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Sustainable light-emitting devices through control of dynamic doping

Project description

A novel sustainable light-emission technology through control of dynamic doping

Artificial illumination is essential in modern society, with LEDs and OLEDs playing a key role. However, their production consumes significant amounts of critical raw materials and energy, and their recycling remains challenging. The light-emitting electrochemical cell (LEC) presents a promising, sustainable alternative through its energy-efficient CRM-free printing fabrication, but it currently lags in emission performance. To render LECs more efficient and sustainable, it is critical to suppress exciton quenching by nearby dopants in the p-n junction region. The ERC-funded InnovaLEC project aims to develop means for the control of the in-situ formed p-n junction doping structure, and through a subsequent tuning of this doping structure enable efficient LEC emission. This approach presents a novel path to high-efficiency LECs without relying on energy-intensive processes or toxic materials.

Objective

Artificial illumination is fundamental and ubiquitous in modern society, and the cuArtificial illumination is fundamental and ubiquitous in modern society, and the current large-scale commercialization of more efficient and practical technologies, in the form of LEDs and OLEDs, is therefore important. This development is not only resulting in improved luminaires and displays, but also paving the way for a wide range of applications in, e.g. medtech, security, and communication. However, a growing concern is related to that the fabrication of LEDs and OLEDs consumes large amounts of critical raw materials (CRMs) and energy, and that their recycling is poorly developed and difficult.

A novel illumination technology, the light-emitting electrochemical cell (LEC), is in this context interesting, and we and others have recently developed concepts for its material- and energy-efficient and CRM-free printing fabrication and its delivery of efficient emission (although not yet on par with LED/OLED). These combined achievements now pave the way for a timely and important challenge: can the LEC become the first emissive technology that is truly sustainable through its entire lifecycle?

We boldly argue that this vision can turn true if we can take control of the defining LEC feature, viz. the dynamic formation of a p-n junction by electrochemical doping. It was recently shown that current LECs suffer from severe quenching of the excitons (the photon precursors formed in the p-n junction) by too-nearby dopants, and we here introduce new insights and methodologies that address this setback through rational design and careful development of new materials. A key task is to tune the mobility of the electronic charge carriers and excitons, through guidelines established by modeling, for the attainment of a sharp p-n junction boundary. We emphasize that our proposed path to high-efficiency LECs does not depend on energy-intense processes or the use of toxic or CRM-based materials.

Fields of science (EuroSciVoc)

Keywords

Programme(s)

Topic(s)

Funding Scheme

HORIZON-ERC - HORIZON ERC Grants

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Call for proposal

(opens in new window) ERC-2022-ADG

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Host institution

UMEA UNIVERSITET
Net EU contribution
€ 2 500 000,00
Address
UNIVERSITETOMRADET
901 87 UMEA
Sweden
Region
Östra Sverige Stockholm Stockholms län
Activity type
Higher or Secondary Education Establishments
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Total cost
€ 2 500 000,00

Beneficiaries (1)