOI: 10.1016/j.matt.2022.05.024

An Interlaboratory Study on the Stability of All‐Printable Hole Transport Material–Free Perovskite Solar Cells

Author(s): Francesca De Rossi, Jérémy Barbé, David M. Tanenbaum, Lucio Cinà, Luigi Angelo Castriotta, Vasil Stoichkov, Zhengfei Wei, Wing Chung Tsoi, Jeffrey Kettle, Artem Sadula, John Chircop, Brian Azzopardi, Haibing Xie, Aldo Di Carlo, Monica Lira-Cantú, Eugene A. Katz, Trystan M. Watson, Francesca Brunetti
Published in: Energy Technology, Issue 8/12, 2020, Page(s) 2000134, ISSN 2194-4288
Publisher: Wiley
DOI: 10.1002/ente.202000134

Efficient fully blade-coated perovskite solar cells in air with nanometer-thick bathocuproine buffer layer

Author(s): Sergio Castro-Hermosa, Luana Wouk, Izabela Silva Bicalho, Luiza de Queiroz Corrêa, Bas de Jong, Lucio Cinà, Thomas M. Brown, Diego Bagnis
Published in: Nano Research, Issue 14/4, 2021, Page(s) 1034-1042, ISSN 1998-0124
Publisher: Tsinghua Univ Press
DOI: 10.1007/s12274-020-3147-4

The Nature of Methylamine-MAPbI 3 Complex: Fundamentals of Gas-Induced Perovskite Liquefaction and Crystallization

Author(s): Dmitry Bogachuk, Lukas Wagner, Simone Mastroianni, Michael Daub, Harald Hillebrecht, Andreas Hinsch
Published in: Journal of Materials Chemistry A, Issue 20507488, 2020, Page(s) 9788-9796, ISSN 2050-7488
Publisher: Royal Society of Chemistry
DOI: 10.1039/d0ta02494e

Phenethylammonium Iodide Passivation Layers for Flexible Planar Perovskite Solar Cells

Author(s): Lucarelli, G., De Rossi, F., Taheri, B., Brown, T.M., Brunetti, F.
Published in: Energy Technology, Issue 21944288, 2022, ISSN 2194-4288
Publisher: John Wiley and Sons Inc
DOI: 10.1002/ente.202200314

Self‐Crystallized Multifunctional 2D Perovskite for Efficient and Stable Perovskite Solar Cells

Author(s): Hobeom Kim, Mingyuan Pei, Yonghui Lee, Albertus A. Sutanto, Sanghyun Paek, Valentin I. E. Queloz, Aron J. Huckaba, Kyung Taek Cho, Hyung Joong Yun, Hoichang Yang, Mohammad Khaja Nazeeruddin
Published in: Advanced Functional Materials, Issue 30/19, 2020, Page(s) 1910620, ISSN 1616-301X
Publisher: John Wiley & Sons Ltd.
DOI: 10.1002/adfm.201910620

Intellectual Property Rights

Composition photopolymérisable adhésive pour l’encapsulation de dispositifs électroniques ou optoélectroniques

Application/Publication number: FR 2114208
Date: 2021-12-22
Applicant(s): ARKEMA FRANCE SA

Composition photopolymérisable adhésive pour l’encapsulation de dispositifs électroniques ou optoélectroniques

Application/Publication number: FR 2114208
Date: 2021-12-22

BLOQUE CONSTRUCTIVO FOTOELÉCTRICO

Application/Publication number: P 202230221
Date: 2022-03-16
Applicant(s): FLEXBRICK SL

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