DistributEd Chemicals And fuels production from CO2 in photoelectrocatalytic DEvices

Project Information

DECADE

Grant agreement ID: 862030

DOI

10.3030/862030

Project closed

EC signature date 8 April 2020

Start date 1 May 2020

End date 31 January 2025

Funded under

• INDUSTRIAL LEADERSHIP - Leadership in enabling and industrial technologies - Advanced materials

Total cost

€ 5 358 672,49

EU contribution

€ 5 198 756,69

Coordinated by

European Research Institute of Catalysis A.I.S.B.L.
Belgium

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Deliverables

Websites, patent fillings, videos etc. (1)

Project Website

M3onwards Website platform is available and continuously updated

Documents, reports (1)

Dissemination and Communication Plan

M6 with updates at M18 M36 and M48 Report on the proposed dissemination and communication activities and all which have taken place It will include List of project contributions to conferences publications symposia workshops

Publications

Peer reviewed articles (31)

Defect engineering over anisotropic brookite toward substrate-specific photo-oxidation of alcohols

Author(s): S. M. Hossein Hejazi, Mahdi Shahrezaei, Piotr Błoński, Mattia Allieta, Polina M. Sheverdyaeva, Paolo Moras, Zdeněk Baďura, Sergii Kalytchuk, Elmira Mohammadi, Radek Zbořil, Štěpán Kment, Michal Otyepka, Alberto Naldoni, Paolo Fornasiero
Published in: Chem Catalysis, Issue 2, 2024, Page(s) 1177-1190, ISSN 2667-1093
Publisher: Elsevier BV
DOI: 10.1016/j.checat.2022.03.015

Driving up the Electrocatalytic Performance for Carbon Dioxide Conversion through Interface Tuning in Graphene Oxide-Bismuth Oxide Nanocomposites

Author(s): Melchionna, M; Moro, M; Adorinni, S; Nasi, L; Colussi, S; Poggini, L; Marchesan, S; Valenti, G; Paolucci, F; Prato, M; Fornasiero, P.
Published in: ACS Applied Energy Materials, Issue 5-11, 2022, Page(s) 13356-13366, ISSN 2574-0962
Publisher: American Chemical Society
DOI: 10.1021/acsaem.2c02013

Photocatalytic C−H Amination of Electron‐rich Aromatic Hydrocarbons by Carbon Nitride Photocatalysis

Author(s): Stefano Mazzanti, Yevheniia Markushyna, Oleksandr Savateev
Published in: ChemCatChem, Issue 15, 2023, ISSN 1867-3880
Publisher: Wiley - VCH Verlag GmbH & CO. KGaA
DOI: 10.1002/cctc.202201388

Advanced (photo)electrocatalytic approaches to substitute the use of fossil fuels in chemical production

Author(s): Gabriele Centi; Siglinda Perathoner; Chiara Genovese; Rosa Arrigo
Published in: Chem. Commun.,, Issue 59, 2023, Page(s) 3005-3023, ISSN 1359-7345
Publisher: Royal Society of Chemistry
DOI: 10.1039/d2cc05132j

Nitrogen Reduction Reaction to Ammonia at Ambient Conditions: A Short Review Analysis of the Critical Factors Limiting Electrocatalytic Performance

Author(s): Francesco Tavella; Daniele Giusi; Claudio Ampelli
Published in: Current Opinion in Green and Sustainable Chemistry Volume 35, June 2022, Issue 35, 2022, Page(s) 100604, ISSN 2452-2236
Publisher: Elsevier
DOI: 10.1016/j.cogsc.2022.100604

Elucidating the electronic properties of single-wall carbon nanohorns

Author(s): Zieleniewska, A; Lodermeyer, F; Prato, M; Rumbles, G; Guldi, DM; Blackburn, JL.
Published in: Journal of Materials Chemistry C, Issue 10 - 15, 2022, Page(s) 5783-5786, ISSN 2050-7534
Publisher: Royal Society of Chemistry
DOI: 10.1039/d2tc00179a

Nanostructured electrocatalysts for organic synthetic transformations

Author(s): Francesco Mancuso, Paolo Fornasiero, Maurizio Prato, Michele Melchionna, Federico Franco, Giacomo Filippini
Published in: Nanoscale, Issue 16, 2024, Page(s) 5926-5940, ISSN 2040-3364
Publisher: Royal Society of Chemistry
DOI: 10.1039/d3nr06669j

Electrocatalytic CO₂ reduction: role of the cross-talk at nano-carbon interfaces

Author(s): Michele Melchionna, Paolo Fornasiero, Maurizio Prato, Marcella Bonchio
Published in: Energy & Environmental Science, Issue 14, 2024, Page(s) 5816-5833, ISSN 1754-5692
Publisher: Royal Society of Chemistry
DOI: 10.1039/d1ee00228g

Challenges in temperature measurements in gas-phase photothermal catalysis

Author(s): Luca Mascaretti, Andrea Schirato, Tiziano Montini, Alessandro Alabastri, Alberto Naldoni, Paolo Fornasiero
Published in: Joule, Issue 6, 2023, Page(s) 1727-1732, ISSN 2542-4351
Publisher: Elsevier
DOI: 10.1016/j.joule.2022.06.019

Calix[4]arene-based molecular photosensitizers for sustainable hydrogen production and other solar applications

Author(s): Chiara Liliana Boldrini, Norberto Manfredi, Tiziano Montini, Laura Baldini, Alessandro Abbotto, Paolo Fornasiero
Published in: Current Opinion in Green and Sustainable Chemistry, Issue 32, 2021, Page(s) 100534, ISSN 2452-2236
Publisher: Elsevier BV
DOI: 10.1016/j.cogsc.2021.100534

Electrode and cell design for CO2 reduction: A viewpoint

Author(s): Claudio Ampelli, Francesco Tavella, Daniele Giusi, Angela Mercedes Ronsisvalle, Siglinda Perathoner, Gabriele Centi
Published in: Catalysis Today, Issue 421, 2021, Page(s) 114217, ISSN 0920-5861
Publisher: Elsevier BV
DOI: 10.1016/j.cattod.2023.114217

CO2 conversion to solar fuels and chemicals: Opening the new paths

Author(s): Gabriele Centi, Claudio Ampelli
Published in: Journal of Energy Chemistry, Issue 91, 2024, Page(s) 680-683, ISSN 2095-4956
Publisher: Elsevier BV
DOI: 10.1016/j.jechem.2024.01.021

Photoelectrocatalysis for Hydrogen Evolution Ventures into the World of Organic Synthesis

Author(s): Giuseppe Sportelli, Miriam Marchi, Paolo Fornasiero, Giacomo Filippini, Federico Franco, Michele Melchionna
Published in: Global Challenges, Issue 8, 2024, ISSN 2056-6646
Publisher: WILEY-V C H VERLAG GMBH
DOI: 10.1002/gch2.202400012

Water-Mediated ElectroHydrogenation of CO2 at Near-Equilibrium Potential by Carbon Nanotubes/Cerium Dioxide Nanohybrids

Author(s): Valenti, G; Melchionna, M; Montini, T; Boni, A; Nasi, L; Fonda, E; Criado, A; Zitolo, A; Voci, S; Bertoni, G; Bonchio, M; Fornasiero, P; Paolucci, F; Prato, M.
Published in: ACS Applied Energy Materials, Issue 3 - 9, 2020, Page(s) 8509-8518, ISSN 2574-0962
Publisher: American Chemical Society
DOI: 10.1021/acsaem.0c01145

Well-defined Cu₂O photocatalysts for solar fuels and chemicals

Author(s): Sourav Rej, Matteo Bisetto, Alberto Naldoni, Paolo Fornasiero
Published in: Journal of Materials Chemistry A, Issue 9, 2024, Page(s) 5915-5951, ISSN 2050-7488
Publisher: Royal Society of Chemistry
DOI: 10.1039/d0ta10181h

Electrocatalytic CO 2 reduction: role of the cross-talk at nano-carbon interfaces

Author(s): Michele Melchionna, Paolo Fornasiero, Maurizio Prato, Marcella Bonchio
Published in: Energy & Environmental Science, 2021, ISSN 1754-5692
Publisher: Royal Society of Chemistry
DOI: 10.1039/d1ee00228g

Best practices for experiments and reporting in photocatalytic CO2 reduction

Author(s): Marcella Bonchio, Julien Bonin, Osamu Ishitani, Tong-Bu Lu, Takeshi Morikawa, Amanda J. Morris, Erwin Reisner, Debashrita Sarkar, Francesca M. Toma, Marc Robert
Published in: Nature Catalysis, Issue 6, 2023, Page(s) 657-665, ISSN 2520-1158
Publisher: NATURE PORTFOLIO
DOI: 10.1038/s41929-023-00992-7

Electrocatalysis: Prospects and Role to Enable an E‐Chemistry Future

Author(s): Gabriele Centi, Siglinda Perathoner
Published in: The Chemical Record, Issue early view, 2025, Page(s) e202400259, ISSN 1527-8999
Publisher: John Wiley & Sons Inc.
DOI: 10.1002/tcr.202400259

Comparing Molecular Mechanisms in Solar NH3 Production and Relations with CO2 Reduction.

Author(s): Domenico Mallamace; Georgia Papanikolaou; Siglinda Perathoner; Gabriele Centi; Paola Lanzafame
Published in: Int. J. Mol. Sci., Issue 22(1), 2021, Page(s) 139, ISSN 1422-0067
Publisher: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/ijms22010139

Enhancing Oxygenic Photosynthesis by Cross-Linked Perylenebisimide “Quantasomes”

Author(s): Gobbato, T; Rigodanza, F; Benazzi, E; Costa, P; Garrido, M; Sartorel, A; Prato, M; Bonchio, M.
Published in: Journal of the American Chemical Society, Issue 44 - 31, 2022, Page(s) 14021–14025, ISSN 1520-5126
Publisher: American Chemical Society
DOI: 10.1021/jacs.2c05857

Current density in solar fuel technologies

Author(s): Valentino Romano; Giovanna D'Angelo; Siglinda Perathoner; Gabriele Centi
Published in: Energy Environ. Sci., Issue 14, 2021, Page(s) 5760-5787, ISSN 0974-7451
Publisher: RSC
DOI: 10.1039/d1ee02512k

Challenges and prospects of plasmonic metasurfaces for photothermal catalysis

Author(s): Luca Mascaretti, Andrea Schirato, Paolo Fornasiero, Alexandra Boltasseva, Vladimir M. Shalaev, Alessandro Alabastri, Alberto Naldoni
Published in: Nanophotonics, Issue 11, 2023, Page(s) 3035-3056, ISSN 2192-8614
Publisher: Walter de Gruyter GmbH
DOI: 10.1515/nanoph-2022-0073

The role of ceria/precious metal interfaces in catalysis

Author(s): Michele Melchionna, Paolo Fornasiero
Published in: RSC Applied Interfaces, Issue 1, 2024, Page(s) 70-79, ISSN 2755-3701
Publisher: Royal Chemical Society
DOI: 10.1039/d3lf00202k

In situ electrochemical characterization of CuxO-based gas-diffusion electrodes (GDEs) for CO2 electrocatalytic reduction in presence and absence of liquid electrolyte and relationship with C2+ products formation

Author(s): Daniele Giusi, Matteo Miceli, Chiara Genovese, Gabriele Centi, Siglinda Perathoner, Claudio Ampelli
Published in: Applied Catalysis B: Environmental, Issue 318, 2022, Page(s) 121845, ISSN 0926-3373
Publisher: Elsevier BV
DOI: 10.1016/j.apcatb.2022.121845

Catalysis for e-Chemistry: Need and Gaps for a Future De-Fossilized Chemical Production, with Focus on the Role of Complex (Direct) Syntheses by Electrocatalysis

Author(s): Siglinda Perathoner; PAOLA LANZAFAME; GEORGIA PAPANIKOLAOU; Gabriele Centi
Published in: ACS Catalysis, Issue 12(5), 2022, Page(s) 2861–2876, ISSN 2155-5435
Publisher: American Chemical Society
DOI: 10.1021/acscatal.2c00099

Reuse of CO₂ in energy intensive process industries

Author(s): Siglinda Perathoner, Kevin M. Van Geem, Guy B. Marin, Gabriele Centi
Published in: Chemical Communications, Issue 57, 2024, Page(s) 10967-10982, ISSN 1359-7345
Publisher: Royal Society of Chemistry
DOI: 10.1039/d1cc03154f

An artificial leaf device built with earth-abundant materials for combined H₂ production and storage as formate with efficiency > 10%

Author(s): Claudio Ampelli; Daniele Giusi; Matteo Miceli; Tsvetelina Merdzhanova; Vladimir Smirnov; Ugochi Chime; Oleksandr Astakhov; Antonio José Martín; Florentine Louise Petronella Veenstra; Felipe Andrés Garcés Pineda; Jesús González-Cobos; Miguel García-Tecedor; Sixto Giménez; Wolfram Jaegermann; Gabriele Centi; Javier Pérez-Ramírez; José Ramón Galán-Mascarós; Siglinda Perathoner
Published in: Energy & environmental science 16(4), 1644-1661 (2023). doi:10.1039/D2EE03215E, Issue 8, 2023, Page(s) 1644-1661, ISSN 0974-7451
Publisher: RSC
DOI: 10.1039/d2ee03215e

Design of dye-sensitized TiO₂ materials for photocatalytic hydrogen production: light and shadow

Author(s): Lorenzo Zani, Michele Melchionna, Tiziano Montini, Paolo Fornasiero
Published in: Journal of Physics: Energy, Issue 3, 2021, Page(s) 031001, ISSN 2515-7655
Publisher: IOP Publishing
DOI: 10.1088/2515-7655/abe04b

Light-driven, heterogeneous organocatalysts for C-C bond formation toward valuable perfluoroalkylated intermediates

Author(s): Filippini, G; Longobardo, F; Forster, L; Criado, A; Di Carmine, G; Nasi, L; DAgostino, C; Melchionna, M; Fornasiero, P; Prato, M.
Published in: Science Advances, Issue 6 - 46, 2020, Page(s) eabc9923, ISSN 2375-2548
Publisher: American Association for the Advancement of Science
DOI: 10.1126/sciadv.abc9923

Thin silicon heterojunction solar cells in perovskite shadow: Bottom cell prospective

Author(s): U. Chime, W. Duan, A. Lambertz, K. Bittkau, V. Lauterbach, K. Ding, U. Rau, T. Merdzhanova, O. Astakhov
Published in: Solar Energy Materials and Solar Cells, Issue 270, 2024, Page(s) 112813, ISSN 0927-0248
Publisher: Elsevier BV
DOI: 10.1016/j.solmat.2024.112813

Multibranched Calix[4]arene‐Based Sensitizers for Efficient Photocatalytic Hydrogen Production

Author(s): Norberto Manfredi, Cristina Decavoli, Chiara Liliana Boldrini, Tarekegn Heliso Dolla, Federica Faroldi, Francesco Sansone, Tiziano Montini, Laura Baldini, Paolo Fornasiero, Alessandro Abbotto
Published in: European Journal of Organic Chemistry, Issue 2021, 2023, Page(s) 284-288, ISSN 1434-193X
Publisher: John Wiley & Sons Ltd.
DOI: 10.1002/ejoc.202001296