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Advancing CO2 Capture Materials by Atomic Scale Design: the Quest for Understanding

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Publications

CaO-Based CO 2 Sorbents with a Hierarchical Porous Structure Made via Microfluidic Droplet Templating

Author(s): Alexey Kurlov, Andac Armutlulu, Felix Donat, André R. Studart, Christoph R. Müller
Published in: Industrial & Engineering Chemistry Research, 59/15, 2020, Page(s) 7182-7188, ISSN 0888-5885
Publisher: American Chemical Society
DOI: 10.1021/acs.iecr.9b05996

Assessment of the Effect of Process Conditions and Material Characteristics of Alkali Metal Salt Promoted MgO-Based Sorbents on Their CO2 Capture Performance

Author(s): Jian Chen, Lunbo Duan, Felix Donat, Christoph R. Müller
Published in: ACS Sustainable Chemistry & Engineering, 9(19), 2021, Page(s) 6659-6672, ISSN 2168-0485
Publisher: American Chemical Society
DOI: 10.1021/acssuschemeng.1c00262

CO2 Capture at Medium to High Temperature Using Solid Oxide-Based Sorbents: Fundamental Aspects, Mechanistic Insights, and Recent Advances

Author(s): Matthew T. Dunstan, Felix Donat, Alexander H. Bork, Clare P. Grey, Christoph R. Müller
Published in: Chemical Reviews, 121(20), 2021, Page(s) 12681-12745, ISSN 0009-2665
Publisher: American Chemical Society
DOI: 10.1021/acs.chemrev.1c00100

Engineering the Cu/Mo2CTx (MXene) interface to drive CO2 hydrogenation to methanol

Author(s): Hui Zhou, Zixuan Chen, Anna Vidal López, Estefanía Díaz López, Erwin Lam, Athanasia Tsoukalou, Elena Willinger, Denis A. Kuznetsov, Deni Mance, Agnieszka Kierzkowska, Felix Donat, Paula M. Abdala, Aleix Comas-Vives, Christophe Copéret, Alexey Fedorov, Christoph R. Müller
Published in: Nature Catalysis, 4(10), 2021, Page(s) 860 - 871, ISSN 2520-1158
Publisher: Springer Nature
DOI: 10.1038/s41929-021-00684-0

Peering into buried interfaces with X-rays and electrons to unveil MgCO3 formation during CO2 capture in molten salt-promoted MgO

Author(s): Alexander H. Bork, Margarita Rekhtina, Elena Willinger, Pedro Castro-Fernández, Jakub Drnec, Paula M. Abdala, Christoph R. Müller
Published in: Proceedings of the National Academy of Sciences (PNAS), 118(26), 2021, Page(s) e2103971118, ISSN 0027-8424
Publisher: National Academy of Sciences
DOI: 10.1073/pnas.2103971118

Na 2 CO 3 -modified CaO-based CO 2 sorbents: the effects of structure and morphology on CO 2 uptake

Author(s): Alexey Kurlov, Agnieszka M. Kierzkowska, Thomas Huthwelker, Paula M. Abdala, Christoph R. Müller
Published in: Physical Chemistry Chemical Physics, 22/42, 2020, Page(s) 24697-24703, ISSN 1463-9076
Publisher: Royal Society of Chemistry
DOI: 10.1039/d0cp04410e

Structural insight into an atomic layer deposition (ALD) grown Al2O3 layer on Ni/SiO2: impact on catalytic activity and stability in dry reforming of methane

Author(s): Sung Min Kim, Andac Armutlulu, Wei-Chih Liao, Davood Hosseini, Dragos Stoian, Zixuan Chen, Paula M. Abdala, Christophe Copéret, Christoph Müller
Published in: Catalysis Science & Technology, 11, 2021, Page(s) 7563-7577, ISSN 2044-4753
Publisher: Royal Society of Chemistry
DOI: 10.1039/d1cy01149a

Mechanistic Understanding of CaO‐Based Sorbents for High‐Temperature CO 2 Capture: Advanced Characterization and Prospects

Author(s): Maximilian Krödel, Annelies Landuyt, Paula M. Abdala, Christoph R. Müller
Published in: ChemSusChem, 13(23), 2020, Page(s) 6259 - 6272, ISSN 1864-5631
Publisher: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/cssc.202002078

Surface Intermediates in In-Based ZrO2-Supported Catalysts for Hydrogenation of CO2 to Methanol

Author(s): Athanasia Tsoukalou; Nikolai S. Bushkov; Scott R. Docherty; Deni Mance; Alexander I. Serykh; Paula M. Abdala; Christophe Copéret; Alexey Fedorov; Christoph R. Müller
Published in: The Journal of Physical Chemistry C, 136(4), 2022, Page(s) 1793 - 1799, ISSN 1932-7447
Publisher: American Chemical Society
DOI: 10.1021/acs.jpcc.1c08814

Photo-Switchable Nanoripples in Ti3C2Tx MXene

Author(s): Mikhail Volkov, Elena Willinger, Denis A. Kuznetsov, Christoph R. Müller, Alexey Fedorov, Peter Baum
Published in: ACS Nano, 15(9), 2021, Page(s) 14071-14079, ISSN 1936-0851
Publisher: American Chemical Society
DOI: 10.1021/acsnano.1c03635

Atomic-Scale Structure and Its Impact on Chemical Properties of Aluminum Oxide Layers Prepared by Atomic Layer Deposition on Silica

Author(s): Monu Kaushik, César Leroy, Zixuan Chen, David Gajan, Elena Willinger, Christoph R. Müller, Franck Fayon, Dominique Massiot, Alexey Fedorov, Christophe Copéret, Anne Lesage, Pierre Florian
Published in: Chemistry of Materials, 33(9), 2021, Page(s) 3335-3348, ISSN 0897-4756
Publisher: American Chemical Society
DOI: 10.1021/acs.chemmater.1c00516

Bulk and surface transformations of Ga<sub>2</sub>O<sub>3</sub> nanoparticle catalysts for propane dehydrogenation induced by a H<sub>2</sub> treatment

Author(s): Pedro Castro-Fernández; Deni Mance; Chong Liu; Paula M. Abdala; Elena Willinger; Aurelio A. Rossinelli; Alexander I. Serykh; Evgeny A. Pidko; Christophe Copéret; Alexey Fedorov; Christoph R. Müller
Published in: Journal of Catalysis, 408, 2022, Page(s) 155-164, ISSN 0021-9517
Publisher: Academic Press
DOI: 10.1016/j.jcat.2022.02.025

Uncovering selective and active Ga surface sites in gallia–alumina mixed-oxide propane dehydrogenation catalysts by dynamic nuclear polarization surface enhanced NMR spectroscopy

Author(s): Pedro Castro-Fernández, Monu Kaushik, Zhuoran Wang, Deni Mance, Evgenia Kountoupi, Elena Willinger, Paula M. Abdala, Christophe Copéret, Anne Lesage, Alexey Fedorov, Christoph R. Müller
Published in: Chemical Science, 12(46), 2021, Page(s) 15273 - 15283, ISSN 2041-6520
Publisher: Royal Society of Chemistry
DOI: 10.1039/d1sc05381g

Effect of molten sodium nitrate on the decomposition pathways of hydrated magnesium hydroxycarbonate to magnesium oxide probed by in situ total scattering

Author(s): Margarita Rekhtina; Alessandro Dal Pozzo; Dragos Stoian; Andaç Armutlulu; Felix Donat; Maria Valeria Blanco; Zhu-Jun Wang; Marc Willinger; Alexey Fedorov; Paula M. Abdala; Christoph R. Müller
Published in: Nanoscale, 12(31), 2020, Page(s) 16462 - 16473, ISSN 2040-3364
Publisher: Royal Society of Chemistry
DOI: 10.1039/d0nr01760d

Hydrogen dissociation sites on indium-based ZrO2-supported catalysts for hydrogenation of CO2 to methanol

Author(s): Athanasia Tsoukalou, Alexander I. Serykh, Elena Willinger, Agnieszka Kierzkowska, Paula M. Abdala, Alexey Fedorov, Christoph R. Müller
Published in: Catalysis Today, 2021, ISSN 0920-5861
Publisher: Elsevier BV
DOI: 10.1016/j.cattod.2021.04.010