Efficient CO2 conversion over multisite Zeolite-Metal nanocatalysts to fuels and OlefinS

Livrables

Organisation of a workshop, open to public and private stakeholders, students, the press and the public, for the dissemination of the project results, held in conjunction with the mid-term review. Refers to Task 5.2

Communication marketing material

Preparation of dissemination materials such as flyers, posters and brochures that provide an overview of the project and project partners, for distribution by all partners at conferences and exhibitions, in addition to logo and dissemination templates. Refers to Task 5.1

COZMOS website

Establishment of an external project website. The website will include information on the project and project partners. Refers to Task 5.1

Final workshop

Organisation of a final workshop, open to public and private stakeholders, students, the press and the public, for the dissemination of the final project results. Refers to Task 5.2

Report on the performance of zeolitic catalyst

Report on catalytic test results on zeolitic catalysts for the MTO reaction, including the catalysts’ relative activity for methylation and hydrogenation of alkenes in the targeted temperature and pressure rangesRefers to Task 1.2

Report on pilot plant operation

A public report including the pilot plant operations is prepared. The results and studies are summarized considering evaluations using COZMOS technology. Refers to task 3.5

White paper on CCU realisation and perception, with a focus on COZMOS' technology

The report will summarize the key aspects of TEAs and LCAs developed in WP4 and will aim at communicating the main insights of the studies to a non-technical audience with particular focus on policy maker audience. The content and the format of the white paper shall be agreed by the whole consortium and contain clear and rigorous statements (supported by verifiable data) on the conditions and circumstances (geographical, techno-economical etc.) under which the CCU, in general and COZMOS process in particular, represent a sustainable route to the overall reduction of carbon emissions. Refers to Task 5.4

Report describing optimised and fully integrated process scheme

This public report will describe the principal process setup, features and boundary conditions. An overall mass and energy balance will be included. Refers to Task 2.3

Report on combined catalyst synthesis

Report on the synthesis of combined catalysts including characterisation. Refers to Task 1.1 and 1.3

Public report on the social readiness of the COZMOS process

The public report will be informed by the initial report described in D4.4 and will be subject to peer review by experts before publication. We will act on the recommendations of the review as appropriate. The report will only be published once the consent of all partners has been received. Refers to Task 4.4

Report on catalyst synthesis and testing

Final, public report comprising lab.scale synthesis, characterization and test results for all catalysts produced in the project, including performance discussion and site-performance correlations. Test results will range from performance optimization (activity, selectivity, stability) to mechanistic studies, and discussion of the correlation between these two approaches to catalyst performance evaluation. The report will be published after obtaining the consent of all partners.Refers to Task 1.1, 1.2 and 1.3

Publications

Analytical Review of Life‐Cycle Environmental Impacts of Carbon Capture and Utilization Technologies

Auteurs: Guillermo Garcia‐Garcia, Marta Cruz Fernandez, Katy Armstrong, Steven Woolass and Peter Styring
Publié dans: ChemSusChem, Numéro 14, 2021, Page(s) 995-1015, ISSN 1864-564X
Éditeur: Wiley
DOI: 10.1002/cssc.202002126

PdZn/ZrO2+SAPO-34 bifunctional catalyst for CO2 conversion: Further insights by spectroscopic characterization

Auteurs: Ticali, Pierfrancesco; Morandi, Sara; Shterk, Genrikh; Ould-Chikh, Samy; Ramirez, Adrian; Gascon, Jorge; Chung, Sang-Ho; Ruiz-Martinez, Javier; Bordiga, Silvia
Publié dans: Applied Catalysis A: General, Numéro 655, 2023, Page(s) 119100, ISSN 0926-860X
Éditeur: Elsevier BV
DOI: 10.1016/apcata.2023.119100

Highly selective hydrogenation of CO2 to propane over GaZrOx/H-SSZ-13 composite

Auteurs: Sen Wang, Li Zhang, Pengfei Wang, Weiyong Jiao, Zhangfeng Qin, Mei Dong, Jianguo Wang, Unni Olsbye and Weibin Fan
Publié dans: Nature Catalysis, Numéro 5, 2022, Page(s) 1038-1050, ISSN 2520-1158
Éditeur: Springer Nature
DOI: 10.1038/s41929-022-00871-7

MAPO-18 Catalysts for the Methanol to Olefins Process: Influence of Catalyst Acidity in a High-Pressure Syngas (CO and H2) Environment

Auteurs: Jingxiu Xie, Daniel S. Firth, Tomás Cordero-Lanzac, Alessia Airi, Chiara Negri, Sigurd Øien-Ødegaard, Karl Petter Lillerud, Silvia Bordiga, and Unni Olsbye
Publié dans: ACS Catalysis, Numéro 12, 2022, Page(s) 1510-1531, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.1c04694

On the conversion of CO2 to value added products over composite PdZn and H-ZSM-5 catalysts: excess Zn over Pd, a compromise or a penalty?

Auteurs: Christian Ahoba-Sam; Elisa Borfecchia; Andrea Lazzarini; Aram Bugaev; Abdulrahman Adamu Isah; Mostafa Taoufik; Silvia Bordiga; Unni Olsbye
Publié dans: Catalysis Science & Technology, Numéro 10/13, 2020, Page(s) 4373-4385, ISSN 2044-4761
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0cy00440e

CO2 hydrogenation to methanol and hydrocarbons over bifunctional Zn-doped ZrO2/zeolite catalysts

Auteurs: Pierfrancesco Ticali; Davide Salusso; Rafia Ahmad; Christian Ahoba-Sam; Adrian Ramirez; Genrikh Shterk; Kirill A. Lomachenko; Elisa Borfecchia; Sara Morandi; Luigi Cavallo; Jorge Gascon; Silvia Bordiga; Unni Olsbye
Publié dans: Catalysis Science & Technology, Numéro 11, 2021, Page(s) 1249-1268, ISSN 2044-4761
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0cy01550d

Supported PdZn nanoparticles for selective CO2 conversion, through the grafting of a heterobimetallic complex on CeZrOx

Auteurs: Paolo Ruzzi, Davide Salusso, Matilde Baravaglio, Kai C. Szeto, Aimery De Mallmann, Laia Gil Jiménez, Cyril Godard, Anass Benayad, Sara Morandi, Silvia Bordiga, Mostafa Taoufik
Publié dans: Applied Catalysis A, Numéro 635, 2022, Page(s) 118568, ISSN 0926-860X
Éditeur: Elsevier BV
DOI: 10.1016/j.apcata.2022.118568

A Toroidal Zr 70 Oxysulfate Cluster and Its Diverse Packing Structures

Auteurs: Sigurd Øien‐Ødegaard, Calliope Bazioti, Evgeniy A. Redekop, Øystein Prytz, Karl Petter Lillerud, Unni Olsbye
Publié dans: Angewandte Chemie International Edition, Numéro 59/48, 2020, Page(s) 21397-21402, ISSN 1433-7851
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202010847

From Lab to Technical CO2 Hydrogenation Catalysts: Understanding PdZn Decomposition

Auteurs: Ticali, Pierfrancesco; Salusso, Davide; Airi, Alessia; Morandi, Sara; Borfecchia, Elisa; Ramirez, Adrian; Cordero-Lanzac, Tomás; Gascon, Jorge; Olsbye, Unni; Joensen, Finn; Bordiga, Silvia
Publié dans: ACS Applied Materials and Interfaces, Numéro 15, 2023, Page(s) 5218-5228, ISSN 1944-8252
Éditeur: American Chemical Society
DOI: 10.1021/acsami.2c19357

Catalyst sites and active species in the early stages of MTO conversion over cobalt AlPO-18 followed by IR spectroscopy

Auteurs: Alessia Airi, Alessandro Damin, Jingxiu Xie, Unni Olsbye and Silvia Bordiga
Publié dans: Catalysis Science & Technology, Numéro 12, 2022, ISSN 2044-4761
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d2cy00303a

Multifunctional Catalyst Combination for the Direct Conversion of CO2 to Propane

Auteurs: Adrian Ramirez; Pierfrancesco Ticali; Davide Salusso; Tomás Cordero-Lanzac; Samy Ould-Chikh; Christian Ahoba-Sam; Aram L. Bugaev; Elisa Borfecchia; Sara Morandi; Matteo Signorile; Silvia Bordiga; Jorge Gascon; Unni Olsbye
Publié dans: JACS Au, Numéro 1, 2021, Page(s) 1719-1732, ISSN 2691-3704
Éditeur: Americal Chemical Society
DOI: 10.1021/jacsau.1c00302

Selective Conversion of CO2 into Propene and Butene

Auteurs: Sen Wang, Li Zhang, Wenyu Zhang, Pengfei Wang. Zhangfeng Qin, Wenjun Yan, Mei Dong, Junfen Li. Jianguo Wang, Lin He, Unni Olsbye and Weibin Fan
Publié dans: Chem, 2020, ISSN 2451-9294
Éditeur: Cell Press
DOI: 10.1016/j.chempr.2020.09.025

Combining X-ray Diffraction and X-ray Absorption Spectroscopy to Unveil Zn Local Environment in Zn-Doped ZrO2 Catalysts

Auteurs: Davide Salusso, Elisa Borfecchia, and Silvia Bordiga
Publié dans: Journal of Physical Chemistry C, Numéro 40, 2021, Page(s) 22249-22261, ISSN 1932-7447
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpcc.1c06202

A CO2 valorization plant to produce light hydrocarbons: Kinetic model, process design and life cycle assessment

Auteurs: Cordero-Lanzac, Tomás; Ramirez, Adrian; Cruz-Fernandez, Marta; Zander, Hans-Jörg; Joensen, Finn; Woolass, Steven; Meiswinkel, Andreas; Styring, Peter; Gascon, Jorge; Olsbye, Unni
Publié dans: Journal of CO2 Utilization, Numéro 67, 2023, Page(s) 102337, ISSN 2212-9820
Éditeur: Elsevier BV
DOI: 10.1016/j.jcou.2022.102337

Highly effective conversion of CO2 into light olefins abundant in ethene

Auteurs: Sen Wang, Li Zhang, Pengfei Wang, Xingchen Liu, Yanyan Chen, Zhangfeng Qin, Mei Dong, Jianguo Wang, Lin He, Unni Olsbye and Weibin Fan
Publié dans: CHEM, 2022, ISSN 2451-9294
Éditeur: Cell Press
DOI: 10.1016/j.chempr.2022.01.004

The Oxygenate-Mediated Conversion of COx to Hydrocarbons─On the Role of Zeolites in Tandem Catalysis

Auteurs: Xie, Jingxiu; Olsbye, Unni
Publié dans: Chemical Reviews, Numéro 123, 2023, Page(s) 11775-11816, ISSN 1520-6890
Éditeur: American Chemical Society
DOI: 10.1021/acs.chemrev.3c00058

Droits de propriété intellectuelle

PROCESS AND PLANT FOR PRODUCING ONE OR MORE HYDROCARBONS

Numéro de demande/publication: 20 21080669
Date: 2021-11-04
Demandeur(s):

METHOD AND SYSTEM FOR PRODUCING ONE OR MORE OLEFINS

Numéro de demande/publication: 20 21050686
Date: 2021-01-14
Demandeur(s):

Livrables

Publications

Droits de propriété intellectuelle

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