Sodium-Ion and sodium Metal BAtteries for efficient and sustainable next-generation energy storage

Livrables

Module testing results
Dissemination plan

A report describing the plan for dissemination and communication actions

A Report regarding standards and regulations for stationary sodium ion based batteries will be delivered

Baseline cell, electrochemical and physical characterisation

In order to accurately record the technical advances it is first necessary to baseline what is currently achievable This will be done at pouch cell level using materials available within the consortium

Development of novel all-solid-state cell

Combining all learning to date within the WP will allow for trialling of a novel all solid state cell.

Stationary Energy Storage - Use Cases and Requirements

This deliverable will include a key requirements for stationary energy storage and b use case profiles to assess the batteries on use case specific KPIs

Develop a safe storage, transport and opening protocol for the solid-state batteries at end of life

A process will be evaluated for disassembly of the solid state batteries and the opening of these cells. A report will be written detailing the protocols.

Operational in-situ NMR and SPM /first tests demonstration

A report describing briefly the main steps of setting up the NMRSMP equipment inclusing the results of the first measurements

Dissemination tools (website, flyer, project templates)

A report describing the status of the website flyer and project templates

Quantification of Na+ transfer at electrode/electrolyte interfaces

A report including the diffusion coefficients of sodium in the electrode electrolyte and well as the charge transfer resistances across the electrodeelectrolyte interface

Report on the interpretation of the atomic scale/mesoscopic data

Report on the interpretation of the atomic scale data. Atomistic models of individual battery components (Prussian white cathode, polymer electrolyte, porous SiOC/SiC/hard carbon anodes) and of relevant interfaces are developed and verified against NMR and XPS data.

Publications

SiCO Ceramics as Storage Materials for Alkali Metals/Ions: Insights on Structure Moieties from Solid-State NMR and DFT Calculations

Auteurs: Edina Šić, Jochen Rohrer, Emmanuel III Ricohermoso, Karsten Albe, Emmanuel Ionescu, Ralf Riedel, Hergen Breitzke, Torsten Gutmann, Gerd Buntkowsky
Publié dans: ChemSusChem, Numéro 24 issues per year, 2023, ISSN 1864-5631
Éditeur: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/cssc.202202241

On the reversible sodium plating/stripping reaction in a hierarchical silicon carbonitride ceramic: feasibility study

Auteurs: Marco Melzi d'Eril, Magdalena Joanna Graczyk-Zajac, Ralf Riedel
Publié dans: Batteries & Supercaps, Numéro 12 issues per year, 2023, ISSN 2022-0049
Éditeur: Wiley-VCH
DOI: 10.1002/batt.202200491

Mechanism of gelation in high nickel content cathode slurries for sodium-ion batteries

Auteurs: Samuel Roberts, Lin Chen, Brij Kishore, Claire E.J. Dancer, Mark J.H. Simmons, Emma Kendrick
Publié dans: Journal of Colloid and Interface Science, Numéro 627, 2023, Page(s) 427-437, ISSN 0021-9797
Éditeur: Academic Press
DOI: 10.1016/j.jcis.2022.07.033

Optimization of Sodium Bis(oxalato)borate (NaBOB) in Triethyl Phosphate (TEP) by Electrolyte Additives

Auteurs: Jonas Welch, Ronnie Mogensen, Wessel van Ekeren, Henrik Eriksson, Andrew J. Naylor, Reza Younesi
Publié dans: Journal of The Electrochemical Society, Numéro 169, 2022, Page(s) 120523, ISSN 0013-4651
Éditeur: Electrochemical Society, Inc.
DOI: 10.1149/1945-7111/acaa5e

On the compatibility of high mass loading bismuth anodes for full-cell sodium-ion batteries

Auteurs: Lars Olow Simon Colbin, Tochukwu E. Nwafornso, Yunjie Li, Reza Younesi
Publié dans: Dalton Transactions, Numéro 51, 2024, Page(s) 16852-16860, ISSN 1477-9226
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d2dt02686d

A compatibility study of protective coatings for temperature sensor integration into sodium-ion battery cells

Auteurs: Timothy A Vincent, Faduma M Maddar, Sheng Chao, Erdogan Guk, Jonathan E H Sansom, Begum Gulsoy, Mark Copley, Ivana Hasa, James Marco
Publié dans: Journal of Physics: Energy, Numéro 6, 2024, Page(s) 025002, ISSN 2515-7655
Éditeur: IOP Publishing Ltd
DOI: 10.1088/2515-7655/ad1e38

Tin-functionalized silicon oxycarbide as a stable, high-capacity anode material for Na-ion batteries

Auteurs: Alexander Kempf; Samira Kiefer; Magdalena Graczyk-Zajac; Emanuel Ionescu; Ralf Riedel
Publié dans: Open Ceramics, Numéro 6, 2023, Page(s) Vol. 15 p. 100388, ISSN 2666-5395
Éditeur: Elsevier
DOI: 10.1016/j.oceram.2023.100388

Revisiting Amides as Cosolvents for Flame Resistant Sodium Bis(oxalato)borate in Triethyl Phosphate Electrolyte

Auteurs: Charles Aram Hall, Lars O. Simon Colbin, Alexander Buckel, Reza Younesi
Publié dans: Batteries & Supercaps, Numéro 7, 2024, ISSN 2566-6223
Éditeur: Wiley-VCH GmbH
DOI: 10.1002/batt.202300338

Fluorine‐Free Electrolytes for Lithium and Sodium Batteries

Auteurs: Hernández, Guiomar; Morgensen, Ronnie; Younesi, Reza; Mindemark, Jonas
Publié dans: Batteries & Supercaps, Numéro 12, 2022, Page(s) Vol. 5, e202100373, ISSN 2566-6223
Éditeur: WIley-VCH
DOI: 10.1002/batt.202100373

Structure–property relations of silicon oxycarbides studied using a machine learning interatomic potential

Auteurs: Niklas Leimeroth, Jochen Rohrer, Karsten Albe
Publié dans: Journal of the American Ceramic Society, Numéro 107, 2024, Page(s) 6896-6910, ISSN 0002-7820
Éditeur: American Ceramic Society
DOI: 10.1111/jace.19932

SiCN Ceramics as Electrode Materials for Sodium/Sodium Ion Cells – Insights from 23Na In-Situ Solid-State NMR

Auteurs: Edina Šić, Marco Melzi d'Eril, Konstantin Schutjajew, Magdalena J. Graczyk-Zajac, Hergen Breitzke, Ralf Riedel, Martin Oschatz, Torsten Gutmann, Gerd Buntkowsky
Publié dans: Batteries & Supercaps, Numéro 12 issues per year, 2022, ISSN 2566-6223
Éditeur: Wiley
DOI: 10.1002/batt.202200066

Elucidating Gas Evolution of Prussian White Cathodes for Sodium‐ion Battery Application: The Effect of Electrolyte and Moisture

Auteurs: Sören L. Dreyer, Faduma M. Maddar, Aleksandr Kondrakov, Jürgen Janek, Ivana Hasa, Torsten Brezesinski
Publié dans: Batteries & Supercaps, Numéro 7, 2024, ISSN 2566-6223
Éditeur: Wiley-VCH GmbH
DOI: 10.1002/batt.202300595

Effect of ultra-fast pyrolysis on polymer-derived SiOC aerogels and their application as anodes for Na-ion batteries

Auteurs: Marco Melzi d’Eril, Andrea Zambotti, Magdalena Graczyk-Zajac, Emanuel Ionescu, Gian Domenico Sorarù, Ralf Riedel
Publié dans: Open Ceramics, Numéro 4 issues per year, 2023, ISSN 2666-5395
Éditeur: Elsevier
DOI: 10.1016/j.oceram.2023.100354

Improved Lifetime of Na-Ion Batteries With a Water-Scavenging Electrolyte Additive

Auteurs: Lin Chen, Brij Kishore, Tengfei Song, Marc Walker, Claire Dancer, Emma Kendrick
Publié dans: Frontiers in Energy Research, Numéro 10, 2022, ISSN 2296-598X
Éditeur: Frontiers in Energy research
DOI: 10.3389/fenrg.2022.925430

Anodic dissolution of aluminum in non-aqueous electrolyte solutions for sodium-ion batteries

Auteurs: Lars Olow Simon Colbin; Charles Aram Hall; Ahmed S. Etman; Alexander Buckel; Leif Nyholm; Reza Younesi
Publié dans: Energy Advances, Numéro 12, volume 3, 2024, Page(s) 143-148, ISSN 2753-1457
Éditeur: RSC
DOI: 10.1039/d3ya00233k

Sodium 4-styrenesulfonyl(trifluoromethanesulfonyl)imide-based Single-Ion Conducting Polymer Electrolyte Incorporating Molecular Transporters for Solid-State Sodium Batteries. (2024), accepted

Auteurs: Wunder, C., Lai, T.-L., Šić, E., Gutmann, T., de Vito, E., Buntkowsky, G., Zarrabeitia, M., Passerini, S.
Publié dans: J. Mater. Chem. A, 2024, Page(s) Manuscript ID: TA-ART-04-2024-002329.R1, ISSN 2050-7496
Éditeur: RSC
DOI: 10.1039/d4ta02329c

Electrochemical Sodium Storage in Hard Carbon Powder Electrodes Implemented in an Improved Cell Assembly: Insights from In-Situ and Ex-Situ Solid-State NMR

Auteurs: Edina Šić, Dr. Konstantin Schutjajew, Ulrich Haagen, Dr. Hergen Breitzke, Prof. Martin Oschatz, Prof. Gerd Buntkowsky, Prof. Torsten Gutmann
Publié dans: ChemSusChem, 2024, Page(s) e202301300, ISSN 1864-5631
Éditeur: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/cssc.202301300

Si-based polymer-derived ceramics for energy conversion and storage

Auteurs: Qingbo Wen, Fangmu Qu, Zhaoju Yu, Magdalena Graczyk-Zajac, Xiang Xiong, Ralf Riedel
Publié dans: Journal of Advanced Ceramics, Numéro 4-12 issues per year, 2022, ISSN 2226-4108
Éditeur: Springer Link
DOI: 10.1007/s40145-021-0562-2

Understanding dehydration of Prussian white: from material to aqueous processed composite electrodes for sodium-ion battery application

Auteurs: F. M. Maddar, D. Walker, T. W. Chamberlain, J. Compton, A. S. Menon, M. Copley, I. Hasa
Publié dans: Journal of Materials Chemistry A, Numéro 11, 2024, Page(s) 15778-15791, ISSN 2050-7488
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d3ta02570e

Enabling Aqueous Processing of Prussian White Cathodes for Sodium Ion Cells By Understanding the Effect of Structural Water

Auteurs: Faduma Maddar, Ashok Menon, Katerina Gonos, Jacob Compton, Daniel Atkinson, Louis F.J. Piper, Mark Copley, Ivana Hasa
Publié dans: ECS Meeting Abstracts, Volume MA2022-02, A04: Next Generation Batteries, Numéro 2022 Meet. Abstr. MA2022-02 500, 2022
Éditeur: 2022 ECS - The Electrochemical Society
DOI: 10.1149/ma2022-024500mtgabs

Improvement of the performance of Silicon-graphite anodes in Li-ion batteries by application of self-healing binder

Auteurs: Alper Güneren, Zoltan Lenčéš, Ahmed Nada
Publié dans: Proceedings of the Processing and properties of advanced ceramics and glasses, Numéro 1 per year, 2022, ISBN 978-80-973578-1-8
Éditeur: Slovak Silicate Scientific-Technological Society

Battery Cell Temperature Sensing Towards Smart Sodium-Ion Cells for Energy Storage Applications

Auteurs: Timothy A. Vincent, Ivana Hasa, Begum Gulsoy, Jonathan E.H. Sansom, James Marco
Publié dans: 2022 IEEE 16th International Conference on Compatibility, Power Electronics, and Power Engineering (CPE-POWERENG), Numéro 1 per conference, 2022, ISBN 9781665496780
Éditeur: IEEE
DOI: 10.1109/cpe-powereng54966.2022.9880876

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