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Development of bottom-up custom-functionalized graphene/porphyrin nanoarchitectures with atomic precision

Objective

The ongoing miniaturization of electronic devices has been raising awareness for the need to develop alternative high-performance and energy-efficient semiconductor materials. The current project (GRAPHYRIN) aims to synthesize new atomically precise hybrid nanoarchitectures, comprising graphene nanostructures (graphene nanoribbons, GNRs, or nanoporous graphene, NPG) and porphyrins (PORs), with promising properties to fabricate next-generation materials to be used, for example, in gas sensing electronic devices. First, multistage organic synthesis will be carried out to obtain individual or fused precursors of GNRs and PORs (“seeding stages”), which will later allow the construction of partially and fully conjugated hybrid systems. Here, we will synthesize appropriate bianthracence-based reactants (or equivalent derivatives) as molecular building blocks of GNRs and, in parallel, several PORs (tetra- or di-substituted) with appropriate structural features to functionalize GNRs. Alternatively, POR-fused GNRs hybrid precursors will be synthesized via direct functionalization of PORs with GNRs precursors or via synthesis of GNRs precursors bearing aldehyde groups. Several polymerization strategies will be explored (“growing stages”), using in-solution synthesis (ISS) or on-surface synthesis (OSS), namely on Au(111) surfaces. The polymerization reactions will involve, for example, Suzuki or Ullmann coupling. Depending on the properties of the starting GNRs and POR precursors, the final structures may either be one- or two-dimensional (1D GNRs/PORs or 2D NPG/PORs, respectively). Finally, the successfully synthesized hybrid materials will be explored as gas sensors for future electronic devices. It is expected that the outcomes from GRAPHYRIN will allow to go beyond the state-of-the-art and take a step further towards the synthesis of new custom-made graphene/POR nanoarchitectures for ideal gas sensing electronic devices.

Fields of science (EuroSciVoc)

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Keywords

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Programme(s)

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Topic(s)

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Funding Scheme

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HORIZON-TMA-MSCA-PF-EF - HORIZON TMA MSCA Postdoctoral Fellowships - European Fellowships

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Call for proposal

Procedure for inviting applicants to submit project proposals, with the aim of receiving EU funding.

(opens in new window) HORIZON-MSCA-2023-PF-01

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Coordinator

UNIVERSIDAD DE SANTIAGO DE COMPOSTELA
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 181 152,96
Address
COLEXIO DE SAN XEROME PRAZA DO OBRADOIRO S/N
15782 Santiago De Compostela
Spain

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Region
Noroeste Galicia A Coruña
Activity type
Higher or Secondary Education Establishments
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

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