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A Unified Route to Polycyclic Terpenes

Project description

A shorter path for the synthesis of polycyclic terpenes

Xanthates comprise a class of organic salts formed by the treatment of an alcohol with carbon disulfide in the presence of an alkali. These organosulphur compounds are versatile intermediates in organic synthesis. The EU-funded Route2polyTepr project will demonstrate how xanthates could significantly shorten the synthesis path of synthetic polycyclic terpenes and terpene alkaloids. Xanthates enable the formation of new carbon–carbon bonds on unactivated alkenes as well as the formation of rings that are impossible to achieve with other methods. The project will generate new knowledge on xanthates' potential in radical reactions (powerful carbon–carbon bond-forming processes).

Objective

In this proposal we would like to demonstrate the strategic role that xanthates could play in providing a unified approach to a multitude of polycyclic terpenes and in shortening considerably the synthetic routes. By enabling the strategic intermolecular creation of new carbon-carbon bonds on unactivated alkenes and the formation of rings not readily accessible by other methods, the degenerative radical exchange of xanthates opens numerous synthetic avenues not hitherto available. Unusual retrosynthetic disconnections will now be envisaged, and it is hoped that a unified, short, and practical route to numerous classes of polycyclic terpenes and terpene alkaloids can be implemented. Demonstration of the advantage of using xanthate transfer to the synthesis of polycyclic terpenes will bring the academic’s attention to novel applications of radical reactions, promoting the development in the area.

Keywords

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Programme(s)

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Topic(s)

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Funding Scheme

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MSCA-IF - Marie Skłodowska-Curie Individual Fellowships (IF)

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Call for proposal

Procedure for inviting applicants to submit project proposals, with the aim of receiving EU funding.

(opens in new window) H2020-MSCA-IF-2019

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Coordinator

ECOLE POLYTECHNIQUE
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 184 707,84
Address
ROUTE DE SACLAY
91128 PALAISEAU CEDEX
France

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Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 184 707,84
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