Solar Energy for Carbon-Free Liquid Fuel

Livrables

Membrane photocathode assembly suitable for gas-phase operation with performance suitable for integration into a tandem cell for 10% STH efficiency

A set of photocathode membrane assemblies with included protection layers and/or HER electrocatalysts, with at least one asssembly that achieves (or has a concrete action plan to achieve) a water splitting photocurrent of 8.2 mA/cm2 under standard solar illumination.

Visual identity, project website and social media accounts

Visual identity (including a logo) and website will be designed to ensure brand consistency, recognition and visibility of Sun-To-X. Social media accounts (Twitter and LinkedIn) will be created and fed through for the project duration to communicate about the project and disseminate its key results.

Development of a catalytic system able to utilize HydroSil in the reduction of esters and carbonates

A catalytic system will be developped and its potential in the conversion of model substrates representatives of the chemical linkages present in waste plastics will be demonstrated This deliverable hence include the reduction of aliphatic and aromatic esters as well as organic carbonates using HydroSil as the reductant

Intermediate Advisory Board recommendations report

Report summarising the advisory board recommendations after the first meeting The meeting should have been attended by all advisory board members and the coordinator Relevant feedback should be discussed between the coordinator and SuntoX participants Where relevant a clear plan for implementing advice should be made

Final Advisory Board recommendations report

Report summarising the advisory board recommendations after the second meeting. The meeting should have been attended by all advisory board members and the coordinator. Relevant feedback should be discussed between the coordinator and Sun-to-X participants (EPFL / ENGIE). Where relevant, a clear plan for implementing advice in the demonstrator stage should be made.

Data Management Plan

Description of the data management plan for the project

Report on the activities of collaboration with IC5

Report summarising the actions during the project with Mission Innovation IC5- contributions to their roadmap, demonstration activites, synergies / interactions with other IC5 projects

Guidelines generated from the validated multi-physics model of the PEC device

Model should give reasonable predictions of photocurrent same order of magnitude after validation Strategies to improve performance by considering for example efficiency of light absorption and current collection should be presented

Publications

The 2022 Solar Fuels Roadmap

Auteurs: Gideon Segev; Jakob Kibsgaard; Christopher Hahn; Zhichuan J Xu; Wen-Hui (Sophia) Cheng; Todd G Deutsch; Chengxiang Xiang; Jenny Z Zhang; Leif Hammarström; Daniel G Nocera; Adam Z Weber; Peter Agbo; Takashi Hisatomi; Frank E Osterloh; Kazunari Domen; Fatwa F Abdi; Sophia Haussener; Daniel J Miller; Shane Ardo; Paul C McIntyre; Thomas Hannappel; Shu Hu; Harry Atwater; John M Gregoire; Mehmed Z Erte
Publié dans: Journal of Physics D: Applied Physics, 2022, Page(s) Volume 55 Article 323003, ISSN 0022-3727
Éditeur: Institute of Physics Publishing
DOI: 10.1088/1361-6463/ac6f97

Easy Diameter Tuning of Silicon Nanowires with Low-Cost SnO2-Catalyzed Growth for Lithium-Ion Batteries

Auteurs: Caroline Keller Yassine Djezzar, Jingxian Wang, Saravanan Karuppiah, Gérard Lapertot, Cédric Haon, and Pascale Chenevier
Publié dans: Nanomaterials, Numéro 28 July 2022, 2022, Page(s) 2601, ISSN 2079-4991
Éditeur: MDPI
DOI: 10.3390/nano12152601

Zirconium-catalysed hydrosilylation of esters and depolymerisation of polyester plastic waste

Auteurs: Marie Kobylarski, Liam J. Donnelly, Jean-Claude Berthet and Thibault Cantat
Publié dans: Green Chemistry, Numéro 27 Aug 2022, 2022, Page(s) 6810-6815, ISSN 1463-9262
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d2gc02186b

Transparency and Morphology Control of Cu2O Photocathodes via an in Situ Electroconversion

Auteurs: Marina Caretti, Linda Lazouni, Meng Xia, Rebekah A. Wells, Simon Nussbaum, Dan Ren, Michael Grätzel, and Kevin Sivula*
Publié dans: ACS Energy Letters, 2022, ISSN 2380-8195
Éditeur: American Chemical Society
DOI: 10.1021/acsenergylett.2c00474

Porous silicon-nanowire-based electrode for the photoelectrocatalytic production of hydrogen

Auteurs: Jingxian Wang, Caroline Keller, Marc Dietrich, Paul E. Olli, Pascal Gentile, Stéphanie Pouget, Hanako Okuno, Mohamed Boutghatin, Yan Pennec, Valérie Reita, Duc N. Nguyen, Hannah Johnson, Adina Morozan, Vincent Artero and Pascale Chenevier
Publié dans: Sustainable Energy & Fuels, Numéro 23 August 2023, 2023, Page(s) 4864-4876, ISSN 2398-4902
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d3se00408b

Transparent Porous Conductive Substrates for Gas-Phase Photoelectrochemical Hydrogen Production

Auteurs: Marina Caretti, Elizaveta Mensi, Raluca-Ana Kessler, Linda Lazouni, Benjamin Goldman, Loï Carbone, Simon Nussbaum, Rebekah A. Wells, Hannah Johnson, Emeline Rideau, Jun-ho Yum, Kevin Sivula
Publié dans: Advanced Materials, Numéro 28 November 2022, 2022, Page(s) 2208740, ISSN 1521-4095
Éditeur: Wiley
DOI: 10.1002/adma.202208740

Selective Reduction of Secondary Amides to Imines Catalysed by Schwartz's Reagent

Auteurs: Dr. Liam J. Donnelly, Dr. Jean-Claude Berthet, Dr. Thibault Cantat
Publié dans: Angewandte Chemie, Numéro 18 May 2022, 2022, Page(s) e202206170, ISSN 1433-7851
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202206170

Sun-To-X: Using solar energy to produce a carbon-free liquid fuel

Auteurs: Hannah Johnson
Publié dans: Innovation News Network, Numéro 19th April 2023, 2023
Éditeur: Innovation News Network

Lifecycle Assessment and Public Acceptance Study into Green Hydrogen Storage in Liquid Carrier

Auteurs: Mary Hanhoun, Jonas Pigeon, Julie Clavreul, Laurent Baraton, Hannah Johnson
Publié dans: FISITA Conference Proceedings, Numéro 12th September 2023, 2023
Éditeur: FISITA

Livrables

Publications

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