Water Forced in Hydrophobic Nano-Confinement: Tunable Solvent System

Publications

Engineering of Phenylpyridine- and Bipyridine-Based Covalent Organic Frameworks for Photocatalytic Tandem Aerobic Oxidation/Povarov Cyclization

Author(s): Maarten Debruyne; Sander Borgmans; Sambhu Radhakrishnan; Eric Breynaert; Henk Vrielinck; Karen Leus; Andreas Laemont; Juul De Vos; Kuber Singh Rawat; Siebe Vanlommel; Hannes Rijckaert; Hadi Salemi; Jonas Everaert; Flore Vanden Bussche; Dirk Poelman; Rino Morent; Nathalie De Geyter; Pascal Van Der Voort; Veronique Van Speybroeck; Christian V. Stevens
Published in: ACS Applied Materials & Interfaces, Issue Vol. 15; iss. 29, 2023, Page(s) 35092-35106, ISSN 1944-8244
Publisher: American Chemical Society
DOI: 10.1021/acsami.3c07036

Hierarchical COK-X Materials for Applications in Catalysis and Adsorptive Separation and Controlled Release

Author(s): Sreeprasanth Pulinthanathu Sree, Eric Breynaert, Christine E. A. Kirschhock and Johan A. Martens
Published in: Frontiers in Chemical Engineering, Issue 26732718, 2022, ISSN 2673-2718
Publisher: Frontiers Research Foundation
DOI: 10.3389/fceng.2022.810443

Non-Isothermal Kinetic Model of Water Vapor Adsorption on a Desiccant Bed for Harvesting Water from Atmospheric Air

Author(s): Peeters R, Verbruggen V, Ronge J, Martens JA
Published in: Industrial & Engineering Chemistry Research, Issue Vol. 60, Iss. 31, 2021, Page(s) 11812-11823, ISSN 0888-5885
Publisher: American Chemical Society
DOI: 10.1021/acs.iecr.1c01733

Structure I methane hydrate confined in C8-grafted SBA-15: A highly efficient storage system enabling ultrafast methane loading and unloading

Author(s): Emile Jules Beckwée; Maarten Houlleberghs; Radu-George Ciocarlan; C. Vinod Chandran; Sambhu Radhakrishnan; Lucas Hanssens; Pegie Cool; Johan Martens; Eric Breynaert; Gino V. Baron; Joeri F.M. Denayer
Published in: Applied Energy, Issue Vol. 353, Issue A, 2024, ISSN 0306-2619
Publisher: Pergamon Press Ltd.
DOI: 10.1016/j.apenergy.2023.122120

Long-term Generation of Longitudinal Spin Order Controlled by Ammonia Ligation Enables Rapid SABRE Hyperpolarized 2D NMR

Author(s): Vaneeckhaute E, De Ridder S, Tyburn J-M, Kempf J, Taulelle F, Martens J, Breynaert E
Published in: Chemphyschem, Issue Vol. 22, Iss. 12, 2021, Page(s) 1170-1177, ISSN 1439-4235
Publisher: John Wiley & Sons Ltd.
DOI: 10.1002/cphc.202100079

Interfacial study of clathrates confined in reversed silica pores

Author(s): Mileo, Paulo G. M.; Rogge, Sven M. J.; Houlleberghs, Maarten; Breynaert, Eric; Martens, Johan A.; Van Speybroeck, Veronique
Published in: Journal of Materials Chemistry A, Issue 4, 2021, ISSN 2050-7488
Publisher: Royal Society of Chemistry
DOI: 10.1039/d1ta03105h

Hyperpolarised Magnetic Resonance of Exchangeable Protons Using Parahydrogen and Aminosilane

Author(s): Ewoud Vaneeckhaute, J Tyburn, D Kilgour, JG Kempf, Francis Taulelle, Johan A Martens, Eric Breynaert
Published in: The Journal of Physical Chemistry C: Energy Conversion and Storage, Optical and Electronic Devices, Interfaces, Nanomaterials, and Hard Matter, Issue Vol. 124; iss. 27, 2020, Page(s) 14541 - 14549, ISSN 1932-7447
Publisher: American Chemical Society
DOI: 10.1021/acs.jpcc.0c01149

Magneto-Hydrodynamic Mixing: a New Technique for Preparing Carbomer Hydrogels

Author(s): Maarten Houlleberghs,Loes Verheyden,Filip Voorspoels,C. Vinod Chandran,Karel Duerinckx,Sambhu Radhakrishnan,Johan A. Martens,Eric Breynaert
Published in: AIChE journal, Issue 00011541, 2022, ISSN 0001-1541
Publisher: American Institute of Chemical Engineers
DOI: 10.1002/aic.17911

Hydrogen-Bonded Water-Aminium Assemblies for Synthesis of Zeotypes with Ordered Heteroatoms

Author(s): Park, S. H.; Radhakrishnan, S.; Choi, W.; Chandran, C. V.; Kemp, K. C.; Breynaert, E.; Bell, R. G.; Kirschhock, C. E. A.; Hong, S. B.
Published in: Journal Of The American Chemical Society, Issue 00027863, 2022, Page(s) 18054–18061, ISSN 0002-7863
Publisher: American Chemical Society
DOI: 10.1021/jacs.2c07661

Nucleation of Porous Crystals from Ion-Paired Prenucleation Clusters

Author(s): Nick Pellens; Nikolaus Doppelhammer; Sambhu Radhakrishnan; Karel Asselman; C. Vinod Chandran; Dries Vandenabeele; Bernhard Jakoby; Johan A. Martens; Francis Taulelle; Erwin K. Reichel; Eric Breynaert; Christine E. A. Kirschhock
Published in: Chemistry of Materials, Issue 08974756, 2022, Page(s) 7139–7149, ISSN 0897-4756
Publisher: American Chemical Society
DOI: 10.1021/acs.chemmater.2c00418

Illuminating the Black Box: A Perspective on Zeolite Crystallization in Inorganic Media

Author(s): Karel Asselman; Christine Kirschhock; Eric Breynaert
Published in: Accounts of Chemical Research, Issue Vol. 56, 2023, Page(s) 2391-2402, ISSN 0001-4842
Publisher: American Chemical Society
DOI: 10.1021/acs.accounts.3c00269

Absolute Quantification of Residual Solvent in Mesoporous Silica Drug Formulations Using Magic-Angle Spinning NMR Spectroscopy

Author(s): Hannah Vanderschaeghe; Maarten Houlleberghs; Loes Verheyden; Dirk Dom; C. Vinod Chandran; Sambhu Radhakrishnan; Johan A. Martens; Eric Breynaert
Published in: Analytical Chemistry, Issue Vol. 95; iss. 3, 2023, Page(s) 1880-1887, ISSN 0003-2700
Publisher: American Chemical Society
DOI: 10.1021/acs.analchem.2c03646

Dispersing carbomers, mixing technology matters!

Author(s): Houlleberghs, Maarten; Verheyden, Loes; Voorspoels, Filip; Chandran, C. Vinod; Duerinckx, Karel; Radhakrishnan, Sambhu; Martens, Johan; Breynaert, Eric
Published in: RSC Advances, Issue vol 12, Iss. 13, 2022, Page(s) 7830 - 7834, ISSN 2046-2069
Publisher: Royal Society of Chemistry
DOI: 10.1039/d2ra00176d

Eu3+ doped ZnAl layered double hydroxides as calibrationless, fluorescent sensors for carbonate

Author(s): Alysson F. Morais; Ivan G. N. Silva; Bruno J. Ferreira; Alexandre C. Teixeira; Sreeprasanth P. Sree; Huayna Terraschke; Fernando A. Garcia; Eric Breynaert; Danilo Mustafa
Published in: Chemical Communications, Issue Vol. 59, 2023, Page(s) 13571-13574, ISSN 1359-7345
Publisher: Royal Society of Chemistry
DOI: 10.1039/d3cc03066k

A zeolite crystallisation model confirmed by in-situ observation.

Author(s): Nick Pellens, Nikolaus Doppelhammer, Karel Asselman, Barbara Thijs, Bernhard Jakoby, Erwin K. Konrad Reichel, Francis Taulelle, Johan Martens, Eric Breynaert and Christine Kirschhock
Published in: Faraday Discussions, Issue accepted, 2022, Page(s) https://lirias.kuleuven.be/handle/20.500.12942/694201, ISSN 1359-6640
Publisher: Royal Society of Chemistry
DOI: 10.1039/d1fd00093d

A Pyrrolidine Functionalized Poly[(Ethylene Glycol) Methacrylate] Resin as a Heterogeneous Catalyst for Aqueous Aldol Reactions

Author(s): Bert Biesemans; Noor Aljammal; Sambhu Radhakrishnan; Eric Breynaert; Christian V. Stevens; Jeroen Lauwaert; Joris W. Thybaut
Published in: Catalysts, Issue Vol. 12; iss. 11, 2022, ISSN 2073-4344
Publisher: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/catal12111389

Building a Cost-Efficient High-Pressure Cell for Online High-Field NMR and MRI Using Standard Static Probe Heads: An In Situ Demonstration on Clathrate Hydrate Formation

Author(s): Maarten Houlleberghs; Shannon Helsper; Dirk Dom; Thierry Dubroca; Bianca Trociewitz; Robert W. Schurko; Sambhu Radhakrishnan; Eric Breynaert
Published in: Analytical Chemistry, Issue Vol. 95; iss. 46, 2023, Page(s) 16936–16942, ISSN 0003-2700
Publisher: American Chemical Society
DOI: 10.1021/acs.analchem.3c03050

A Porous POSiSil Suited for Pressure-Driven Reversible Confinement of Solutions: PSS-2

Author(s): Sam Smet; Pieter Verlooy; Sreeprasanth Pulinthanathu; Christine Kirschhock; Francis Taulelle; Eric Breynaert
Published in: Chemistry-A European Journal, Issue Vol. 25; iss. 56, 2019, Page(s) 12957-12965, ISSN 0947-6539
Publisher: John Wiley & Sons Ltd.
DOI: 10.1002/chem.201901913

Framework flexibility-driven CO2 adsorption on a zeolite

Author(s): Hyun June Choi, Jung Gi Min, Sang Hyun Ahn, Jiho Shin, Suk Bong Hong, Sambhu Radhakrishnan, Vinod C Chandran, Robert G Bell, Eric Breynaert, Christine EA Kirschhock
Published in: Materials Horizons, Issue Vol. 7; iss. 6, 2020, Page(s) 1528 - 1532, ISSN 2051-6347
Publisher: ROYAL SOCIETY OF CHEMISTRY
DOI: 10.1039/d0mh00307g

Hydrogen Clathrates: Next Generation Hydrogen Storage Materials

Author(s): Gupta A, Baron GV, Perreault P, Lenaerts S, Ciocarlan R, Cool P, Mileo PGM, Rogge S, Van Speybroeck V, Watson G, Van Der Voort P, Houlleberghs M, Breynaert E, Martens J, Denayer JFM
Published in: Energy Storage Materials, Issue Vol. 41, 2021, Page(s) 69-107, ISSN 2405-8297
Publisher: Elsevier
DOI: 10.1016/j.ensm.2021.05.044

Isotopological Fingerprinting Using 1H/D Scrambling Identifies the Stereochemistry of Hyperpolarization Catalysts Transferring Spin Polarization from Parahydrogen to Substrates Using Signal Amplification by Reversible Exchange

Author(s): Ewoud Vaneeckhaute; Jean-Max Tyburn; James G. Kempf; Johan A. Martens; Eric Breynaert
Published in: Journal of Physical Chemistry Letters, Issue 19487185, 2022, Page(s) 3516-3522, ISSN 1948-7185
Publisher: American Chemical Society
DOI: 10.1021/acs.jpclett.2c00185

RHO Zeolites with High Hydrothermal Stability

Author(s): Hannelore Geerts-Claes; Gina Vanbutsele; Sreeprasanth Pulinthanathu Sree; Sambhu Radhakrishnan; C. Vinod Chandran; Eric Breynaert; Johan A. Martens; Sam Smet
Published in: Crystal Growth & Design, Issue Vol. 23; iss. 11, 2023, Page(s) 7829-7840, ISSN 1528-7483
Publisher: American Chemical Society
DOI: 10.1021/acs.cgd.3c00643

Super-ions of sodium cations with hydrated hydroxide anions: inorganic structure-directing agents in zeolite synthesis

Author(s): Asselman K, Pellens N, Radhakrishnan S, Chandran CV, Martens JA, Taulelle F, Verstraelen T, Hellström M, Breynaert E, Kirschhock CEA
Published in: Materials Horizons, Issue Vol. 8, Iss. 9, 2021, Page(s) 2576-2583, ISSN 2051-6347
Publisher: The Royal Society of Chemistry
DOI: 10.1039/d1mh00733e

Ion-Pairs in Aluminosilicate-Alkali Synthesis Liquids Determine the Aluminum Content and Topology of Crystallizing Zeolites

Author(s): Karel Asselman; Nick Pellens; Barbara Thijs; Nikolaus Doppelhammer; Mohamed Haouas; Francis Taulelle; Johan A. Martens; Eric Breynaert; Christine E.A. Kirschhock
Published in: Chemistry of Materials, Issue 08974756, 2022, Page(s) 7150-7158, ISSN 0897-4756
Publisher: American Chemical Society
DOI: 10.1021/acs.chemmater.2c00773

Prediction of Cu Zeolite NH3-SCR Activity from Variable Temperature 1H NMR Spectroscopy

Author(s): Sambhu Radhakrishnan; Sam Smet; C. Vinod Chandran; Sreeprasanth Pulinthanathu Sree; Karel Duerinckx; Gina Vanbutsele; Johan A. Martens; Eric Breynaert
Published in: Molecules, Issue Vol. 28; iss. 18, 2023, ISSN 1420-3049
Publisher: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/molecules28186456

Fresh water production from atmospheric air: Technology and innovation outlook

Author(s): Robin Peeters, Hannah Vanderschaeghe, Jan Rongé, Johan A. Martens
Published in: iScience, Issue 25890042, 2021, Page(s) 103266-103266, ISSN 2589-0042
Publisher: elsevier inc.
DOI: 10.1016/j.isci.2021.103266

Does Water Enable Porosity in Aluminosilicate Zeolites? Porous Frameworks versus Dense Minerals

Author(s): Karel Asselman; Mohamed Haouas; Maarten Houlleberghs; Sambhu Radhakrishnan; Wauter Wangermez; Christine E. A. Kirschhock; Eric Breynaert
Published in: Crystal Growth & Design, Issue Vol. 23; iss. 5, 2023, Page(s) 3338-3348, ISSN 1528-7483
Publisher: American Chemical Society
DOI: 10.1021/acs.cgd.2c01476

Structural Aspects Affecting Phase Selection in Inorganic Zeolite Synthesis

Author(s): Karel Asselman; Dries Vandenabeele; Nick Pellens; Nikolaus Doppelhammer; Christine E.A. Kirschhock; Eric Breynaert
Published in: Chemistry of Materials, Issue Vol. 34; iss. 24, 2022, Page(s) 11081-11092, ISSN 0897-4756
Publisher: American Chemical Society
DOI: 10.1021/acs.chemmater.2c03204

Water as a tuneable solvent: a perspective

Author(s): Eric Breynaert, Maarten Houlleberghs, Sambhu Radhakrishnan, Gerhard Grübel, Francis Taulelle, Johan A. Martens
Published in: Chemical Society Reviews, 2020, ISSN 0306-0012
Publisher: Royal Society of Chemistry
DOI: 10.1039/c9cs00545e

Energy performance and climate dependency of technologies for fresh water production from atmospheric water vapour

Author(s): Robin Peeters, Hannah Vanderschaeghe, Jan Rongé, Johan A Martens,
Published in: Environmental Science-Water Research & Technology, Issue Vol. 6, iss. 8, 2020, Page(s) 2016-2034, ISSN 2053-1419
Publisher: Royal Society of Chemistry
DOI: 10.1039/d0ew00128g

Noncontact In Situ Multidiagnostic NMR/Dielectric Spectroscopy

Author(s): Alysson F. Morais; Sambhu Radhakrishnan; Gavriel Arbiv; Dirk Dom; Karel Duerinckx; C. Vinod Chandran; Johan A. Martens; Eric Breynaert
Published in: Analytical Chemistry, Issue Vol. 96; iss. 13, 2024, Page(s) 5071-5077, ISSN 0003-2700
Publisher: American Chemical Society
DOI: 10.1021/acs.analchem.3c03007

Polysilicate Porous Organic Polymers (PSiPOPs), a Family of Porous, Ordered 3D Reticular Materials with Polysilicate Nodes and Organic Linkers

Author(s): Jelle Jamoul; Sam Smet; Sambhu Radhakrishnan; C. Vinod Chandran; Johan A. Martens; Eric Breynaert
Published in: Chemistry of Materials, Issue Vol. 36; iss. 3, 2024, Page(s) 1385-1394, ISSN 0897-4756
Publisher: American Chemical Society
DOI: 10.1021/acs.chemmater.3c02546

Reversible Parahydrogen Induced Hyperpolarization of 15N in Unmodified Amino Acids Unraveled at High Magnetic Field

Author(s): Ewoud Vaneeckhaute; Jean-Max Tyburn; James G. Kempf; Johan A. Martens; Eric Breynaert
Published in: Advanced Science, Issue Vol. 10; iss. 23, 2023, ISSN 2198-3844
Publisher: Wiley-VCH GmbH
DOI: 10.1002/advs.202207112

Enabling hydrate-based methane storage under mild operating conditions by periodic mesoporous organosilica nanotubes

Author(s): Emile Jules Beckwée; Geert Watson; Maarten Houlleberghs; Daniel Arenas Esteban; Sara Bals; Pascal Van Der Voort; Eric Breynaert; Johan Martens; Gino V. Baron; Joeri F.M. Denayer
Published in: Heliyon, Issue Vol. 9; iss. 7, 2023, ISSN 2405-8440
Publisher: Elsevier
DOI: 10.1016/j.heliyon.2023.e17662

HSIL-Based Synthesis of Ultracrystalline K,Na-JBW, a Zeolite Exhibiting Exceptional Framework Ordering and Flexibility

Author(s): Karel Asselman; Sambhu Radhakrishnan; Nick Pellens; C. Vinod Chandran; Maarten Houlleberghs; Yijue Xu; Johan A. Martens; Sreeprasanth Pulinthanathu Sree; Christine E.A. Kirschhock; Eric Breynaert
Published in: Chemistry of Materials, Issue 08974756, 2022, Page(s) 7159–7166, ISSN 0897-4756
Publisher: American Chemical Society
DOI: 10.1021/acs.chemmater.2c01059

Hydrogen bonding to oxygen in siloxane bonds drives liquid phase adsorption of primary alcohols in high-silica zeolites

Author(s): Sambhu Radhakrishnan; Charlotte Lejaegere; Karel Duerinckx; Wei-Shang Lo; Alysson F. Morais; Dirk Dom; C. Vinod Chandran; Ive Hermans; Johan A. Martens; Eric Breynaert
Published in: Materials Horizons, Issue Vol. 10, 2023, Page(s) 3702-3711, ISSN 2051-6347
Publisher: Royal Society of Chemistry
DOI: 10.1039/d3mh00888f

Strongly Reducing (Diarylamino)benzene-Based Covalent Organic Framework for Metal-Free Visible Light Photocatalytic H2O2 Generation

Author(s): Chidharth Krishnaraj, Himanshu Sekhar Jena, Laurens Bourda, Andreas Laemont, Pradip Pachfule, Jerome Roeser, Vinod C Chandran, Sander Borgmans, Sven MJ Rogge, Karen Leus, Christian Stevens, Johan A Martens, Veronique Van Speybroeck, Eric Breynaert, Arne Thomas, Pascal Van der Voort
Published in: Journal Of The American Chemical Society, Issue Vol. 142; iss. 47, 2020, Page(s) 20107 - 20116, ISSN 0002-7863
Publisher: American Chemical Society
DOI: 10.1021/jacs.0c09684

Online Solid-Phase Extraction–Gas Chromatography–Flame Ionization Detection System for Monitoring Contaminants at Parts-Per-Trillion Concentrations in Process Waters

Author(s): Lejaegere, Charlotte; Vercammen, Joeri; Verheyden, Loes; Martens, Johan
Published in: Lc Gc Europe, Issue Vol. 36; iss. 01, 2023, Page(s) 7-13, ISSN 1471-6577
Publisher: Advanstar Communications Inc.
DOI: 10.56530/lcgc.eu.eb6169h7

IZM-7: A new stable aluminosilicogermanate with a promising catalytic activity

Author(s): El Hayek, E.; Radhakrishnan, S.; Vanbutsele, G.; Pulinthanathu Sree, S.; Rivallan, M.; Soyer, E.; Bouchy, C.; Breynaert, Eric; Martens, J.; Chizallet, C.; Harbuzaru, B.
Published in: Journal of Catalysis, Issue 00219517, 2021, Page(s) 601-605, ISSN 0021-9517
Publisher: Academic Press
DOI: 10.1016/j.jcat.2021.11.006

NMR crystallography reveals carbonate induced Al-ordering in ZnAl layered double hydroxide

Author(s): Sambhu Radhakrishnan; Karl Lauwers; C. Vinod Chandran; Julien Trébosc; Sreeprasanth Pulinthanathu Sree; Johan A. Martens; Francis Taulelle; Christine E. A. Kirschhock; Eric Breynaert
Published in: Chemistry—A European Journal, Issue 3, 2021, ISSN 0947-6539
Publisher: John Wiley & Sons Ltd.
DOI: 10.1002/chem.202101275

Engineering of hollow periodic mesoporous organosilica nanorods for augmented hydrogen clathrate formation

Author(s): Geert Watson; Nithin B. Kummamuru; Sammy W. Verbruggen; Patrice Perreault; Maarten Houlleberghs; Johan Martens; Eric Breynaert; Pascal Van Der Voort
Published in: Journal of Materials Chemistry A, Issue Vol. 11, 2023, Page(s) 26265-26276, ISSN 2050-7488
Publisher: Royal Society of Chemistry
DOI: 10.1039/d3ta05530b

How Water and Ion Mobility Affect the NMR Fingerprints of the Hydrated JBW Zeolite: a Combined Computational-Experimental Investigation

Author(s): Vanlommel, S.; Hoffman, A. E. J.; Smet, S.; Radhakrishnan, S.; Asselman, K.; Chandran, C. V.; Breynaert, E.; Kirschhock, C. E. A.; Martens, J. A.; Van Speybroeck, V.
Published in: Chemistry-A European Journal, Issue 09476539, 2022, ISSN 0947-6539
Publisher: John Wiley & Sons Ltd.
DOI: 10.1002/chem.202202621

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