Angular studies of photoelectrons in innovative research environments

Deliverables

Multiphoton PECD from limonene demonstrated
Generation of high harmonics from an OPCPA
Measurement and interpretation of MF-PADs from alanine
PhD theses
Demonstration of PECD on aromatic amino-acids (Tyrosine and/or tryptophane): from the monomers to the nanoparticles
Measurement of MFPADs from oriented OCS molecules with few-cycle carrier envelope stable laser pulses
Measurement of PADs from aligned benzonitrile
Demonstration of Coulomb explosion imaging from selected bonds in an organic chiral molecule
Publications in the primary literature
Measurement of MFPADs from NO2 using coincidence methodology
Laser induced electron diffraction measurements of complex molecular systems, such as molecules embedded in He nanodroplets
3D PADs following the excitation of wavepackets in molecules

Availability of multidimensional imaging detectors
Availability of detectors capable of discriminating the multiple charged particles ejected following the interaction of complex molecules with extreme radiation
Availability of new software for data storage and analysis

Project website up and running

Outreach events
Advertising vacancies
Organization of network events
Training courses and workshops

Publications

CEP-stable few-cycle pulses with more than 190 μJ of energy at 100 kHz from a noncollinear optical parametric amplifier

Author(s): Federico J. Furch, Tobias Witting, Achut Giree, Chao Luan, Felix Schell, Gunnar Arisholm, Claus P. Schulz, Marc J. J. Vrakking
Published in: Optics Letters, Issue 42/13, 2017, Page(s) 2495, ISSN 0146-9592
Publisher: Optical Society of America
DOI: 10.1364/OL.42.002495

Intense Vibronic Modulation of the Chiral Photoelectron Angular Distribution Generated by Photoionization of Limonene Enantiomers with Circularly Polarized Synchrotron Radiation

Author(s): Mohammad M. Rafiee Fanood, Hassan Ganjitabar, Gustavo A. Garcia, Laurent Nahon, Stefano Turchini, Ivan Powis
Published in: ChemPhysChem, Issue 19/8, 2018, Page(s) 921-933, ISSN 1439-4235
Publisher: John Wiley & Sons Ltd.
DOI: 10.1002/cphc.201701248

Multiple-orbital effects in laser-induced electron diffraction of aligned molecules

Author(s): Faruk Krečinić, Philipp Wopperer, Biagio Frusteri, Felix Brauße, Jean-Gabriel Brisset, Umberto De Giovannini, Angel Rubio, Arnaud Rouzée, Marc J. J. Vrakking
Published in: Physical Review A, Issue 98/4, 2018, ISSN 2469-9926
Publisher: American Physical Society
DOI: 10.1103/PhysRevA.98.041401

Electron asymmetries in the photoionization of chiral molecules: possible astrophysical implications

Author(s): Rim Hadidi, Dusan K. Bozanic, Gustavo A. Garcia, Laurent Nahon
Published in: Advances in Physics: X, Issue 3/1, 2018, Page(s) 1477530, ISSN 2374-6149
Publisher: Taylor-Francis
DOI: 10.1080/23746149.2018.1477530

Vibrationally-resolved photoelectron spectroscopy and photoelectron circular dichroism of bicyclic monoterpene enantiomers

Author(s): Hassan Ganjitabar, Rim Hadidi, Gustavo A. Garcia, Laurent Nahon, Ivan Powis
Published in: Journal of Molecular Spectroscopy, Issue 353, 2018, Page(s) 11-19, ISSN 0022-2852
Publisher: Academic Press
DOI: 10.1016/j.jms.2018.08.007

High-order harmonic generation spectroscopy by recolliding electron caustics

Author(s): D Faccialà, S Pabst, B D Bruner, A G Ciriolo, M Devetta, M Negro, P Prasannan Geetha, A Pusala, H Soifer, N Dudovich, S Stagira, C Vozzi
Published in: Journal of Physics B: Atomic, Molecular and Optical Physics, Issue 51/13, 2018, Page(s) 134002, ISSN 0953-4075
Publisher: Institute of Physics Publishing
DOI: 10.1088/1361-6455/aac351

Communication: Switched wave packets with spectrally truncated chirped pulses

Author(s): Adam S. Chatterley, Evangelos T. Karamatskos, Constant Schouder, Lars Christiansen, Anders V. Jørgensen, Terry Mullins, Jochen Küpper, Henrik Stapelfeldt
Published in: The Journal of Chemical Physics, Issue 148/22, 2018, Page(s) 221105, ISSN 0021-9606
Publisher: American Institute of Physics
DOI: 10.1063/1.5028359

43 W, 155 μm and 125 W, 31 μm dual-beam, sub-10 cycle, 100 kHz optical parametric chirped pulse amplifier

Author(s): Mark Mero, Zsuzsanna Heiner, Valentin Petrov, Horst Rottke, Federico Branchi, Gabrielle M. Thomas, Marc J. J. Vrakking
Published in: Optics Letters, Issue 43/21, 2018, Page(s) 5246, ISSN 0146-9592
Publisher: Optical Society of America
DOI: 10.1364/OL.43.005246

Accessing the molecular frame through strong-field alignment of distributions of gas phase molecules

Author(s): Katharine L. Reid
Published in: Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Issue 376/2115, 2018, Page(s) 20170158, ISSN 1364-503X
Publisher: Royal Society of London
DOI: 10.1098/rsta.2017.0158

Long-lasting field-free alignment of large molecules inside helium nanodroplets

Author(s): Adam S. Chatterley, Constant Schouder, Lars Christiansen, Benjamin Shepperson, Mette Heidemann Rasmussen, Henrik Stapelfeldt
Published in: Nature Communications, Issue 10/1, 2019, ISSN 2041-1723
Publisher: Nature Publishing Group
DOI: 10.1038/s41467-018-07995-0

Structure determination of the tetracene dimer in helium nanodroplets using femtosecond strong-field ionization

Author(s): Constant Schouder, Adam S. Chatterley, Florent Calvo, Lars Christiansen, Henrik Stapelfeldt
Published in: Structural Dynamics, Issue 6/4, 2019, Page(s) 044301, ISSN 2329-7778
Publisher: American Crystallographic Association
DOI: 10.1063/1.5118005

Laser-induced alignment dynamics of gas phase CS 2 dimers

Author(s): Adam S. Chatterley, Mia O. Baatrup, Constant A. Schouder, Henrik Stapelfeldt
Published in: Physical Chemistry Chemical Physics, Issue 22/6, 2020, Page(s) 3245-3253, ISSN 1463-9076
Publisher: Royal Society of Chemistry
DOI: 10.1039/c9cp06260b

Photon-Momentum-Induced Molecular Dynamics in Photoionization of N 2 at h ν

Author(s): M. Kircher, J. Rist, F. Trinter, S. Grundmann, M. Waitz, N. Melzer, I. Vela-Perez, T. Mletzko, A. Pier, N. Strenger, J. Siebert, R. Janssen, V. Honkimäki, J. Drnec, Ph. V. Demekhin, L. Ph. H. Schmidt, M. S. Schöffler, T. Jahnke, R. Dörner
Published in: Physical Review Letters, Issue 123/19, 2019, ISSN 0031-9007
Publisher: American Physical Society
DOI: 10.1103/physrevlett.123.193001

Kinematically complete experimental study of Compton scattering at helium atoms near the threshold

Author(s): Max Kircher, Florian Trinter, Sven Grundmann, Isabel Vela-Perez, Simon Brennecke, Nicolas Eicke, Jonas Rist, Sebastian Eckart, Salim Houamer, Ochbadrakh Chuluunbaatar, Yuri V. Popov, Igor P. Volobuev, Kai Bagschik, M. Novella Piancastelli, Manfred Lein, Till Jahnke, Markus S. Schöffler, Reinhard Dörner
Published in: Nature Physics, 2020, ISSN 1745-2473
Publisher: Nature Publishing Group
DOI: 10.1038/s41567-020-0880-2

Breakdown of the Spectator Concept in Low-Electron-Energy Resonant Decay Processes

Author(s): A. Mhamdi, J. Rist, D. Aslitürk, M. Weller, N. Melzer, D. Trabert, M. Kircher, I. Vela-Pérez, J. Siebert, S. Eckart, S. Grundmann, G. Kastirke, M. Waitz, A. Khan, M. S. Schöffler, F. Trinter, R. Dörner, T. Jahnke, Ph. V. Demekhin
Published in: Physical Review Letters, Issue 121/24, 2018, ISSN 0031-9007
Publisher: American Physical Society
DOI: 10.1103/physrevlett.121.243002

Recoil-Induced Asymmetry of Nondipole Molecular Frame Photoelectron Angular Distributions in the Hard X-ray Regime

Author(s): M. Kircher, J. Rist, F. Trinter, S. Grundmann, M. Waitz, N. Melzer, I. Vela-Pérez, T. Mletzko, A. Pier, N. Strenger, J. Siebert, R. Janssen, L. Ph. H. Schmidt, A. N. Artemyev, M. S. Schöffler, T. Jahnke, R. Dörner, Ph. V. Demekhin
Published in: Physical Review Letters, Issue 123/24, 2019, ISSN 0031-9007
Publisher: American Physical Society
DOI: 10.1103/physrevlett.123.243201

Frustrated Coulomb explosion of small helium clusters

Author(s): S. Kazandjian, J. Rist, M. Weller, F. Wiegandt, D. Aslitürk, S. Grundmann, M. Kircher, G. Nalin, D. Pitters, I. Vela Pérez, M. Waitz, G. Schiwietz, B. Griffin, J. B. Williams, R. Dörner, M. Schöffler, T. Miteva, F. Trinter, T. Jahnke, N. Sisourat
Published in: Physical Review A, Issue 98/5, 2018, ISSN 2469-9926
Publisher: American Physical Society
DOI: 10.1103/physreva.98.050701

Molecular Orbital Tomography Based on High-Order Harmonic Generation: Principles and Perspectives

Author(s): Anna Gabriella Ciriolo, Michele Devetta, Davide Faccialà, Prabhash Prasannan Geetha, Aditya Pusala, Caterina Vozzi, Salvatore Stagira
Published in: Advances in the Application of Lasers in Materials Science, Issue 274, 2018, Page(s) 191-216, ISBN 978-3-319-96844-5
Publisher: Springer International Publishing
DOI: 10.1007/978-3-319-96845-2_7

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