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Development of all thin-film PERovskite on CIS TANDem photovoltaics

Resultado final

25 % monolithic tandem module

Report on monolithic perovskite-on-CIS tandem mini-module demonstrator (10 cm2). End-of-project efficiency target is 25 %. Discussion of interlayer selection, concept development, and their upscaling.

30 % stacked tandem cell

Report on stacked perovskite-on-CIS tandem solar cell demonstrator (0.5 cm2 aperture area). End-of-project efficiency target is 30 %.

10 % small-area CIS cell under NIR

Report on smallarea CIS solar cell demonstrator 10 efficiency for NIRillumination 20 for 1sun illumination and its stability Efficiency target is 10 215 mAcm2 JSC 600 mV VOC and 78 FF under NIRillumination and 20 43 mAcm2 JSC 600 mV VOC and 78 FF under 1sun illumination Stability target is T80 performance under 1sun at 85 C load for 1000 h Report on approach to reduce root mean square roughness Rt 40 nm for the CIS cell stack

30 % monolithic tandem cell

Report on monolithically grown perovskite/CIS tandem solar cell demonstrator (aperture area = 0.5 cm2). End-of-project efficiency target is 30 %. Discussion of interlayer selection and concept development.

20 % semi-transparent perovskite cell

Report on the – solar cell, TCO’s and simulation – development of the 20 % semi-transparent perovskite solar cell demonstrator. End-of-project targets: efficiency above 20 %, 1200 mV VOC, and 90 % transparency (below band gap) at a band gap of 1.6-1.7 eV.

Model LCA and TEA for tandem

Report on the final model for LCA and TEA of the stacked and monolothic perovskite-on-CIS tandem technology, discussing the scientific, technological, environmental and economic potential of perovskite-on-CIS tandem technologies. Final statement regarding the reduced use of critical materials, e.g. Indium. Final statement regarding the emissions reductions.

8 % CIS cell on large-area under NIR

Report on CIS development for large-area: 10 cm × 10 cm demonstrator with 8 % (NIR) and 18 % (1-sun) mean efficiency, CIS cell stack on 20 cm × 20 cm sample (with bandgap of 1.0 eV), and CIS cell stack (with Rt < 40 nm) for monolithic tandem module development

25 % stacked tandem module

Report on stacked perovskiteonCIS tandem minimodule demonstrator Endofproject efficiency target is 25

Scientific workshop

Report on the 1st scientific workshop (incl. all relevant stakeholders) and co-creation session (with social groups of interest).

Special issue with workshop proceedings

Report on special issue journal as a followup of the scientific conference D72

White paper initiative

Report on white paper initiative very similar to the current CIGS white paper initiative see httpscigspvnetcigswhitepaperinitiative discussing the scientific technological environmental an economic potential of perovskiteonCIS tandem

Technological/Industrial workshop

Report on the 2nd technologicalindustrial workshop incl all relevant stakeholders and cocreation session with social groups of interest

Publicaciones

Compositional Investigation for Bandgap Engineering of Wide Bandgap Triple Cation Perovskite

Autores: Jacopo Sala, Maryamsadat Heydarian, Stijn Lammar, Yaser Abdulraheem, Tom Aernouts, Afshin Hadipour, and Jef Poortmans
Publicado en: ACS Appl. Energy Mater., 2021, ISSN 2574-0962
Editor: American Chemical Society
DOI: 10.1021/acsaem.1c00810

A study of quenching approaches to optimize ultrasonic spray coated perovskite layers scalable for PV

Autores: Joao Silvano, Jacopo Sala, Tamara Merckx, Yinghuan Kuang, Pieter Verding, Jan D'Haen, Tom Aernouts, Bart Vermang, and Wim Deferme
Publicado en: EPJ Photovoltaics, 2022, ISSN 2105-0716
Editor: EDP Sciences
DOI: 10.1051/epjpv/2022008

Near-Infrared-Transparent Perovskite Solar Cells and Perovskite-Based Tandem Photovoltaics

Autores: Radha K. Kothandaraman, Yan Jiang, Thomas Feurer, Ayodhya N. Tiwari, Fan Fu
Publicado en: Small Methods, 2020, ISSN 2366-9608
Editor: Wiley
DOI: 10.1002/smtd.202000395

Upscaling of perovskite solar modules: The synergy of fully evaporated layer fabrication and all-laser-scribed interconnections

Autores: David B. Ritzer, Tobias Abzieher, Agit Basibüyük, Thomas Feeney, Felix Laufer, Simon Ternes, Bryce S. Richards, Stefan Bergfeld, Ulrich W. Paetzold
Publicado en: Progress in Photovoltaics: Research and Applications, 2021, ISSN 1099-159X
Editor: Wiley
DOI: 10.1002/pip.3489

A review on barrier layers used in flexible stainless-steel based CIGS photovoltaic devices

Autores: Sarallah Hamtaei, Guy Brammertz, Jef Poortmans & Bart Vermang
Publicado en: npj Flexible Electronics, 2023, ISSN 2397-4621
Editor: Nature Publishing Group
DOI: 10.1038/s41528-023-00266-z

Silver‐Promoted High‐Performance (Ag,Cu)(In,Ga)Se 2 Thin‐Film Solar Cells Grown at Very Low Temperature

Autores: Shih-Chi Yang, Jordi Sastre, Maximilian Krause, Xiaoxiao Sun, Ramis Hertwig, Mario Ochoa, Ayodhya N. Tiwari, Romain Carron
Publicado en: Solar RRL, 2021, Página(s) 2100108, ISSN 2367-198X
Editor: Wiley
DOI: 10.1002/solr.202100108

Two birds with one stone: dual grain-boundary and interface passivation enables >22% efficient inverted methylammonium-free perovskite solar cells

Autores: Saba Gharibzadeh, Paul Fassl, Ihteaz M. Hossain, Pascal Rohrbeck, Markus Frericks, Moritz Schmidt, The Duong, Motiur Rahman Khan, Tobias Abzieher, Bahram Abdollahi Nejand, Fabian Schackmar, Osbel Almora, Thomas Feeney, Roja Singh, Dirk Fuchs, Uli Lemmer, Jan P. Hofmann, Stefan A. L. Weber, Ulrich W. Paetzold
Publicado en: Energy & Environmental Science, 2021, ISSN 1754-5692
Editor: Royal Society of Chemistry
DOI: 10.1039/d1ee01508g

Investigation and Mitigation of Sputter Damage on Co-Evaporated Cu(In,Ga)Se2 Absorbers for Photovoltaic Applications

Autores: Ramis Hertwig, Shiro Nishiwaki, Ayodhya N. Tiwari, Romain Carron
Publicado en: Solar RRL, 2022, ISSN 2367-198X
Editor: Wiley
DOI: 10.1002/solr.202200268

Laser Patterned Flexible 4T Perovskite-Cu(In,Ga)Se2 Tandem Mini-module with Over 18% Efficiency

Autores: Radha K. Kothandaraman, Huagui Lai, Abdessalem Aribia, Shiro Nishiwaki, Severin Siegrist, Maximilian Krause, Yannick Zwirner, Galo Torres Sevilla, Kerem Artuk, Christian M. Wolff, Romain Carron, Ayodhya N. Tiwari, Fan Fu
Publicado en: Solar RRL, 2022, ISSN 2367-198X
Editor: Wiley
DOI: 10.1002/solr.202200392

Translucent perovskite photovoltaics for building integration

Autores: D. B. Ritzer, B. Abdollahi Nejand, M. A. Ruiz-Preciado, S. Gharibzadeh, H. Hu, A. Diercks, T. Feeney, B. S. Richards, T. Abzieher, and U. W. Paetzold
Publicado en: Energy & Environmental Science, 2023, ISSN 1754-5706
Editor: Royal Society of Chemistry
DOI: 10.1039/d2ee04137e

Optical simulations and optimization of perovskite/CI(G)S tandem solar cells using the transfer matrix method

Autores: Aleksandra Bojar, Daniel Micha, Maxime Giteau, Marco A Ruiz-Preciado, Ulrich W Paetzold, Marcel Simor, Veronique S Gevaerts, Romain Carron, Karim Medjoubi, Stéphane Collin, Negar Naghavi, Jean-François Guillemoles, and Philip Schulz
Publicado en: JPhys Energy, 2023, ISSN 2515-7655
Editor: IOP Science
DOI: 10.1088/2515-7655/accf34

Toward the Design of High-Efficiency Perovskite Solar Cells

Autores: Philip Schulz and Jiong Lu
Publicado en: ACS Energy Lett., 2022, ISSN 2380-8195
Editor: American Chemical Society
DOI: 10.1021/acsenergylett.2c01434

Investigating the experimental space for two-step Cu(In,Ga)(S,Se)2 absorber layer fabrication: A design of experiment approach

Autores: Hamtaei, S., Brammertz, G., Kohl, T., Buldu, D.G., Birant, G., de Wild, J., Meuris, M., Poortmans, J., and Vermang, B.
Publicado en: Thin Solid Films, 2021, ISSN 1879-2731
Editor: Elsevier
DOI: 10.1016/j.tsf.2021.138958

The Role of SnF2 Additive on Interface Formation in All Lead-Free FASnI3 Perovskite Solar Cells

Autores: Zillner, Julia; Boyen, Hans-Gerd; Schulz, Philip; Hanisch, Jonas; Gauquelin, Nicolas; Verbeeck, Johan; Küffner, Johannes; Desta, Derese; Eisele Lisa; Ahlswede, Erik; Powalla, Michael
Publicado en: Advanced Functional Materials, 2022, ISSN 1616-3028
Editor: Wiley
DOI: 10.1002/adfm.202109649

Critical Role of Perovskite Film Stoichiometry in Determining Solar Cell Operational Stability: a Study on the Effects of Volatile A-Cation Additives

Autores: Wenya Song, Xin Zhang, Stijn Lammar, Weiming Qiu, Yinghuan Kuang, Bart Ruttens, Jan D'Haen, Inge Vaesen, Thierry Conard, Yaser Abdulraheem, Tom Aernouts, Yiqiang Zhan, and Jef Poortmans
Publicado en: ACS Appl. Mater. Interfaces, 2022, ISSN 1944-8244
Editor: American Chemical Society
DOI: 10.1021/acsami.2c05241

Towards market commercialization: Lifecycle economic and environmental evaluation of scalable perovskite solar cells

Autores: Alessandro Martulli; Neethi Rajagopalan; Fabrizio Gota; Toby Meyer; Ulrich Wilhelm Paetzold; Steven Claes; Alberto Salone; Jordy Verboven; Robert Malina; Bart Vermang; Sebastien Lizin
Publicado en: Progress in Photovoltaics: Research and Applications, 2022, ISSN 1099-159X
Editor: Wiley
DOI: 10.1002/pip.3623

Nanoparticle Wetting Agent for Gas Stream-Assisted Blade-Coated Inverted Perovskite Solar Cells and Modules

Autores: Johannes Küffner, Tina Wahl, Moritz Schultes, Jonas Hanisch, Julia Zillner, Erik Ahlswede, Michael Powalla
Publicado en: ACS Applied Materials & Interfaces, Edición 12/47, 2020, Página(s) 52678-52690, ISSN 1944-8244
Editor: American Chemical Society
DOI: 10.1021/acsami.0c15428

Triple-cation perovskite solar cells fabricated by a hybrid PVD/blade coating process using green solvents

Autores: Severin Siegrist, Shih-Chi Yang, Evgeniia Gilshtein, Xiaoxiao Sun, Ayodhya N. Tiwari, and Fan Fu
Publicado en: Journal of Materials Chemistry A, 2021, ISSN 2050-7496
Editor: Royal Society of Chemistry
DOI: 10.1039/d1ta07579a

Monolithic Two-Terminal Perovskite/CIS Tandem Solar Cells with Efficiency Approaching 25%

Autores: Marco A. Ruiz-Preciado, Fabrizio Gota, Paul Fassl, Ihteaz M. Hossain, Roja Singh, Felix Laufer, Fabian Schackmar, Thomas Feeney, Ahmed Farag, Isabel Allegro, Hang Hu, Saba Gharibzadeh, Bahram Abdollahi Nejand, Veronique S. Gevaerts, Marcel Simor, Pieter J. Bolt, and Ulrich W. Paetzold
Publicado en: ACS Energy Lett., 2022, ISSN 2380-8195
Editor: American Chemical Society
DOI: 10.1021/acsenergylett.2c00707

From Groundwork to Efficient Solar Cells: On the Importance of the Substrate Material in Co-Evaporated Perovskite Solar Cells

Autores: Tobias Abzieher, Thomas Feeney, Fabian Schackmar, Yidenekachew J. Donie, Ihteaz M. Hossain, Jonas A. Schwenzer, Tim Hellmann, Thomas Mayer, Michael Powalla, Ulrich W. Paetzold
Publicado en: Advanced Functional Materials, 2021, ISSN 1616-3028
Editor: Wiley
DOI: 10.1002/adfm.202104482

Silver-Alloyed Low-Bandgap CuInSe2 Solar Cells for Tandem Applications

Autores: Maximilian Krause, Shih-Chi Yang, Simon Moser, Shiro Nishiwaki, Ayodhya N. Tiwari, Romain Carron
Publicado en: Solar RRL, 2023, ISSN 2367-198X
Editor: Wiley
DOI: 10.1002/solr.202201122

Understanding Coating Thickness and Uniformity of Blade-Coated SnO2 Electron Transport Layer for Scalable Perovskite Solar Cells

Autores: Severin Siegrist, Pranjal Nandi, Radha K. Kothandaraman, Aribia Abdessalem, Ayodhya N. Tiwari, Fan Fu
Publicado en: Solar RRL, 2023, ISSN 2367-198X
Editor: Wiley
DOI: 10.1002/solr.202300273

Efficiency boost of bifacial Cu(In,Ga)Se2 thin-film solar cells for flexible and tandem applications with silver-assisted low-temperature process

Autores: Shih-Chi Yang, Tzu-Ying Lin, Mario Ochoa, Huagui Lai, Radha Kothandaraman, Fan Fu, Ayodhya N. Tiwari & Romain Carron
Publicado en: Nature Energy, 2023, ISSN 2058-7546
Editor: Nature Publishing Group
DOI: 10.1038/s41560-022-01157-9

An Integrated Bulk and Surface Modification Strategy for Gas-Quenched Inverted Perovskite Solar Cells with Efficiencies Exceeding 22%

Autores: Xin Zhang, Weiming Qiu, Wenya Song, Zafer Hawash, Yaxin Wang, Bapi Pradhan, Yiyue Zhang, Denys Naumenko, Heinz Amenitsch, Ellen Moons, Tamara Merckx, Aranzazu Aguirre, Yaser Abdulraheem, Tom Aernouts, Yiqiang Zhan, Yinghuan Kuang, Johan Hofkens, Jef Poortmans
Publicado en: Solar RRL, 2021, ISSN 2367-198X
Editor: Wiley
DOI: 10.1002/solr.202200053

Revealing the perovskite formation kinetics during chemical vapour deposition

Autores: Thierry Moser, Kerem Artuk, Yan Jiang, Thomas Feurer, Evgeniia Gilshtein, Ayodhya N. Tiwari, Fan Fu
Publicado en: Journal of Materials Chemistry A, Edición 8/42, 2020, Página(s) 21973-21982, ISSN 2050-7488
Editor: Royal Society of Chemistry
DOI: 10.1039/d0ta04501b

EYcalc - Energy yield calculator for multi-junction solar modules with realistic irradiance data and textured interfaces

Autores: Schmager, Raphael; Paetzold, Ulrich W.; Langenhorst, Malte; Gota, Fabrizio; Lehr, Jonathan
Publicado en: Zenodo, 2021
Editor: CERN
DOI: 10.5281/zenodo.4696257

Derechos de propiedad intelectual

Forming of perovskite-based optoelectronic devices

Número de solicitud/publicación: IPR 4199126
Fecha: 2023-06-21
Solicitante(s): INTERUNIVERSITAIR MICRO-ELECTRONICA CENTRUM

Forming of perovskite-based optoelectronic devices

Número de solicitud/publicación: IPR 4199126
Fecha: 2023-06-21
Solicitante(s): UNIVERSITEIT HASSELT

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