Livrables Documents, reports (6) Assessment of the State-of-the-Art of mult-physics modeling of gel-based and all-solid-state Li-Ion batteries The state-of-the-art on multi-physics modeling of electrochemical energy storage systems will be assessed and the resulting document will be shared with the consortium. Both gel-based and all-solid-state Li-Ion technologies will be considered. Evaluation of generic processes for ceramic and composites The main objective is to evaluate the generic processes developed previously and adapt them for as broad use as possible. The promising electrolyte candidates identified in WP7 will be ranked in terms of processability, costs and upscale production, always considering their physicochemical and electrochemical properties. Environmental assessment A prospective life cycle assessment LCA will be conducted by the VUB The full LCA will identify the key performance indicators for the environmental impact including climate change energy efficiency resource depletion toxicity during mining water footprint land usage and external cost calculation Furthermore the environmental impacts will be complemented with social impacts to highlight the excellence on sustainability Study on the impact of future cell technologies on module and pack concept The goal is to evaluate the implication of ASSB properties on module and pack concepts One of the most significant property with a very high potential impact is the operating temperature which is usually higher than in the stateoftheart Li ion technologies Roadmap for competitive production of all-solid batteries including considerations of other emerging technologies The roadmap will provide an overall vision of potential processes within the different stages of manufacturing and the impact they could provide in terms of cost quality performance safety and lifetime Special emphasis will be given to the applicability of the manufacturing solutions to the several emerging battery technology possibilities and the identification of potential breakthroughs related to production Furthermore the potential benefits and future markets of novel production Technologies will be identified and evaluated Document with final Cell Requirement and Specification for Automotive and Stationary Application The top-level Li-ion cell specifications and requirements will be broken down from the requirements for an automotive and a stationary battery-system to provide a real industrial guideline. BMW is responsible for the automotive requirements and VARTA Storage for the stationary requirements. Websites, patent fillings, videos etc. (1) Project Website VMB will develop and maintain a project website and corporative image including logo flyer rollups in order to create a project identity increase the awareness of IMAGE and provide the interested public with information concerning the project itself and other relevant topics and events Publications Peer reviewed articles (24) Rapid Low-Dimensional Li + Ion Hopping Processes in Synthetic Hectorite-Type Li 0.5 [Mg 2.5 Li 0.5 ]Si 4 O 10 F 2 Auteurs: Caroline Hiebl, Patrick Loch, Marina Brinek, Maria Gombotz, Bernhard Gadermaier, Paul Heitjans, Josef Breu, H. Martin. R. Wilkening Publié dans: Chemistry of Materials, Issue 32/17, 2020, Page(s) 7445-7457, ISSN 0897-4756 Éditeur: American Chemical Society DOI: 10.1021/acs.chemmater.0c02460 Fuzzy logic: about the origins of fast ion dynamics in crystalline solids Auteurs: M. Gombotz, K. Hogrefe, R. Zettl, B. Gadermaier, H. Martin. R. Wilkening Publié dans: Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Issue 379/2211, 2021, ISSN 1364-503X Éditeur: Royal Society of London DOI: 10.1098/rsta.2020.0434 The Electronic Conductivity of Single Crystalline Ga‐Stabilized Cubic Li 7 La 3 Zr 2 O 12 : A Technologically Relevant Parameter for All‐Solid‐State Batteries Auteurs: Martin Philipp, Bernhard Gadermaier, Patrick Posch, Ilie Hanzu, Steffen Ganschow, Martin Meven, Daniel Rettenwander, Günther J. Redhammer, H. Martin R. Wilkening Publié dans: Advanced Materials Interfaces, Issue 7/16, 2020, Page(s) 2000450, ISSN 2196-7350 Éditeur: John Wiley & Sons DOI: 10.1002/admi.202000450 Structural Disorder in Li 6 PS 5 I Speeds 7 Li Nuclear Spin Recovery and Slows Down 31 P Relaxation–Implications for Translational and Rotational Jumps as Seen by Nuclear Magnetic Resonance Auteurs: M. Brinek, C. Hiebl, K. Hogrefe, I. Hanghofer, H. M. R. Wilkening Publié dans: The Journal of Physical Chemistry C, Issue 124/42, 2020, Page(s) 22934-22940, ISSN 1932-7447 Éditeur: American Chemical Society DOI: 10.1021/acs.jpcc.0c06090 Conductor–Insulator Interfaces in Solid Electrolytes: A Design Strategy to Enhance Li-Ion Dynamics in Nanoconfined LiBH 4 /Al 2 O 3 Auteurs: Roman Zettl, Katharina Hogrefe, Bernhard Gadermaier, Ilie Hanzu, Peter Ngene, Petra E. de Jongh, H. Martin R. Wilkening Publié dans: The Journal of Physical Chemistry C, Issue 125/27, 2021, Page(s) 15052-15060, ISSN 1932-7447 Éditeur: American Chemical Society DOI: 10.1021/acs.jpcc.1c03789 Improvement of Lithium Metal Polymer Batteries through a Small Dose of Fluorinated Salt Auteurs: Alexander Santiago, Xabier Judez, Julen Castillo, Iñigo Garbayo, Amaia Sáenz de Buruaga, Lixin Qiao, Giorgio Baraldi, José Antonio Coca-Clemente, Michel Armand, Chunmei Li, Heng Zhang Publié dans: The Journal of Physical Chemistry Letters, Issue 11/15, 2020, Page(s) 6133-6138, ISSN 1948-7185 Éditeur: American Chemical Society DOI: 10.1021/acs.jpclett.0c01883 Incremental Pressure Curves to Assess Capacity Fade in Next-Generation Li-ion Pouch Cells Auteurs: Lysander De Sutter, Gert Berckmans, Mario Marinaro, Joeri Van Mierlo Publié dans: IEEE Conference on Vehicle Power and Propulsion, 2019, ISSN 1938-8756 Éditeur: IEEE DOI: 10.1109/vppc46532.2019.8952313 Lithium solid-state batteries: State-of-the-art and challenges for materials, interfaces and processing Auteurs: Nicola Boaretto, Iñigo Garbayo, Sona Valiyaveettil Sobhanraj, Amaia Quintela, Chunmei Li, Montse Casas-Cabanas, Frederic Aguesse Publié dans: Journal of Power Sources, Issue 502, 2021, Page(s) 229919, ISSN 0378-7753 Éditeur: Elsevier BV DOI: 10.1016/j.jpowsour.2021.229919 Production of high-energy Li-ion batteries comprising silicon-containing anodes and insertion-type cathodes Auteurs: Gebrekidan Gebresilassie Eshetu, Heng Zhang, Xabier Judez, Henry Adenusi, Michel Armand, Stefano Passerini and Egbert Figgemeier Publié dans: Nature Communications, Issue 5459/12, 2021, ISSN 2041-1723 Éditeur: Nature Publishing Group DOI: 10.1038/s41467-021-25334-8 Realizing a high-performance LiNi 0.6 Mn 0.2 Co 0.2 O 2 /silicon–graphite full lithium ion battery cell via a designer electrolyte additive Auteurs: Felix Aupperle, Gebrekidan Gebresilassie Eshetu, Kevin W. Eberman, Ang Xioa, Jean-Sebastien Bridel, Egbert Figgemeier Publié dans: Journal of Materials Chemistry A, Issue 8/37, 2020, Page(s) 19573-19587, ISSN 2050-7488 Éditeur: Royal Society of Chemistry DOI: 10.1039/d0ta05827k High Li+ and Na+ Conductivity in New Hybrid Solid Electrolytes based on the Porous MIL-121 Metal Organic Framework Auteurs: Roman Zettl, Sarah Lunghammer, Bernhard Gadermaier, Athmane Boulaoued, Patrik Johansson,H. Martin R. Wilkening, Ilie Hanzu Publié dans: Advanced Energy Materials, Issue 11/16, 2021, Page(s) 2003542, ISSN 1614-6832 Éditeur: Wiley-VCH Verlag DOI: 10.1002/aenm.202003542 Suppressed Mobility of Negative Charges in Polymer Electrolytes with an Ether‐Functionalized Anion Auteurs: Heng Zhang, Fangfang Chen, Oier Lakuntza, Uxue Oteo, Lixin Qiao, Maria Martinez‐Ibañez, Haijin Zhu, Javier Carrasco, Maria Forsyth, Michel Armand Publié dans: Angewandte Chemie, Issue 131/35, 2019, Page(s) 12198-12203, ISSN 0044-8249 Éditeur: John Wiley & Sons Ltd. DOI: 10.1002/ange.201905794 Importance of Composite Electrolyte Processing to Improve the Kinetics and Energy Density of Li Metal Solid-State Batteries Auteurs: Jakub Zagórski, Begoña Silván, Damien Saurel, Frédéric Aguesse, Anna Llordés Publié dans: ACS Applied Energy Materials, Issue 3/9, 2020, Page(s) 8344-8355, ISSN 2574-0962 Éditeur: American Chemical Society DOI: 10.1021/acsaem.0c00935 Lowering the Interfacial Resistance in Li6.4La3Zr1.4Ta0.6O12|Poly(Ethylene Oxide) Composite Electrolytes Auteurs: Eveline Kuhnert, Lukas Ladenstein, Anna Jodlbauer, Christian Slugovc, Gregor Trimmel, H. Martin R. Wilkening, Daniel Rettenwander Publié dans: Cell Reports Physical Science, Issue 1/10, 2020, Page(s) 100214, ISSN 2666-3864 Éditeur: Elsevier DOI: 10.1016/j.xcrp.2020.100214 Fast Li Ion Dynamics in the Mechanosynthesized Nanostructured Form of the Solid Electrolyte Li 3 YBr 6 Auteurs: Maria Gombotz, H. Martin R. Wilkening Publié dans: ACS Sustainable Chemistry & Engineering, Issue 9/2, 2021, Page(s) 743-755, ISSN 2168-0485 Éditeur: American Chemical Society DOI: 10.1021/acssuschemeng.0c06694 Lithium ion dynamics in LiZr 2 (PO 4 ) 3 and Li 1.4 Ca 0.2 Zr 1.8 (PO 4 ) 3 Auteurs: Isabel Hanghofer, Bernhard Gadermaier, Alexandra Wilkening, Daniel Rettenwander, H. Martin R. Wilkening Publié dans: Dalton Transactions, 2019, ISSN 1477-9226 Éditeur: Royal Society of Chemistry DOI: 10.1039/c9dt01786k Fast Rotational Dynamics in Argyrodite-Type Li 6 PS 5 X (X: Cl, Br, I) as Seen by 31 P Nuclear Magnetic Relaxation—On Cation–Anion Coupled Transport in Thiophosphates Auteurs: Isabel Hanghofer, Bernhard Gadermaier, H. Martin R. Wilkening Publié dans: Chemistry of Materials, 2019, ISSN 0897-4756 Éditeur: American Chemical Society DOI: 10.1021/acs.chemmater.9b01435 Understanding the Origin of Enhanced Li-Ion Transport in Nanocrystalline Argyrodite-Type Li 6 PS 5 I Auteurs: Marina Brinek, Caroline Hiebl, H. Martin R. Wilkening Publié dans: Chemistry of Materials, Issue 32/11, 2020, Page(s) 4754-4766, ISSN 0897-4756 Éditeur: American Chemical Society DOI: 10.1021/acs.chemmater.0c01367 In Situ Optical Investigations of Lithium Depositions on Pristine and Aged Lithium Metal Electrodes Auteurs: Hannes Kühnle, Edwin Knobbe and Egbert Figgemeier Publié dans: Journal of The Electrochemical Society, Issue 168, 2021, Page(s) 020510, ISSN 0013-4651 Éditeur: Electrochemical Society, Inc. DOI: 10.1149/1945-7111/abdeeb Direct Assessment of Ultralow Li+ Jump Rates in Single Crystalline Li3N by Evolution-Time-Resolved 7Li Spin-Alignment Echo NMR Auteurs: Bernhard Gadermaier, Katharina Hogrefe, Prof. Dr. Paul Heitjans, Prof. Dr. H. Martin R. Wilkening Publié dans: European Journal of Inorganic Chemistry, 2021, Page(s) 1028-1033, ISSN 1434-1948 Éditeur: John Wiley & Sons Ltd. DOI: 10.1002/ejic.202000941 Anomalies in Bulk Ion Transport in the Solid Solutions of Li 7 La 3 M 2 O 12 (M = Hf, Sn) and Li 5 La 3 Ta 2 O 12 Auteurs: Lukas Ladenstein, Sanja Simic, Gerald Kothleitner, Daniel Rettenwander, H. Martin R. Wilkening Publié dans: The Journal of Physical Chemistry C, Issue 124/31, 2020, Page(s) 16796-16805, ISSN 1932-7447 Éditeur: American Chemical Society DOI: 10.1021/acs.jpcc.0c03558 Ion dynamics in Al-Stabilized Li7La3Zr2O12 single crystals – Macroscopic transport and the elementary steps of ion hopping Auteurs: Patrick Posch, Sarah Lunghammer, Stefan Berendts, Steffen Ganschow, Günther J. Redhammer, Alexandra Wilkening, Martin Lerch, Bernhard Gadermaier, Daniel Rettenwander, H. Martin R. Wilkening Publié dans: Energy Storage Materials, Issue 24, 2020, Page(s) 220-228, ISSN 2405-8297 Éditeur: Elsevier DOI: 10.1016/j.ensm.2019.08.017 With a Little Help from 31 P NMR: The Complete Picture on Localized and Long-Range Li + Diffusion in Li 6 PS 5 I Auteurs: Katharina Hogrefe, Isabel Hanghofer, H. Martin R. Wilkening Publié dans: The Journal of Physical Chemistry C, Issue 125/41, 2021, Page(s) 22457-22463, ISSN 1932-7447 Éditeur: American Chemical Society DOI: 10.1021/acs.jpcc.1c06242 Tracking Ions the Direct Way: Long-Range Li + Dynamics in the Thio-LISICON Family Li 4 MCh 4 (M = Sn, Ge; Ch = S, Se) as Probed by 7 Li NMR Relaxometry and 7 Li Spin-Alignment Echo NMR Auteurs: Katharina Hogrefe, Nicolò Minafra, Wolfgang G. Zeier, H. Martin R. Wilkening Publié dans: The Journal of Physical Chemistry C, Issue 125/4, 2021, Page(s) 2306-2317, ISSN 1932-7447 Éditeur: American Chemical Society DOI: 10.1021/acs.jpcc.0c10224 Recherche de données OpenAIRE... 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