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Gases in Water

Project description

The structure of water and breathing of fish

Water is one of the most important substances in chemistry and biology with a vital role in life on Earth. Evidence is mounting that water can exist in two liquid forms of high- or low-density and that at normal conditions there are local fluctuations between the two. The EU-funded GAS-WAT focuses on understanding how such fluctuations in the structure of water facilitate oxygen dissolution in water and how fish can extract it. Has evolution found a way to optimise the structure of water near the gills of fish to facilitate the exchange? Through a combination of modelling and experimental work, researchers will characterise water structure in gills and determine the mechanism by which fish extract oxygen from water.

Objective

Is there “hidden” structure in normal liquid water? Do nanoscopic structural heterogeneities in ambient water exist and affect solution chemistry? In this project we will focus on structural fluctuations in simulations of liquid water as observed through the enhancement of the isothermal compressibility. From both experiment and theory a two-state picture of water is emerging with fluctuations between high- (HDL) and low-density (LDL) local structures. The structure of these is unknown. Moreover, present simulation models require a pressure shift of one thousand atmospheres to reproduce the experimental compressibility maximum at ambient pressure. We propose to develop a unique description of the liquid that extends to take into account that the water molecule exists in two forms, ortho and para, with different rotational properties. We will use Argon dissolved in water as discrete probe of the LDL local environments in high-resolution EXAFS measurements to discern their structure in combination. Finally, in a two-state picture with LDL structures providing “pockets of stability” for dissolved oxygen, the question arises how fish entice the oxygen to leave the water and enter the gills. We will carry out a combined experimental X-ray spectroscopic and theoretical modeling study of water in polyelectrolyte and polysaccharide models of the mucous layer found outside lamella of fish gills and specifically determine how water structure there differs from the bulk. Has Nature through evolution found a way to restructure the water to enhance exchange of gases?

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ERC-ADG - Advanced Grant

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Call for proposal

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(opens in new window) ERC-2020-ADG

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Host institution

STOCKHOLMS UNIVERSITET
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 2 295 625,00
Address
UNIVERSITETSVAGEN 10
10691 Stockholm
Sweden

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Region
Östra Sverige Stockholm Stockholms län
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 2 295 625,00

Beneficiaries (1)

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