Critical Raw material ElectrocatalystS replacement ENabling Designed pOst-2020 PEMFC

Livrables

Report on the ex situ AST peroxide protocol definition and its application to selected benchmark catalysts
Report on site density and turn over frequency of selected benchmark catalysts
Report on the benchmarking of international state-of-the-art (industrial academic) non-PGM catalysts and/or CCMs
Ultra-low PGM anode catalyst with improved resistance to CO poisoning
Final report on WP achievements in terms of activity of new catalysts
Report on cell and system requirements and cell testing protocols
Survey of dissemination activities and final plan for dissemination and exploitation of project results

Project website
"Organisation of the 2nd conference on “Challenges for Zero Platinum for Oxygen Reduction and Hydrogen Oxidation"""

Publications

Stable, Active, and Methanol-Tolerant PGM-Free Surfaces in an Acidic Medium: Electron Tunneling at Play in Pt/FeNC Hybrid Catalysts for Direct Methanol Fuel Cell Cathodes

Auteurs: Tomasz Kosmala, Nicolas Bibent, Moulay Tahar Sougrati, Goran Dražić, Stefano Agnoli, Frédéric Jaouen, Gaetano Granozzi
Publié dans: ACS Catalysis, Numéro 10/14, 2020, Page(s) 7475-7485, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.0c01288

Deactivation, reactivation and super-activation of Fe-N/C oxygen reduction electrocatalysts: Gas sorption, physical and electrochemical investigation using NO and O2

Auteurs: Paul Boldrin, Daniel Malko, Asad Mehmood, Ulrike I. Kramm, Stephan Wagner, Stephen Paul, Natascha Weidler, Anthony Kucernak
Publié dans: Applied Catalysis B: Environmental, Numéro 292, 2021, Page(s) 120169, ISSN 0926-3373
Éditeur: Elsevier BV
DOI: 10.1016/j.apcatb.2021.120169

Identification of durable and non-durable FeNx sites in Fe–N–C materials for proton exchange membrane fuel cells

Auteurs: Jingkun Li, Moulay Tahar Sougrati, Andrea Zitolo, James M. Ablett, Ismail Can Oğuz, Tzonka Mineva, Ivana Matanovic, Plamen Atanassov, Ying Huang, Iryna Zenyuk, Andrea Di Cicco, Kavita Kumar, Laetitia Dubau, Frédéric Maillard, Goran Dražić, Frédéric Jaouen
Publié dans: Nature Catalysis, Numéro 4/1, 2021, Page(s) 10-19, ISSN 2520-1158
Éditeur: Springer Nature
DOI: 10.1038/s41929-020-00545-2

Understanding Active Sites in Pyrolyzed Fe–N–C Catalysts for Fuel Cell Cathodes by Bridging Density Functional Theory Calculations and 57 Fe Mössbauer Spectroscopy

Auteurs: Tzonka Mineva, Ivana Matanovic, Plamen Atanassov, Moulay-Tahar Sougrati, Lorenzo Stievano, Martin Clémancey, Amélie Kochem, Jean-Marc Latour, Frédéric Jaouen
Publié dans: ACS Catalysis, Numéro 9/10, 2019, Page(s) 9359-9371, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.9b02586

Noncovalent Integration of a Bioinspired Ni Catalyst to Graphene Acid for Reversible Electrocatalytic Hydrogen Oxidation

Auteurs: Bertrand Reuillard, Matías Blanco, Laura Calvillo, Nathan Coutard, Ahmed Ghedjatti, Pascale Chenevier, Stefano Agnoli, Michal Otyepka, Gaetano Granozzi, Vincent Artero
Publié dans: ACS Applied Materials & Interfaces, Numéro 12/5, 2020, Page(s) 5805-5811, ISSN 1944-8244
Éditeur: American Chemical Society
DOI: 10.1021/acsami.9b18922

Sulfur Doping versus Hierarchical Pore Structure: The Dominating Effect on the Fe–N–C Site Density, Activity, and Selectivity in Oxygen Reduction Reaction Electrocatalysis

Auteurs: Giorgia Daniel, Marco Mazzucato, Riccardo Brandiele, Laura De Lazzari, Denis Badocco, Paolo Pastore, Tomasz Kosmala, Gaetano Granozzi, Christian Durante
Publié dans: ACS Applied Materials & Interfaces, Numéro 13/36, 2021, Page(s) 42693-42705, ISSN 1944-8244
Éditeur: American Chemical Society
DOI: 10.1021/acsami.1c09659

Effects of the induced micro- and meso-porosity on the single site density and turn over frequency of Fe-N-C carbon electrodes for the oxygen reduction reaction

Auteurs: Marco Mazzucato, Giorgia Daniel, Asad Mehmood, Tomasz Kosmala, Gaetano Granozzi, Anthony Kucernak, Christian Durante
Publié dans: Applied Catalysis B: Environmental, Numéro 291, 2021, Page(s) 120068, ISSN 0926-3373
Éditeur: Elsevier BV
DOI: 10.1016/j.apcatb.2021.120068

Advancements in cathode catalyst and cathode layer design for proton exchange membrane fuel cells

Auteurs: Yanyan Sun, Shlomi Polani, Fang Luo, Sebastian Ott, Peter Strasser, Fabio Dionigi
Publié dans: Nature Communications, Numéro 12/1, 2021, ISSN 2041-1723
Éditeur: Nature Publishing Group
DOI: 10.1038/s41467-021-25911-x

Highly Graphitized Fe-N-C Electrocatalysts Prepared from Chitosan Hydrogel Frameworks

Auteurs: Giorgia Daniel, Tomasz Kosmala, Federico Brombin, Marco Mazzucato, Alessandro Facchin, Maria Chiara Dalconi, Denis Badocco, Paolo Pastore, Gaetano Granozzi, Christian Durante
Publié dans: Catalysts, Numéro 11/3, 2021, Page(s) 390, ISSN 2073-4344
Éditeur: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/catal11030390

Toward Platinum Group Metal-Free Catalysts for Hydrogen/Air Proton-Exchange Membrane Fuel Cells

Auteurs: Frédéric Jaouen, Deborah Jones, Nathan Coutard, Vincent Artero, Peter Strasser, Anthony Kucernak
Publié dans: Johnson Matthey Technology Review, Numéro 62/2, 2018, Page(s) 231-255, ISSN 2056-5135
Éditeur: Johnson Matthey plc
DOI: 10.1595/205651318x696828

Accurate Evaluation of Active-Site Density (SD) and Turnover Frequency (TOF) of PGM-Free Metal–Nitrogen-Doped Carbon (MNC) Electrocatalysts using CO Cryo Adsorption

Auteurs: Fang Luo, Chang Hyuck Choi, Mathias J.M. Primbs, Wen Ju, Shuang Li, Nathaniel D. Leonard, Arne Thomas, Frédéric Jaouen, Peter Strasser
Publié dans: ACS Catalysis, Numéro 9/6, 2019, Page(s) 4841-4852, ISSN 2155-5435
Éditeur: American Chemical Society
DOI: 10.1021/acscatal.9b00588

Impact of ionomer structuration on the performance of bio-inspired noble-metal-free fuel cell anodes

Auteurs: Nathan Coutard, Bertrand Reuillard, Tran Ngoc Huan, Fabrice Valentino, Reuben T. Jane, Solène Gentil, Eugen S. Andreiadis, Alan Le Goff, Tristan Asset, Frédéric Maillard, Bruno Jousselme, Adina Morozan, Sandrine Lyonnard, Vincent Artero, Pascale Chenevier
Publié dans: Chem Catalysis, Numéro 1/1, 2021, Page(s) 88-105, ISSN 2667-1093
Éditeur: Elsevier
DOI: 10.1016/j.checat.2021.01.001

Establishing reactivity descriptors for platinum group metal (PGM)-free Fe–N–C catalysts for PEM fuel cells

Auteurs: Mathias Primbs, Yanyan Sun, Aaron Roy, Daniel Malko, Asad Mehmood, Moulay-Tahar Sougrati, Pierre-Yves Blanchard, Gaetano Granozzi, Tomasz Kosmala, Giorgia Daniel, Plamen Atanassov, Jonathan Sharman, Christian Durante, Anthony Kucernak, Deborah Jones, Frédéric Jaouen, Peter Strasser
Publié dans: Energy & Environmental Science, Numéro 13/8, 2020, Page(s) 2480-2500, ISSN 1754-5692
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0ee01013h

Upcycling of polyurethane into iron-nitrogen-carbon electrocatalysts active for oxygen reduction reaction

Auteurs: Giorgia Daniel, Tomasz Kosmala, Maria Chiara Dalconi, Luca Nodari, Denis Badocco, Paolo Pastore, Alessandra Lorenzetti, Gaetano Granozzi, Christian Durante
Publié dans: Electrochimica Acta, Numéro 362, 2020, Page(s) 137200, ISSN 0013-4686
Éditeur: Pergamon Press Ltd.
DOI: 10.1016/j.electacta.2020.137200

A comparative perspective of electrochemical and photochemical approaches for catalytic H 2 O 2 production

Auteurs: Yanyan Sun, Lei Han, Peter Strasser
Publié dans: Chemical Society Reviews, Numéro 49/18, 2020, Page(s) 6605-6631, ISSN 0306-0012
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0cs00458h

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