Angular studies of photoelectrons in innovative research environments

Livrables

Multiphoton PECD from limonene demonstrated
Generation of high harmonics from an OPCPA
Measurement and interpretation of MF-PADs from alanine
PhD theses
Demonstration of PECD on aromatic amino-acids (Tyrosine and/or tryptophane): from the monomers to the nanoparticles
Measurement of MFPADs from oriented OCS molecules with few-cycle carrier envelope stable laser pulses
Measurement of PADs from aligned benzonitrile
Demonstration of Coulomb explosion imaging from selected bonds in an organic chiral molecule
Publications in the primary literature
Measurement of MFPADs from NO2 using coincidence methodology
Laser induced electron diffraction measurements of complex molecular systems, such as molecules embedded in He nanodroplets
3D PADs following the excitation of wavepackets in molecules

Availability of multidimensional imaging detectors
Availability of detectors capable of discriminating the multiple charged particles ejected following the interaction of complex molecules with extreme radiation
Availability of new software for data storage and analysis

Project website up and running

Outreach events
Advertising vacancies
Organization of network events
Training courses and workshops

Publications

CEP-stable few-cycle pulses with more than 190 μJ of energy at 100 kHz from a noncollinear optical parametric amplifier

Auteurs: Federico J. Furch, Tobias Witting, Achut Giree, Chao Luan, Felix Schell, Gunnar Arisholm, Claus P. Schulz, Marc J. J. Vrakking
Publié dans: Optics Letters, Numéro 42/13, 2017, Page(s) 2495, ISSN 0146-9592
Éditeur: Optical Society of America
DOI: 10.1364/OL.42.002495

Intense Vibronic Modulation of the Chiral Photoelectron Angular Distribution Generated by Photoionization of Limonene Enantiomers with Circularly Polarized Synchrotron Radiation

Auteurs: Mohammad M. Rafiee Fanood, Hassan Ganjitabar, Gustavo A. Garcia, Laurent Nahon, Stefano Turchini, Ivan Powis
Publié dans: ChemPhysChem, Numéro 19/8, 2018, Page(s) 921-933, ISSN 1439-4235
Éditeur: John Wiley & Sons Ltd.
DOI: 10.1002/cphc.201701248

Multiple-orbital effects in laser-induced electron diffraction of aligned molecules

Auteurs: Faruk Krečinić, Philipp Wopperer, Biagio Frusteri, Felix Brauße, Jean-Gabriel Brisset, Umberto De Giovannini, Angel Rubio, Arnaud Rouzée, Marc J. J. Vrakking
Publié dans: Physical Review A, Numéro 98/4, 2018, ISSN 2469-9926
Éditeur: American Physical Society
DOI: 10.1103/PhysRevA.98.041401

Electron asymmetries in the photoionization of chiral molecules: possible astrophysical implications

Auteurs: Rim Hadidi, Dusan K. Bozanic, Gustavo A. Garcia, Laurent Nahon
Publié dans: Advances in Physics: X, Numéro 3/1, 2018, Page(s) 1477530, ISSN 2374-6149
Éditeur: Taylor-Francis
DOI: 10.1080/23746149.2018.1477530

Vibrationally-resolved photoelectron spectroscopy and photoelectron circular dichroism of bicyclic monoterpene enantiomers

Auteurs: Hassan Ganjitabar, Rim Hadidi, Gustavo A. Garcia, Laurent Nahon, Ivan Powis
Publié dans: Journal of Molecular Spectroscopy, Numéro 353, 2018, Page(s) 11-19, ISSN 0022-2852
Éditeur: Academic Press
DOI: 10.1016/j.jms.2018.08.007

High-order harmonic generation spectroscopy by recolliding electron caustics

Auteurs: D Faccialà, S Pabst, B D Bruner, A G Ciriolo, M Devetta, M Negro, P Prasannan Geetha, A Pusala, H Soifer, N Dudovich, S Stagira, C Vozzi
Publié dans: Journal of Physics B: Atomic, Molecular and Optical Physics, Numéro 51/13, 2018, Page(s) 134002, ISSN 0953-4075
Éditeur: Institute of Physics Publishing
DOI: 10.1088/1361-6455/aac351

Communication: Switched wave packets with spectrally truncated chirped pulses

Auteurs: Adam S. Chatterley, Evangelos T. Karamatskos, Constant Schouder, Lars Christiansen, Anders V. Jørgensen, Terry Mullins, Jochen Küpper, Henrik Stapelfeldt
Publié dans: The Journal of Chemical Physics, Numéro 148/22, 2018, Page(s) 221105, ISSN 0021-9606
Éditeur: American Institute of Physics
DOI: 10.1063/1.5028359

43 W, 155 μm and 125 W, 31 μm dual-beam, sub-10 cycle, 100 kHz optical parametric chirped pulse amplifier

Auteurs: Mark Mero, Zsuzsanna Heiner, Valentin Petrov, Horst Rottke, Federico Branchi, Gabrielle M. Thomas, Marc J. J. Vrakking
Publié dans: Optics Letters, Numéro 43/21, 2018, Page(s) 5246, ISSN 0146-9592
Éditeur: Optical Society of America
DOI: 10.1364/OL.43.005246

Accessing the molecular frame through strong-field alignment of distributions of gas phase molecules

Auteurs: Katharine L. Reid
Publié dans: Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Numéro 376/2115, 2018, Page(s) 20170158, ISSN 1364-503X
Éditeur: Royal Society of London
DOI: 10.1098/rsta.2017.0158

Long-lasting field-free alignment of large molecules inside helium nanodroplets

Auteurs: Adam S. Chatterley, Constant Schouder, Lars Christiansen, Benjamin Shepperson, Mette Heidemann Rasmussen, Henrik Stapelfeldt
Publié dans: Nature Communications, Numéro 10/1, 2019, ISSN 2041-1723
Éditeur: Nature Publishing Group
DOI: 10.1038/s41467-018-07995-0

Structure determination of the tetracene dimer in helium nanodroplets using femtosecond strong-field ionization

Auteurs: Constant Schouder, Adam S. Chatterley, Florent Calvo, Lars Christiansen, Henrik Stapelfeldt
Publié dans: Structural Dynamics, Numéro 6/4, 2019, Page(s) 044301, ISSN 2329-7778
Éditeur: American Crystallographic Association
DOI: 10.1063/1.5118005

Laser-induced alignment dynamics of gas phase CS 2 dimers

Auteurs: Adam S. Chatterley, Mia O. Baatrup, Constant A. Schouder, Henrik Stapelfeldt
Publié dans: Physical Chemistry Chemical Physics, Numéro 22/6, 2020, Page(s) 3245-3253, ISSN 1463-9076
Éditeur: Royal Society of Chemistry
DOI: 10.1039/c9cp06260b

Photon-Momentum-Induced Molecular Dynamics in Photoionization of N 2 at h ν

Auteurs: M. Kircher, J. Rist, F. Trinter, S. Grundmann, M. Waitz, N. Melzer, I. Vela-Perez, T. Mletzko, A. Pier, N. Strenger, J. Siebert, R. Janssen, V. Honkimäki, J. Drnec, Ph. V. Demekhin, L. Ph. H. Schmidt, M. S. Schöffler, T. Jahnke, R. Dörner
Publié dans: Physical Review Letters, Numéro 123/19, 2019, ISSN 0031-9007
Éditeur: American Physical Society
DOI: 10.1103/physrevlett.123.193001

Kinematically complete experimental study of Compton scattering at helium atoms near the threshold

Auteurs: Max Kircher, Florian Trinter, Sven Grundmann, Isabel Vela-Perez, Simon Brennecke, Nicolas Eicke, Jonas Rist, Sebastian Eckart, Salim Houamer, Ochbadrakh Chuluunbaatar, Yuri V. Popov, Igor P. Volobuev, Kai Bagschik, M. Novella Piancastelli, Manfred Lein, Till Jahnke, Markus S. Schöffler, Reinhard Dörner
Publié dans: Nature Physics, 2020, ISSN 1745-2473
Éditeur: Nature Publishing Group
DOI: 10.1038/s41567-020-0880-2

Breakdown of the Spectator Concept in Low-Electron-Energy Resonant Decay Processes

Auteurs: A. Mhamdi, J. Rist, D. Aslitürk, M. Weller, N. Melzer, D. Trabert, M. Kircher, I. Vela-Pérez, J. Siebert, S. Eckart, S. Grundmann, G. Kastirke, M. Waitz, A. Khan, M. S. Schöffler, F. Trinter, R. Dörner, T. Jahnke, Ph. V. Demekhin
Publié dans: Physical Review Letters, Numéro 121/24, 2018, ISSN 0031-9007
Éditeur: American Physical Society
DOI: 10.1103/physrevlett.121.243002

Recoil-Induced Asymmetry of Nondipole Molecular Frame Photoelectron Angular Distributions in the Hard X-ray Regime

Auteurs: M. Kircher, J. Rist, F. Trinter, S. Grundmann, M. Waitz, N. Melzer, I. Vela-Pérez, T. Mletzko, A. Pier, N. Strenger, J. Siebert, R. Janssen, L. Ph. H. Schmidt, A. N. Artemyev, M. S. Schöffler, T. Jahnke, R. Dörner, Ph. V. Demekhin
Publié dans: Physical Review Letters, Numéro 123/24, 2019, ISSN 0031-9007
Éditeur: American Physical Society
DOI: 10.1103/physrevlett.123.243201

Frustrated Coulomb explosion of small helium clusters

Auteurs: S. Kazandjian, J. Rist, M. Weller, F. Wiegandt, D. Aslitürk, S. Grundmann, M. Kircher, G. Nalin, D. Pitters, I. Vela Pérez, M. Waitz, G. Schiwietz, B. Griffin, J. B. Williams, R. Dörner, M. Schöffler, T. Miteva, F. Trinter, T. Jahnke, N. Sisourat
Publié dans: Physical Review A, Numéro 98/5, 2018, ISSN 2469-9926
Éditeur: American Physical Society
DOI: 10.1103/physreva.98.050701

Molecular Orbital Tomography Based on High-Order Harmonic Generation: Principles and Perspectives

Auteurs: Anna Gabriella Ciriolo, Michele Devetta, Davide Faccialà, Prabhash Prasannan Geetha, Aditya Pusala, Caterina Vozzi, Salvatore Stagira
Publié dans: Advances in the Application of Lasers in Materials Science, Numéro 274, 2018, Page(s) 191-216, ISBN 978-3-319-96844-5
Éditeur: Springer International Publishing
DOI: 10.1007/978-3-319-96845-2_7

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