Advancing CO2 Capture Materials by Atomic Scale Design: the Quest for Understanding

Información del proyecto

AMADEUS

Identificador del acuerdo de subvención: 819573

DOI

10.3030/819573

Proyecto cerrado

Fecha de la firma de la CE 19 Diciembre 2018

Fecha de inicio 1 Junio 2019

Fecha de finalización 31 Mayo 2024

Financiado con arreglo a

• EXCELLENT SCIENCE - European Research Council (ERC)

Coste total

€ 1 994 900,00

Aportación de la UE

€ 1 994 900,00

Coordinado por

EIDGENOESSISCHE TECHNISCHE HOCHSCHULE ZUERICH
Switzerland

CORDIS proporciona enlaces a los documentos públicos y las publicaciones de los proyectos de los programas marco HORIZONTE.

Los enlaces a los documentos y las publicaciones de los proyectos del Séptimo Programa Marco, así como los enlaces a algunos tipos de resultados específicos, como conjuntos de datos y «software», se obtienen dinámicamente de OpenAIRE .

Publicaciones

Peer reviewed articles (31)

Model structures of molten salt-promoted MgO to probe the mechanism of MgCO3 formation during CO2 capture at a solid-liquid interface

Autores: Hansen Bork, Alexander; Ackerl, Norbert; Reuteler, Joakim; Jog, Sachin; Gut, David; Zboray, Robert; Müller, Christoph R.
Publicado en: Journal of Materials Chemistry A, 10 (32), Edición 1, 2022, Página(s) 16803-16812, ISSN 2050-7488
Editor: Royal Society of Chemistry
DOI: 10.1039/d2ta02897b

CaO-Based CO 2 Sorbents with a Hierarchical Porous Structure Made via Microfluidic Droplet Templating

Autores: Alexey Kurlov, Andac Armutlulu, Felix Donat, André R. Studart, Christoph R. Müller
Publicado en: Industrial & Engineering Chemistry Research, Edición 59/15, 2020, Página(s) 7182-7188, ISSN 0888-5885
Editor: American Chemical Society
DOI: 10.1021/acs.iecr.9b05996

Yolk-shell-type CaO-based sorbents for CO2 capture: assessing the role of nanostructuring for the stabilization of the cyclic CO2 uptake

Autores: Maximilian Krödel, Alexander Oing, Jan Negele, Annelies Landuyt, Agnieszka Kierzkowska, Alexander H. Bork, Felix Donat, Christoph R. Müller
Publicado en: Nanoscale, Edición 14 (45), 2022, Página(s) 16816 - 16828, ISSN 2040-3364
Editor: Royal Society of Chemistry
DOI: 10.1039/d2nr04492g

Assessment of the Effect of Process Conditions and Material Characteristics of Alkali Metal Salt Promoted MgO-Based Sorbents on Their CO2 Capture Performance

Autores: Jian Chen, Lunbo Duan, Felix Donat, Christoph R. Müller
Publicado en: ACS Sustainable Chemistry & Engineering, Edición 9(19), 2021, Página(s) 6659-6672, ISSN 2168-0485
Editor: American Chemical Society
DOI: 10.1021/acssuschemeng.1c00262

CO2 Capture at Medium to High Temperature Using Solid Oxide-Based Sorbents: Fundamental Aspects, Mechanistic Insights, and Recent Advances

Autores: Matthew T. Dunstan, Felix Donat, Alexander H. Bork, Clare P. Grey, Christoph R. Müller
Publicado en: Chemical Reviews, Edición 121(20), 2021, Página(s) 12681-12745, ISSN 0009-2665
Editor: American Chemical Society
DOI: 10.1021/acs.chemrev.1c00100

Engineering the Cu/Mo2CTx (MXene) interface to drive CO2 hydrogenation to methanol

Autores: Hui Zhou, Zixuan Chen, Anna Vidal López, Estefanía Díaz López, Erwin Lam, Athanasia Tsoukalou, Elena Willinger, Denis A. Kuznetsov, Deni Mance, Agnieszka Kierzkowska, Felix Donat, Paula M. Abdala, Aleix Comas-Vives, Christophe Copéret, Alexey Fedorov, Christoph R. Müller
Publicado en: Nature Catalysis, Edición 4(10), 2021, Página(s) 860 - 871, ISSN 2520-1158
Editor: Springer Nature
DOI: 10.1038/s41929-021-00684-0

Peering into buried interfaces with X-rays and electrons to unveil MgCO3 formation during CO2 capture in molten salt-promoted MgO

Autores: Alexander H. Bork, Margarita Rekhtina, Elena Willinger, Pedro Castro-Fernández, Jakub Drnec, Paula M. Abdala, Christoph R. Müller
Publicado en: Proceedings of the National Academy of Sciences (PNAS), Edición 118(26), 2021, Página(s) e2103971118, ISSN 0027-8424
Editor: National Academy of Sciences
DOI: 10.1073/pnas.2103971118

Na 2 CO 3 -modified CaO-based CO 2 sorbents: the effects of structure and morphology on CO 2 uptake

Autores: Alexey Kurlov, Agnieszka M. Kierzkowska, Thomas Huthwelker, Paula M. Abdala, Christoph R. Müller
Publicado en: Physical Chemistry Chemical Physics, Edición 22/42, 2020, Página(s) 24697-24703, ISSN 1463-9076
Editor: Royal Society of Chemistry
DOI: 10.1039/d0cp04410e

Chemical Looping Partial Oxidation of Methane: Reducing Carbon Deposition through Alloying

Autores: Felix Donat, Agnieszka Kierzkowska, and Christoph R. Müller
Publicado en: Energy & Fuels, Edición 36 (17), 2022, Página(s) 9780-9784, ISSN 0887-0624
Editor: American Chemical Society
DOI: 10.1021/acs.energyfuels.2c01345

Investigation of K2CO3-modified CaO sorbents for CO2 capture using in-situ X-ray diffraction

Autores: Yongqing Xu,Felix Donat,Cong Luo, Jian Chen, Agnieszka Kierzkowska, Muhammad Awais Naeem, Liqi Zhang, Christoph R. Müller
Publicado en: Chemical Engineering Journal, Edición 453, 2022, Página(s) 139913, ISSN 1385-8947
Editor: Elsevier BV
DOI: 10.1016/j.cej.2022.139913

Reversible transformation of sub-nanometer Ga-based clusters to isolated ^[4]Ga_(4Si) sites creates active centers for propane dehydrogenation

Autores: Zixuan Chen; Alexander I. Serykh; Agnieszka Kierzkowska; David Gajan; Scott R. Docherty; Alexander V. Yakimov; Paula M. Abdala; Christophe Copéret; Pierre Florian; Alexey Fedorov; Christoph R. Müller
Publicado en: Catalysis Science & Technology, 14 (2), Edición 3, 2024, Página(s) 379 - 390, ISSN 2044-4761
Editor: Royal Society of Chemistry
DOI: 10.1039/d3cy01446k

Structural insight into an atomic layer deposition (ALD) grown Al2O3 layer on Ni/SiO2: impact on catalytic activity and stability in dry reforming of methane

Autores: Sung Min Kim, Andac Armutlulu, Wei-Chih Liao, Davood Hosseini, Dragos Stoian, Zixuan Chen, Paula M. Abdala, Christophe Copéret, Christoph Müller
Publicado en: Catalysis Science & Technology, Edición 11, 2021, Página(s) 7563-7577, ISSN 2044-4753
Editor: Royal Society of Chemistry
DOI: 10.1039/d1cy01149a

Mechanistic Understanding of CaO‐Based Sorbents for High‐Temperature CO 2 Capture: Advanced Characterization and Prospects

Autores: Maximilian Krödel, Annelies Landuyt, Paula M. Abdala, Christoph R. Müller
Publicado en: ChemSusChem, Edición 13(23), 2020, Página(s) 6259 - 6272, ISSN 1864-5631
Editor: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/cssc.202002078

Nature of GaOx Shells Grown on Silica by Atomic Layer Deposition

Autores: Zixuan Chen, Nora K. Zimmerli, Muhammad Zubair, Alexander V. Yakimov, Snædís Björgvinsdóttir, Nicholas Alaniva, Elena Willinger, Alexander B. Barnes, Nicholas M. Bedford, Christophe Copéret, Pierre Florian, Paula M. Abdala, Alexey Fedorov, and Christoph R. Müller
Publicado en: Chemistry of Materials, Edición 35(18), 2023, Página(s) 7475 - 7490, ISSN 0897-4756
Editor: American Chemical Society
DOI: 10.1021/acs.chemmater.3c00923

Surface Intermediates in In-Based ZrO2-Supported Catalysts for Hydrogenation of CO2 to Methanol

Autores: Athanasia Tsoukalou; Nikolai S. Bushkov; Scott R. Docherty; Deni Mance; Alexander I. Serykh; Paula M. Abdala; Christophe Copéret; Alexey Fedorov; Christoph R. Müller
Publicado en: The Journal of Physical Chemistry C, Edición 136(4), 2022, Página(s) 1793 - 1799, ISSN 1932-7447
Editor: American Chemical Society
DOI: 10.1021/acs.jpcc.1c08814

Of Glasses and Crystals: Mitigating the Deactivation of CaO-Based CO2 Sorbents through Calcium Aluminosilicates

Autores: Maximilian Krödel, César Leroy, Sung Min Kim, Muhammad Awais Naeem, Agnieszka Kierzkowska, Yi-Hsuan Wu, Andac Armutlulu, Alexey Fedorov, Pierre Florian, and Christoph R. Müller
Publicado en: JACS Au, Edición 3 (11), 2023, Página(s) 3111–3126, ISSN 2691-3704
Editor: Amercian Chemical Society
DOI: 10.1021/jacsau.3c00475

Photo-Switchable Nanoripples in Ti3C2Tx MXene

Autores: Mikhail Volkov, Elena Willinger, Denis A. Kuznetsov, Christoph R. Müller, Alexey Fedorov, Peter Baum
Publicado en: ACS Nano, Edición 15(9), 2021, Página(s) 14071-14079, ISSN 1936-0851
Editor: American Chemical Society
DOI: 10.1021/acsnano.1c03635

Altering Oxygen Binding by Redox-Inactive Metal Substitution to Control Catalytic Activity: Oxygen Reduction on Manganese Oxide Nanoparticles as a Model System

Autores: Yi-Hsuan Wu, Harshit Mehta, Dr. Elena Willinger, Dr. Jodie A. Yuwono, Dr. Priyank V. Kumar, Dr. Paula M. Abdala, Dr. Anna Wach, Dr. Agnieszka Kierzkowska, Dr. Felix Donat, Dr. Denis A. Kuznetsov, Prof. Dr. Christoph R. Müller
Publicado en: Angewandte Chemie. International Edition, 62 (8), Edición 2, 2023, Página(s) e202217186, ISSN 1433-7851
Editor: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202217186

The structural evolution of Mo2C and Mo2C/SiO2 under dry reforming of methane conditions: morphology and support effects

Autores: Alexey Kurlov; Dragos Stoian; Ali Baghizadeh; Evgenia Kountoupi; Evgeniya B. Deeva; Marc Willinger; Paula M. Abdala; Alexey Fedorov; Christoph R. Müller
Publicado en: Catalysis Science & Technology, Edición 12 (18), 2022, Página(s) 5620 - 5628, ISSN 2044-4753
Editor: Royal Society of Chemistry
DOI: 10.1039/d2cy00729k

Atomic-scale changes of silica-supported catalysts with nanocrystalline or amorphous gallia phases: implications of hydrogen pretreatment on their selectivity for propane dehydrogenation

Autores: Pedro Castro-Fernández, Alexander I. Serykh, Alexander V. Yakimov, Igor P. Prosvirin, Andrey V. Bukhtiyarov, Paula M. Abdala, Christophe Copéret, Alexey Fedorov and Christoph R. Müller.
Publicado en: Catalysis Science & Technology, Edición 12 (12), 2022, Página(s) 3957 - 3968, ISSN 2044-4753
Editor: Royal Society of Chemistry
DOI: 10.1039/d2cy00074a

Prospects of MgO-based sorbents for CO2 capture applications at high temperatures

Autores: Felix Donat; Christoph Müller
Publicado en: Current Opinion in Green and Sustainable Chemistry, Edición 36, 2022, Página(s) 100645, ISSN 2452-2236
Editor: Elsevier
DOI: 10.1016/j.cogsc.2022.100645

Atomic-Scale Structure and Its Impact on Chemical Properties of Aluminum Oxide Layers Prepared by Atomic Layer Deposition on Silica

Autores: Monu Kaushik, César Leroy, Zixuan Chen, David Gajan, Elena Willinger, Christoph R. Müller, Franck Fayon, Dominique Massiot, Alexey Fedorov, Christophe Copéret, Anne Lesage, Pierre Florian
Publicado en: Chemistry of Materials, Edición 33(9), 2021, Página(s) 3335-3348, ISSN 0897-4756
Editor: American Chemical Society
DOI: 10.1021/acs.chemmater.1c00516

Deciphering the structural dynamics in molten salt–promoted MgO-based CO2 sorbents and their role in the CO2 uptake

Autores: Margarita Rekhtina, Maximilian Krödel, Yi-Hsuan Wu, Agnieszka Kierzkowska, Felix Donat, Paula M. Abdala, and Christoph R. Müller
Publicado en: Science Advances, 9 (26), Edición 14, 2023, Página(s) eadg5690, ISSN 1864-5631
Editor: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1126/sciadv.adg5690

Probing the Local Structure of Na in NaNO₃-Promoted, MgO-Based CO₂ Sorbents via X-ray Absorption Spectroscopy

Autores: Rekhtina, Margarita; Bugaev, Aram; Dunstan, Matthew T.; Dal Pozzo, Alessandro; Nadjafi, Manouchehr; Borca, Camelia; Huthwelker, Thomas; Abdala, Paula Macarena; Müller, Christoph R.
Publicado en: Chemistry of Materials, Edición 35 (23), 2023, Página(s) 10060-10069, ISSN 0897-4756
Editor: American Chemical Society
DOI: 10.3929/ethz-b-000645595

Uncovering selective and active Ga surface sites in gallia–alumina mixed-oxide propane dehydrogenation catalysts by dynamic nuclear polarization surface enhanced NMR spectroscopy

Autores: Pedro Castro-Fernández, Monu Kaushik, Zhuoran Wang, Deni Mance, Evgenia Kountoupi, Elena Willinger, Paula M. Abdala, Christophe Copéret, Anne Lesage, Alexey Fedorov, Christoph R. Müller
Publicado en: Chemical Science, Edición 12(46), 2021, Página(s) 15273 - 15283, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/d1sc05381g

Structure of Na Species in Promoted CaO-Based Sorbents and Their Effect on the Rate and Extent of the CO2 Uptake

Autores: Maximilian Krödel, Lorenz Abduly, Manouchehr Nadjafi, Agnieszka Kierzkowska, Alexander Yakimov, Alexander H. Bork, Felix Donat, Christophe Copéret, Paula M. Abdala, Christoph R. Müller
Publicado en: Advanced Functional Materials, 2023, Página(s) 2302916, ISSN 1616-301X
Editor: John Wiley & Sons Ltd.
DOI: 10.1002/adfm.202302916

Uncovering the CO2 Capture Mechanis of NaNO3-Promoted MgO by O-18 Isotope Labeling

Autores: Landuyt, Annelies; Kumar, Priyank V.; Yuwono, Jodie A.; Bork, Alexander H.; Donat, Felix; id_orcid0000-0002-3940-9183; Abdala, Paula M.; Müller, Christoph R.
Publicado en: JACS Au, 2 (12), Edición 1, 2022, Página(s) 2731-2741, ISSN 2691-3704
Editor: American Chemical Society
DOI: 10.1021/jacsau.2c00461

Structure and Role of a Ga-Promoter in Ni-Based Catalysts for the Selective Hydrogenation of CO2 to Methanol

Autores: Nora K. Zimmerli; Lukas Rochlitz; Stefano Checchia; Christoph R. Müller; Christophe Copéret; Paula M. Abdala
Publicado en: JACS Au, Vol 4, Iss 1, Pp 237-252 (2024), Edición 4, 2024, ISSN 2691-3704
Editor: American Chemical Society
DOI: 10.1021/jacsau.3c00677

Effect of molten sodium nitrate on the decomposition pathways of hydrated magnesium hydroxycarbonate to magnesium oxide probed by in situ total scattering

Autores: Margarita Rekhtina; Alessandro Dal Pozzo; Dragos Stoian; Andaç Armutlulu; Felix Donat; Maria Valeria Blanco; Zhu-Jun Wang; Marc Willinger; Alexey Fedorov; Paula M. Abdala; Christoph R. Müller
Publicado en: Nanoscale, Edición 12(31), 2020, Página(s) 16462 - 16473, ISSN 2040-3364
Editor: Royal Society of Chemistry
DOI: 10.1039/d0nr01760d

Hydrogen dissociation sites on indium-based ZrO2-supported catalysts for hydrogenation of CO2 to methanol

Autores: Athanasia Tsoukalou, Alexander I. Serykh, Elena Willinger, Agnieszka Kierzkowska, Paula M. Abdala, Alexey Fedorov, Christoph R. Müller
Publicado en: Catalysis Today, Edición vol 387, 2021, Página(s) 38-46, ISSN 0920-5861
Editor: Elsevier BV
DOI: 10.1016/j.cattod.2021.04.010

Bulk and surface transformations of Ga2O3 nanoparticle catalysts for propane dehydrogenation induced by a H2 treatment

Autores: Pedro Castro-Fernández, Deni Mance, Chong Liu, Paula Macarena Abdala, Elena Willinger, Aurelio A. Rossinelli, Alexander I. Serykh, Evgeny A. Pidko, Christophe Copéret, Alexey Fedorov, Christoph R. Müller
Publicado en: Journal of Catalysis, Edición 408, 2022, Página(s) 155-164, ISSN 0021-9517
Editor: Academic Press
DOI: 10.1016/j.jcat.2022.02.025