A significant portion of the reporting period was dedicated to developing experimental infrastructure tailored for coherent acoustic phonon studies at ultrahigh frequencies. Key setups developed include:
Two coherent generation/detection systems for acoustic phonons;
A Sagnac interferometer for detecting coherent surface displacements;
Experimental setups operational across a wide thermal range (4 K to 600 °C).
One major achievement is the successful implementation of a non-local acoustic transport measurement system, enabling the generation and detection of coherent, quasi-continuous phonons at 20 GHz. This system is based on a ridge waveguide with a Fabry-Perot vertical structure, simultaneously confining near-infrared photons and high-frequency phonons.
By using a focused picosecond-pulsed laser at ~80 MHz repetition rate, we achieved quasi-continuous propagation of coherent phonons with a decay rate of ~1.14 dB/m, far beyond the optical excitation volume. Spatio-temporal interference experiments further confirmed mutual coherence between phonons emitted from distinct sources. This confirms the scalability and coherence of the system, and its potential for programmable phonon networks via spatial light modulation.
In the realm of tunable nanophononic devices, we investigated VO2 thin films, known for their strong temperature-driven optical transitions. While optical signatures of the transition were clear, acoustic transitions were inconclusive, likely hindered by surface roughness impacting the propagation of nanowaves.
We also developed acoustic resonators using mesoporous materials sensitive to ambient conditions. Experimental results show clear shifts in resonance peaks with changing humidity. However, after repeated cycling, tunable behavior degraded, prompting ongoing investigations into the causes (e.g. structural hysteresis or moisture-induced aging).