Critical Raw material ElectrocatalystS replacement ENabling Designed pOst-2020 PEMFC

Leistungen

Report on the ex situ AST peroxide protocol definition and its application to selected benchmark catalysts
Report on site density and turn over frequency of selected benchmark catalysts
Report on the benchmarking of international state-of-the-art (industrial academic) non-PGM catalysts and/or CCMs
Ultra-low PGM anode catalyst with improved resistance to CO poisoning
Final report on WP achievements in terms of activity of new catalysts
Report on cell and system requirements and cell testing protocols
Survey of dissemination activities and final plan for dissemination and exploitation of project results

Project website
"Organisation of the 2nd conference on “Challenges for Zero Platinum for Oxygen Reduction and Hydrogen Oxidation"""

Veröffentlichungen

Stable, Active, and Methanol-Tolerant PGM-Free Surfaces in an Acidic Medium: Electron Tunneling at Play in Pt/FeNC Hybrid Catalysts for Direct Methanol Fuel Cell Cathodes

Autoren: Tomasz Kosmala, Nicolas Bibent, Moulay Tahar Sougrati, Goran Dražić, Stefano Agnoli, Frédéric Jaouen, Gaetano Granozzi
Veröffentlicht in: ACS Catalysis, Ausgabe 10/14, 2020, Seite(n) 7475-7485, ISSN 2155-5435
Herausgeber: American Chemical Society
DOI: 10.1021/acscatal.0c01288

Deactivation, reactivation and super-activation of Fe-N/C oxygen reduction electrocatalysts: Gas sorption, physical and electrochemical investigation using NO and O2

Autoren: Paul Boldrin, Daniel Malko, Asad Mehmood, Ulrike I. Kramm, Stephan Wagner, Stephen Paul, Natascha Weidler, Anthony Kucernak
Veröffentlicht in: Applied Catalysis B: Environmental, Ausgabe 292, 2021, Seite(n) 120169, ISSN 0926-3373
Herausgeber: Elsevier BV
DOI: 10.1016/j.apcatb.2021.120169

Identification of durable and non-durable FeNx sites in Fe–N–C materials for proton exchange membrane fuel cells

Autoren: Jingkun Li, Moulay Tahar Sougrati, Andrea Zitolo, James M. Ablett, Ismail Can Oğuz, Tzonka Mineva, Ivana Matanovic, Plamen Atanassov, Ying Huang, Iryna Zenyuk, Andrea Di Cicco, Kavita Kumar, Laetitia Dubau, Frédéric Maillard, Goran Dražić, Frédéric Jaouen
Veröffentlicht in: Nature Catalysis, Ausgabe 4/1, 2021, Seite(n) 10-19, ISSN 2520-1158
Herausgeber: Springer Nature
DOI: 10.1038/s41929-020-00545-2

Understanding Active Sites in Pyrolyzed Fe–N–C Catalysts for Fuel Cell Cathodes by Bridging Density Functional Theory Calculations and 57 Fe Mössbauer Spectroscopy

Autoren: Tzonka Mineva, Ivana Matanovic, Plamen Atanassov, Moulay-Tahar Sougrati, Lorenzo Stievano, Martin Clémancey, Amélie Kochem, Jean-Marc Latour, Frédéric Jaouen
Veröffentlicht in: ACS Catalysis, Ausgabe 9/10, 2019, Seite(n) 9359-9371, ISSN 2155-5435
Herausgeber: American Chemical Society
DOI: 10.1021/acscatal.9b02586

Noncovalent Integration of a Bioinspired Ni Catalyst to Graphene Acid for Reversible Electrocatalytic Hydrogen Oxidation

Autoren: Bertrand Reuillard, Matías Blanco, Laura Calvillo, Nathan Coutard, Ahmed Ghedjatti, Pascale Chenevier, Stefano Agnoli, Michal Otyepka, Gaetano Granozzi, Vincent Artero
Veröffentlicht in: ACS Applied Materials & Interfaces, Ausgabe 12/5, 2020, Seite(n) 5805-5811, ISSN 1944-8244
Herausgeber: American Chemical Society
DOI: 10.1021/acsami.9b18922

Sulfur Doping versus Hierarchical Pore Structure: The Dominating Effect on the Fe–N–C Site Density, Activity, and Selectivity in Oxygen Reduction Reaction Electrocatalysis

Autoren: Giorgia Daniel, Marco Mazzucato, Riccardo Brandiele, Laura De Lazzari, Denis Badocco, Paolo Pastore, Tomasz Kosmala, Gaetano Granozzi, Christian Durante
Veröffentlicht in: ACS Applied Materials & Interfaces, Ausgabe 13/36, 2021, Seite(n) 42693-42705, ISSN 1944-8244
Herausgeber: American Chemical Society
DOI: 10.1021/acsami.1c09659

Effects of the induced micro- and meso-porosity on the single site density and turn over frequency of Fe-N-C carbon electrodes for the oxygen reduction reaction

Autoren: Marco Mazzucato, Giorgia Daniel, Asad Mehmood, Tomasz Kosmala, Gaetano Granozzi, Anthony Kucernak, Christian Durante
Veröffentlicht in: Applied Catalysis B: Environmental, Ausgabe 291, 2021, Seite(n) 120068, ISSN 0926-3373
Herausgeber: Elsevier BV
DOI: 10.1016/j.apcatb.2021.120068

Advancements in cathode catalyst and cathode layer design for proton exchange membrane fuel cells

Autoren: Yanyan Sun, Shlomi Polani, Fang Luo, Sebastian Ott, Peter Strasser, Fabio Dionigi
Veröffentlicht in: Nature Communications, Ausgabe 12/1, 2021, ISSN 2041-1723
Herausgeber: Nature Publishing Group
DOI: 10.1038/s41467-021-25911-x

Highly Graphitized Fe-N-C Electrocatalysts Prepared from Chitosan Hydrogel Frameworks

Autoren: Giorgia Daniel, Tomasz Kosmala, Federico Brombin, Marco Mazzucato, Alessandro Facchin, Maria Chiara Dalconi, Denis Badocco, Paolo Pastore, Gaetano Granozzi, Christian Durante
Veröffentlicht in: Catalysts, Ausgabe 11/3, 2021, Seite(n) 390, ISSN 2073-4344
Herausgeber: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/catal11030390

Toward Platinum Group Metal-Free Catalysts for Hydrogen/Air Proton-Exchange Membrane Fuel Cells

Autoren: Frédéric Jaouen, Deborah Jones, Nathan Coutard, Vincent Artero, Peter Strasser, Anthony Kucernak
Veröffentlicht in: Johnson Matthey Technology Review, Ausgabe 62/2, 2018, Seite(n) 231-255, ISSN 2056-5135
Herausgeber: Johnson Matthey plc
DOI: 10.1595/205651318x696828

Accurate Evaluation of Active-Site Density (SD) and Turnover Frequency (TOF) of PGM-Free Metal–Nitrogen-Doped Carbon (MNC) Electrocatalysts using CO Cryo Adsorption

Autoren: Fang Luo, Chang Hyuck Choi, Mathias J.M. Primbs, Wen Ju, Shuang Li, Nathaniel D. Leonard, Arne Thomas, Frédéric Jaouen, Peter Strasser
Veröffentlicht in: ACS Catalysis, Ausgabe 9/6, 2019, Seite(n) 4841-4852, ISSN 2155-5435
Herausgeber: American Chemical Society
DOI: 10.1021/acscatal.9b00588

Impact of ionomer structuration on the performance of bio-inspired noble-metal-free fuel cell anodes

Autoren: Nathan Coutard, Bertrand Reuillard, Tran Ngoc Huan, Fabrice Valentino, Reuben T. Jane, Solène Gentil, Eugen S. Andreiadis, Alan Le Goff, Tristan Asset, Frédéric Maillard, Bruno Jousselme, Adina Morozan, Sandrine Lyonnard, Vincent Artero, Pascale Chenevier
Veröffentlicht in: Chem Catalysis, Ausgabe 1/1, 2021, Seite(n) 88-105, ISSN 2667-1093
Herausgeber: Elsevier
DOI: 10.1016/j.checat.2021.01.001

Establishing reactivity descriptors for platinum group metal (PGM)-free Fe–N–C catalysts for PEM fuel cells

Autoren: Mathias Primbs, Yanyan Sun, Aaron Roy, Daniel Malko, Asad Mehmood, Moulay-Tahar Sougrati, Pierre-Yves Blanchard, Gaetano Granozzi, Tomasz Kosmala, Giorgia Daniel, Plamen Atanassov, Jonathan Sharman, Christian Durante, Anthony Kucernak, Deborah Jones, Frédéric Jaouen, Peter Strasser
Veröffentlicht in: Energy & Environmental Science, Ausgabe 13/8, 2020, Seite(n) 2480-2500, ISSN 1754-5692
Herausgeber: Royal Society of Chemistry
DOI: 10.1039/d0ee01013h

Upcycling of polyurethane into iron-nitrogen-carbon electrocatalysts active for oxygen reduction reaction

Autoren: Giorgia Daniel, Tomasz Kosmala, Maria Chiara Dalconi, Luca Nodari, Denis Badocco, Paolo Pastore, Alessandra Lorenzetti, Gaetano Granozzi, Christian Durante
Veröffentlicht in: Electrochimica Acta, Ausgabe 362, 2020, Seite(n) 137200, ISSN 0013-4686
Herausgeber: Pergamon Press Ltd.
DOI: 10.1016/j.electacta.2020.137200

A comparative perspective of electrochemical and photochemical approaches for catalytic H 2 O 2 production

Autoren: Yanyan Sun, Lei Han, Peter Strasser
Veröffentlicht in: Chemical Society Reviews, Ausgabe 49/18, 2020, Seite(n) 6605-6631, ISSN 0306-0012
Herausgeber: Royal Society of Chemistry
DOI: 10.1039/d0cs00458h

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