Electrochemical Bond Functionalization

Publicaciones

Electrochemical Cross-Electrophile-Coupling for Transition-Metal-Free Allylic Carboxylation with Ambient CO2

Autores: Rong Zhao; Zhipeng Lin; Isaac Maksso; Julia Struwe; Lutz Ackermann
Publicado en: ChemElectroChem, 2022, ISSN 2196-0216
Editor: Wiley-VCH
DOI: 10.1002/celc.202200989

Distal Ruthenaelectro‐Catalyzed meta ‐C−H Bromination with Aqueous HBr

Autores: Yulei Wang; Hendrik Simon; Xinran Chen; Zhipeng Lin; Shan Chen; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 1, 2022, ISSN 1521-3757
Editor: Wiley-VCH
DOI: 10.1002/anie.202201595

Ruthenaelectro-catalyzed C–H acyloxylation for late-stage tyrosine and oligopeptide diversification

Autores: Xiaoyan Hou; Nikolaos Kaplaneris; Binbin Yuan; Johanna Frey; Tsuyoshi Ohyama; Antonis M. Messinis; Lutz Ackermann
Publicado en: Chem Sci, Edición 2, 2022, ISSN 2041-6539
Editor: Royal Society of Chemistry
DOI: 10.1039/d1sc07267f

Cobalt-catalyzed radical-mediated carbon–carbon scission via a radical-type migratory insertion

Autores: Jian-Biao Liu; Xiao-Jun Liu; Joao C. A Oiveira; De-Zhan Chen; Lutz Ackermann
Publicado en: Chem Sci, 2023, ISSN 2041-6539
Editor: Royal Society of Chemistry
DOI: 10.1039/d2sc05200h

Enantioselective electrochemical cobalt-catalyzed aryl C–H activation reactions

Autores: Tristan von Münchow; Suman Dana; Yang Xu; Binbin Yuan; Lutz Ackermann
Publicado en: Science, 2023, ISSN 1095-9203
Editor: AAAS
DOI: 10.1126/science.adg2866

Chemo- and Site-Selective Electro-Oxidative Alkane Fluorination by C(sp3)−H Cleavage

Autores: Maximilian Stangier, Alexej Scheremetjew, and Lutz Ackermann
Publicado en: Chemistry - A European Journal, 2022, ISSN 1521-3765
Editor: Wiley-VCH
DOI: 10.1002/chem.202201654

Room temperature photo-promoted iron-catalysed arene C–H alkenylation without Grignard reagents

Autores: Antonis M. Messinis; Tristan von Münchow; Max Surke; Lutz Ackermann
Publicado en: Nature Catalysis, Edición 17, 2024, ISSN 2520-1158
Editor: Springer Nature
DOI: 10.1038/s41929-023-01105-0

Chemodivergent manganese-catalyzed C–H activation: modular synthesis of fluorogenic probes

Autores: Nikolaos Kaplaneris, Jongwoo Son, Lorena Mendive-Tapia, Adelina Kopp, Nicole D. Barth, Isaac Maksso, Marc Vendrell, Lutz Ackermann
Publicado en: Nature communications, 2021, ISSN 2041-1723
Editor: Nature Publishing Group
DOI: 10.1038/s41467-021-23462-9

Synthesis of C ‐Oligosaccharides through Versatile C(sp 3 )−H Glycosylation of Glycosides

Autores: Jun Wu; Adelina Kopp; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 14, 2022, ISSN 1521-3773
Editor: Wiley-VCH
DOI: 10.1002/anie.202114993

Polymer up-cycling by mangana-electrocatalytic C(sp3)–H azidation without directing groups

Autores: Isaac Maksso; Ramesh C. Samanta; Yifei Zhan; Kai Zhang; Svenja Warratz; Lutz Ackermann
Publicado en: Chemical Science, Edición 5, 2023, ISSN 1742-2183
Editor: RSC
DOI: 10.1039/d3sc02549g

Reusable Manganese Catalyst for Site-Selective Pyridine C−H Arylations and Alkylations

Autores: Isaac Choi, Zhigao Shen, Dr. Emanuel Ronge, Dr. Volker Karius, Prof. Dr. Christian Jooss, Prof. Dr. Lutz Ackermann
Publicado en: Chemistry a European Journal, 2021, ISSN 1521-3765
Editor: Wiley-VCH
DOI: 10.1002/chem.202101894

Recent advances in organic electrochemical functionalizations for specialty chemicals

Autores: Li, Yanjun; Dana, Suman; Ackermann, Lutz
Publicado en: Current Opinion in Electrochemistry, Edición 2, 2023, ISSN 2451-9111
Editor: Elsevier
DOI: 10.1016/j.coelec.2023.101312

Photoelectrochemical Si–H and Ge–H activation by iron catalysis

Autores: Wen Wei; Simon L. Homölle; Tristan von Münchow; Yanjun Li; Isaac Maksso; Lutz Ackermann
Publicado en: Cell Reports Physical Science, Edición 6, 2023, ISSN 2666-3864
Editor: Cell Press
DOI: 10.1016/j.xcrp.2023.101550

Distale C−H‐Glykosylierung durch Ruthenium(II)‐Katalyse: Modularer Aufbau von meta ‐ C ‐Aryl‐Glykosiden

Autores: Jun Wu; Nikolaos Kaplaneris; Julia Pöhlmann; Takuya Michiyuki; Binbin Yuan; Lutz Ackermann
Publicado en: Angew. Chem., Edición 8, 2022, ISSN 0044-8249
Editor: Wiley-VCH
DOI: 10.1002/ange.202208620

Synthese von C ‐Oligosacchariden via vielseitiger C(sp 3 )‐H‐Glykosylierung von Glykosiden

Autores: Jun Wu; Adelina Kopp; Lutz Ackermann
Publicado en: Angew. Chem., Edición 6, 2022, ISSN 0044-8249
Editor: Wiley-VCH
DOI: 10.1002/ange.202114993

Cobaltaelectro-Catalyzed C–H Annulation with Allenes for Atropochiral and P-stereogenic Compounds: Late-stage Diversification and Continuous Flow Scale up

Autores: Ye Lin; Tristan von Münchow; Lutz Ackermann
Publicado en: ACS Catalysis, Edición 1, 2023, ISSN 2155-5435
Editor: American Chemical Society
DOI: 10.26434/chemrxiv-2023-7g4z2

Distale Ruthenaelektro‐katalysierte meta ‐C−H‐Bromierung mit wässriger HBr

Autores: Yulei Wang; Hendrik Simon; Xinran Chen; Zhipeng Lin; Shan Chen; Lutz Ackermann
Publicado en: Angew. Chem., Edición 2, 2022, ISSN 0044-8249
Editor: Wiley-VCH
DOI: 10.1002/ange.202201595

Ruthenium(II)/Imidazolidine Carboxylic Acid-Catalyzed C-H Alkylation for Central and Axial Double Enantio-Induction.

Autores: Yanjun Li; Yan‐Cheng Liou; João C. A. Oliveira; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 2, 2022, ISSN 1521-3757
Editor: Wiley-VCH
DOI: 10.1002/anie.202212595

Electrocatalyzed Direct Arene Alkenylations without Directing Groups: Selective Late-Stage Drug Diversification

Autores: Zhipeng Lin; Uttam Dhawa; Binbin Yuan; Yan-Cheng Liou; Magnus Johansson; Lutz Ackermann
Publicado en: Research Square, 2022, ISSN 2693-5015
Editor: Springer Nature
DOI: 10.21203/rs.3.rs-1607467/v1

Electrooxidative tricyclic 6–7–6 fused-system domino assembly to allocolchicines by a removable radical strategy

Autores: Yan Zhang; Chanchan Ma; Zhenzhi Cai; Julia Struwe; Shengjie Chen; Jinming Xu; Shiyin Li; Wangyu Zeng; Lutz Ackermann
Publicado en: Green Chemistry, Edición 5, 2022, ISSN 1463-9270
Editor: Royal Society of Chemistry
DOI: 10.1039/d2gc00684g

Remote C−H Glycosylation by Ruthenium(II) Catalysis: Modular Assembly of meta ‐ C ‐Aryl Glycosides

Autores: Jun Wu; Nikolaos Kaplaneris; Julia Pöhlmann; Takuya Michiyuki; Binbin Yuan; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 6, 2022, ISSN 1521-3757
Editor: Wiley-VCH
DOI: 10.1002/anie.202208620

A Strategy for Site- and Chemoselective C−H Alkenylation through Osmaelectrooxidative Catalysis

Autores: Isaac Choi, Antonis M. Messinis, Xiaoyan Hou, Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., 2021, ISSN 1521-3773
Editor: Wiley-VCH
DOI: 10.1002/anie.202110616

Ruthenium‐Catalyzed Remote Difunctionalization of Nonactivated Alkenes for Double meta‐C(sp2)−H/C‐6(sp3)−H Functionalization

Autores: Chen, Shan; Yuan, Binbin; Wang, Yulei; Ackermann, Lutz; Chen, Shan;; Yuan, Binbin;; Wang, Yulei;; Ackermann, Lutz;
Publicado en: Angewandte Chemie International Edition, Edición 4, 2023, ISSN 1521-3757
Editor: Wiley-VCH Verlag
DOI: 10.1002/anie.202301168

Electrochemical Cage Activation of Carboranes.

Autores: Long Yang; Zi‐Jing Zhang; Becky Bongsuiru Jei; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 2, 2022, ISSN 1521-3757
Editor: Wiley-VCH
DOI: 10.1002/anie.202200323

Electrooxidative Rearrangement for Remote Functionalizations of Unactivated Alkenes through Migration

Autores: Dingyi Wang; Binbin Yuan; Jiawei Xu; Lutz Ackermann
Publicado en: Chemistry A European Journal, 2023, ISSN 1521-3765
Editor: Wiley-VCH
DOI: 10.1002/chem.202300600

Elektrochemische Carborankäfig‐Aktivierung

Autores: Long Yang; Zi‐Jing Zhang; Becky Bongsuiru Jei; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 5, 2022, ISSN 1521-3773
Editor: Wiley-VCH
DOI: 10.1002/ange.202200323

Bifurcated Rhodaelectro-catalyzed C–H Activation for the Synthesis of Pyrroles and Lactones

Autores: Simon L. Homölle; Maximilian Stangier; Efraim Reyes; Lutz Ackermann
Publicado en: Precision Chemistry, Vol 1, Iss 6, Pp 382-387 (2023), Edición 2, 2023, ISSN 2771-9316
Editor: ACS
DOI: 10.1021/prechem.3c00061

Electrooxidative palladium- and enantioselective rhodium-catalyzed [3 + 2] spiroannulations.

Autores: Wen Wei; Alexej Scheremetjew; Lutz Ackermann
Publicado en: Chem Sci, Edición 1, 2022, ISSN 2041-6539
Editor: Royal Society of Chemistry
DOI: 10.1039/d1sc07124f

Earth-abundant 3d transition metals on the rise in catalysis

Autores: Nikolaos Kaplaneris; Lutz Ackermann
Publicado en: Beilstein J. Org. Chem., 2022, ISSN 1860-5397
Editor: Beilstein-Institut
DOI: 10.3762/bjoc.18.8

Chelation-Assisted Iron-Catalyzed C–H Activations: Scope and Mechanism

Autores: Jiayu Mo; Antonis M. Messinis; Jinlian Li; Svenja Warratz; Lutz Ackermann
Publicado en: Accounts of Chemical Reseaarch, Edición 14, 2024, ISSN 1520-4898
Editor: ACS Publications
DOI: 10.1021/acs.accounts.3c00294

Bridging Chemical Knowledge and Machine Learning for Performance Prediction of Organic Synthesis

Autores: Shuo-Qing Zhang; Li-Cheng Xu; Shu-Wen Li; João C. A. Oliveira; Xin Li; Lutz Ackermann; Xin Hong
Publicado en: Chemistry A European Journal, 2022, ISSN 1521-3765
Editor: Wiley-VCH
DOI: 10.1002/chem.202202834

Electrochemical Late-Stage Functionalization

Autores: Yulei Wang; Suman Dana; Hao Long; Yang Xu; Yanjun Li; Nikolaos Kaplaneris; Lutz Ackermann
Publicado en: Chemical Reviews, Edición 4, 2023, ISSN 1520-6890
Editor: ACS
DOI: 10.1021/acs.chemrev.3c00158

Cyclometallated Iron(II) Alkoxides in Iron-Catalyzed C–H Activations by Weak O-Carbonyl Chelation

Autores: Antonis M. Messinis, João C. A. Oliveira, A. Claudia Stückl, and Lutz Ackermann
Publicado en: ACS Catalysis, 2022, ISSN 2155-5435
Editor: American Chemical Society
DOI: 10.1021/acscatal.2c00772

Rhodaelectro‐Catalyzed peri ‐Selective Direct Alkenylations with Weak O ‐Coordination Enabled by the Hydrogen Evolution Reaction (HER)

Autores: Bartłomiej Sadowski; Binbin Yuan; Zhipeng Lin; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 5, 2022, ISSN 1521-3773
Editor: Wiley-VCH
DOI: 10.1002/anie.202117188

When machine learning meets molecular synthesis

Autores: João C.A. Oliveira; Johanna Frey; Shuo-Qing Zhang; Li-Cheng Xu; Xin Li; Shu-Wen Li; Xin Hong; Lutz Ackermann
Publicado en: Trends in Chemistry, 2022, ISSN 2589-5974
Editor: Elsevier
DOI: 10.1016/j.trechm.2022.07.005

The crucial role of silver(<scp>i</scp>)-salts as additives in C–H activation reactions: overall analysis of their versatility and applicability

Autores: Renato L. de Carvalho; Emilay B. T. Diogo; Simon L. Homölle; Suman Dana; Eufrânio N. da Silva Júnior; Lutz Ackermann
Publicado en: Chemical Society Reviews, Edición 4, 2023, ISSN 1460-4744
Editor: RSC
DOI: 10.1039/d3cs00328k

Electrochemical Sulphenylation/Cyclization of Quinones: A Rapid, Green, and Efficient Access to Cytotoxic Compounds

Autores: Emilay B. T. Diogo; Fábio G. Delolo; Gabriela A. P. Graça; Esther R. S. Paz; Ícaro A. O. Bozzi; Renata Diniz; Juliano P. Passos; Tulio Matencio; Liane K. Soares; Diego Alves; Pedro M. S. Costa; Claudia Pessoa; Cynthia L. M. Pereira; Lutz Ackermann; Eufrânio N. da Silva Júnior
Publicado en: European Journal of Chemistry, Edición 3, 2023, ISSN 1099-0690
Editor: Wiley
DOI: 10.1002/ejoc.202300506

Domino meta-C−H Ethyl Glycosylation by Ruthenium(II/III) Catalysis: Modular Assembly of meta-C-Alkyl Glycosides

Autores: Jun Wu; Wen Wei; Julia Pöhlmann; Rajeshwaran Purushothaman; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., 2023, ISSN 1521-3773
Editor: Wiley-VCH
DOI: 10.1002/anie.202219319

Palladium-Catalyzed Electrooxidative Double C–H Arylation

Autores: Zhipeng Lin; João C. A. Oliveira; Alexej Scheremetjew; Lutz Ackermann
Publicado en: Journal of the American Chemical Society, Edición 5, 2024, ISSN 1943-2984
Editor: ACS
DOI: 10.1021/jacs.3c08479

Atropoenantioselective palladaelectro-catalyzed anilide C-H olefinations viable with natural sunlight as sustainable power source.

Autores: Johanna Frey; Xiaoyan Hou; Lutz Ackermann
Publicado en: Chem Sci, Edición 5, 2022, ISSN 2041-6539
Editor: Royal Society of Chemistry
DOI: 10.1039/d1sc06135f

Ruthenium(II)/Imidazolidincarbonsäure‐katalysierte C−H‐Alkylierung für zentrale und axiale Doppelenantioinduktion

Autores: Yanjun Li; Yan‐Cheng Liou; João C. A. Oliveira; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., Edición 1, 2022, ISSN 1521-3757
Editor: Wiley-VCH
DOI: 10.1002/ange.202212595

Close-Shell Reductive Elimination versus Open-Shell Radical Coupling for Site-Selective Ruthenium-Catalyzed C–H Activations by Computation and Experiments

Autores: Xinran Chen; Hasret Can Gülen; Jun Wu; Zi-Jing Zhang; Xin Hong; Lutz Ackermann
Publicado en: Angew. Chem. Int. Ed., 2023, ISSN 1521-3757
Editor: Wiley-VCH
DOI: 10.1002/anie.202302021

Enantioselectivity prediction of pallada-electrocatalysed C–H activation using transition state knowledge in machine learning

Autores: Li-Cheng Xu; Johanna Frey; Xiaoyan Hou; Shuo-Qing Zhang; Yan-Yu Li; João C. A. Oliveira; Shu-Wen Li; Lutz Ackermann; Xin Hong
Publicado en: nature synthesis, 2023, ISSN 2731-0582
Editor: Springer
DOI: 10.1038/s44160-022-00233-y

Rhodaelektro‐katalysierte peri ‐selektive direkte Alkenylierungen mit schwacher O ‐Koordination ermöglicht durch die Wasserstoffbildungsreaktion (HER)

Autores: Bartłomiej Sadowski; Binbin Yuan; Zhipeng Lin; Lutz Ackermann
Publicado en: Angew. Chem., Edición 2, 2022, ISSN 0044-8249
Editor: Wiley-VCH
DOI: 10.1002/ange.202117188

Site-selective electrochemical carboxylation of aromatic C(sp2)–H bonds with CO2

Autores: Rong Zhao; Max Surke; Zhipeng Lin; Ali Alsalme; Lutz Ackermann
Publicado en: Current Research in Green and Sustainable Chemistry, Vol 7, Iss , Pp 100377- (2023), Edición 16, 2023, ISSN 2666-0865
Editor: Elsevier
DOI: 10.1016/j.crgsc.2023.100377

Recent advances in electrooxidative radical transformations of alkynes

Autores: Yan Zhang; Zhenzhi Cai; Svenja Warratz; Chanchan Ma; Lutz Ackermann
Publicado en: Science China Chemistry, 2022, ISSN 1869-1870
Editor: Springer Nature
DOI: 10.1007/s11426-022-1438-0

Thioether-enabled palladium-catalyzed atroposelective C–H olefination for N–C and C–C axial chirality

Autores: Yanjun Li; Yan-Cheng Liou; Xinran Chen; Lutz Ackermann
Publicado en: Chem Sci, Edición 1, 2022, ISSN 2041-6539
Editor: Royal Society of Chemistry
DOI: 10.1039/d2sc00748g

Rational Design of Phe-BODIPY Amino Acids as Fluorogenic Building Blocks for Peptide-Based Detection of Urinary Tract Candida Infections

Autores: Lorena Mendive-Tapia, David Mendive-Tapia, Can Zhao, Doireann Gordon,Sam Benson,Michael J. Bromley,Wei Wang, Jun Wu, Adelina Kopp,Lutz Ackermann, and MarcVendrell
Publicado en: Angew. Chem. Int. Ed., 2022, ISSN 1521-3773
Editor: Wiley-VCH
DOI: 10.1002/anie.202117218

Sustainable Ruthenium(II)-Catalyzed C–H Activations in and on H2O

Autores: Nikolaos Kaplaneris; Marcelo Vilches-Herrera; Jun Wu; Lutz Ackermann
Publicado en: ACS Sus Chem Eng, Edición 1, 2022, ISSN 2168-0485
Editor: American Chemical Society
DOI: 10.1021/acssuschemeng.2c00873

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