Developing New 2D Materials and Heterostructures for Printed Digital Devices

Informations projet

2D-PRINTABLE

N° de convention de subvention: 101135196

DOI

10.3030/101135196

Date de signature de la CE 30 Octobre 2023

Date de début 1 Octobre 2023

Date de fin 30 Septembre 2026

Financé au titre de

• Digital, Industry and Space

Coût total

€ 4 092 496,25

Contribution de l’UE

€ 3 999 996,00

Coordonné par

THE PROVOST, FELLOWS, FOUNDATION SCHOLARS & THE OTHER MEMBERS OF BOARD, OF THE COLLEGE OF THE HOLY & UNDIVIDED TRINITY OF QUEEN ELIZABETH NEAR DUBLIN
Ireland

CORDIS fournit des liens vers les livrables publics et les publications des projets HORIZON.

Les liens vers les livrables et les publications des projets du 7e PC, ainsi que les liens vers certains types de résultats spécifiques tels que les jeux de données et les logiciels, sont récupérés dynamiquement sur OpenAIRE .

Livrables

Documents, reports (10)

Tuneable functionalization of TMDs

Via defect chemistry (e.g., with thiols or diazonium salts) and with metallic nanoparticles

Characterization of nanosheets, networks and heterostacks built from initially available 2D materials

Combination of SEM, AFM, FIB-SEM and various spectroscopies

Synthesis of bulk materials

Done in closed quartz ampoules and CVT

Electrical characterization of LPE derived novel materials

Vertical and horizontal, 2-, 3- or 4-terminal devices: extraction of µFET, Ion/Ioff, VT, SS

Characterization of new materials identified through theory

Using various standardized characterization methods, e.g., Raman, UV-vis-IR spectroscopies, AFM/TEM microscopies

Functionalization of 2D materials beyond TMDs

Use of strong electrophiles (e.g., diazoniums salts, halides, amines and maleimides) or nucleophiles (e.g., hydroxyls, amines)

Formation of discrete assemblies of 2DMs

Use of bi- or multidentate molecular linkers to form heterostructures

Ink production/printing

Controlled rheological properties

Cross-linking forming networks and heterostructures

Use of bi- or multidentate molecular linkers

Theory-identified novel 2D materials

Van der Waals DFT screening

Websites, patent fillings, videos etc. (1)

Project’s corporate identity

Communication toolbox, incl. project website, templates, newsletter, and diss. database

Data sets, microdata, etc (2)

Database on available materials

Including bulk materials, LPE/EE/CE nanosheets and their specifications (quantity, dimensions, defectiveness)

Band gaps of monolayers and multilayers

Direct/indirect band gaps computed for semiconducting monolayers and multilayers

Demonstrators, pilots, prototypes (1)

Beyond-state-of-the-art all-nanosheet TFTs

Optimization of all interfaces and components to maximize charge injection and transport. Quantification of µFET, Ion/Ioff, VT, SS

Publications

Peer reviewed articles (36)

Low-Temperature Electron Spin Resonance Study of MnPS₃ Antiferromagnetic Single Crystal

Auteurs: Moro, Fabrizio; Wu, Bing; Plutnarová, Iva; Plutnar, Jan; Sofer, Zdenek
Publié dans: The Journal of Physical Chemistry C, 2024, ISSN 1932-7455
Éditeur: American Chemical Society (ACS)
DOI: 10.1021/ACS.JPCC.4C06156

Synthesis of Xenes: physical and chemical methods

Auteurs: Molle, Alessandro; Junji, Yuhara; Yukiko, Yamada-Takamura; Sofer, Zd
Publié dans: Chemical Society Reviews, 2025, ISSN 1460-4744
Éditeur: Royal Society of Chemistry
DOI: 10.5281/ZENODO.14760360

Alkaline electrochemical deposition of Pt for alkaline electrolyzers

Auteurs: Valentina Mastronardi a , Agnese Gamberini a , Marilena Isabella Zappia a , Yong Zuo b c , Matteo Abruzzese a , Ahmad Bagheri a , Hossein Beydaghi a , Luca Gabatel a d , Sanjay Thorat a , Michele Ferri b , Filippo Drago b , Lea Pasquale e , Li
Publié dans: International Journal of Hydrogen Energy, 2024, ISSN 1879-3487
Éditeur: Elsevier Ltd
DOI: 10.1016/J.IJHYDENE.2024.07.086

Liquid-Phase Exfoliation of Arsenic Trisulfide (As2S3) Nanosheets and Their Use as Anodes in Potassium-Ion Batteries

Auteurs: KAUR, HARNEET
Publié dans: ACS nano, 2024, ISSN 1936-086X
Éditeur: American Chemical Society (ACS)
DOI: 10.1021/ACSNANO.4C03501

Ionogel-Based Electrodes for Non-Flammable High-Temperature Operating Electrochemical Double-Layer Capacitors

Auteurs: Agnese Gamberini, Tobias Burton, Alix Ladam, Ahmad Bagheri, Matteo Abruzzese, Hossein Beydaghi, Valentina Mastronardi, Elena Calcagno, Samaneh Vaez, Alberto Morenghi, Teresa Gatti, Anais Falgayrat, Francesco Bonaccorso, Sebastien Fantini, Sebastiano Bella
Publié dans: ChemSusChem, 2025, ISSN 1864-564X
Éditeur: Wiley-VCH
DOI: 10.1002/CSSC.202401874

Defect-engineering of liquid-phase exfoliated 2D semiconductors: stepwise covalent growth of electronic lateral hetero-networks

Auteurs: Antonio Gaetano Ricciardulli, Christopher E. Petoukhoff, Anna Zhuravlova, Adam G. Kelly, Chun Ma, Frédéric Laquai, Jonathan N. Coleman, Paolo Samorì
Publié dans: Materials Horizons, Numéro 11, 22, 5614-5621, 2024, ISSN 2051-6355
Éditeur: Royal Society of Chemistry
DOI: 10.1039/D4MH00882K

Molecular Connectors Boosting the Performance of MoS2 Cathodes in Zinc-Ion Batteries

Auteurs: Haipeng Guo, Verónica Montes-García, Haijun Peng, Paolo Samorì, Artur Ciesielski
Publié dans: Small, Numéro 20, 29, 2310338, 2024, ISSN 1613-6810
Éditeur: Wiley-VCH
DOI: 10.1002/SMLL.202310338

Covalent Organic Frameworks and 2D Materials Hybrids: Synthesis Strategies, Properties Enhancements, and Future Directions

Auteurs: Cataldo Valentini, Verónica Montes-García, Dawid Pakulski, Paolo Samorì, Artur Ciesielski
Publié dans: Small, Numéro 21, 8, 2410544, 2025, ISSN 1613-6810
Éditeur: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/SMLL.202410544

Piezoresistive Platinum Diselenide Pressure Sensors with Reliable High Sensitivity and Their Integration into Complementary Metal-Oxide-Semiconductor Circuits

Auteurs: Sebastian LukasNico RademacherSofía CrucesMichael GrossEva DesguéStefan HeisererNikolas DominikMaximilian PrechtlOliver HartwigCormac Ó CoileáinTanja Stimpel-LindnerPierre LegagneuxArto RantalaJuha-Matti SaariMiika SoikkeliGeorg S. DuesbergMax C. Lemme
Publié dans: ACS nano, 2025, ISSN 1936-086X
Éditeur: American Chemical Society
DOI: 10.1021/ACSNANO.4C15098

Dopant-Free Spiro-OMe2 Imidazole-Based Hole-Transporting Material for Stable and Low-Cost Organic–Inorganic Perovskite Solar Cell

Auteurs: Haji-khan Mirzaei, L., Shahroosvand, H., Farokhi, A., Bayat, E., Bellani, S., Anichini, C., Ameri, M., & Bonaccorso, F
Publié dans: ACS Omega, 2024, ISSN 2470-1343
Éditeur: American Chemical Society
DOI: 10.1021/ACSOMEGA.4C05440

High-κ Wide-Gap Layered Dielectric for Two-Dimensional van der Waals Heterostructures

Auteurs: Sofer, Zdenek
Publié dans: ACS Nano, 2024, ISSN 1936-086X
Éditeur: American Chemical Society (ACS)
DOI: 10.1021/ACSNANO.3C10411

Orientation Dependent Interlayer Coupling in Organic–Inorganic Heterostructures

Auteurs: al, StCian Bartlam, Nihit Saigefan Heiserer, Hendrik Lambers, Ursula Wurstbauer, Georg S. Duesberg
Publié dans: Advanced Functional Materials, 2024, ISSN 1616-3028
Éditeur: Wiley
DOI: 10.1002/ADFM.202315302

Covalent organic framework-based Li–S batteries: functional separators promoting Li+ transport and polysulfide trapping

Auteurs: Sara Gullace, Matteo Abruzzese, Luca Cusin, Gabriele Saleh, Sanjay B. Thorat, Agnese Gamberini, Sebastiano Bellani, Artur Ciesielski, Francesco Bonaccorso, Paolo Samorì
Publié dans: Journal of Materials Chemistry A, Numéro 12, 37, 25359-25370, 2024, ISSN 2050-7496
Éditeur: Royal Society of Chemistry
DOI: 10.1039/D4TA03930K

Dressing AgNWs with MXenes Nanosheets: Transparent Printed Electrodes Combining High-Conductivity and Tunable Work Function for High-Performance Opto-Electronics

Auteurs: Zhongshi Ju, Yusheng Chen, Peng Li, Jiangang Ma, Haiyang Xu, Yichun Liu, Paolo Samorì
Publié dans: Advanced Materials, Numéro 36, 48, 2412512, 2024, ISSN 0935-9648
Éditeur: Wiley-VCH
DOI: 10.1002/ADMA.202412512

How Biorecognition Affects the Electronic Properties of Reduced Graphene Oxide in Electrolyte-Gated Transistor Immunosensors

Auteurs: Matteo Sensi, Rafael Furlan de Oliveira, Marcello Berto, Alessandro Paradisi, Pierpaolo Greco, Carlo Augusto Bortolotti, Paolo Samorì, Fabio Biscarini
Publié dans: Advanced Functional Materials, Numéro 34, 19, 2313871, 2024, ISSN 1616-301X
Éditeur: Wiley-VCH
DOI: 10.1002/ADFM.202313871

Responsive Molecules for Organic Neuromorphic Devices: Harnessing Memory Diversification

Auteurs: Yusheng Chen, Bin Han, Marco Gobbi, Lili Hou, Paolo Samorì
Publié dans: Advanced Materials, Numéro 37, 19, 2418281, 2025, ISSN 0935-9648
Éditeur: Wiley-VCH
DOI: 10.1002/ADMA.202418281

Engineering the Interfacing of Molecules with 2D Transition Metal Dichalcogenides: Enhanced Multifunctional Electronics

Auteurs: Bin Han, Paolo Samorì
Publié dans: Accounts of Chemical Research, Numéro 57, 17, 2532–2545, 2024, ISSN 0001-4842
Éditeur: American Chemical Society
DOI: 10.1021/ACS.ACCOUNTS.4C00338

Hydrogen-Assisted Thermal Treatment of Electrode Materials for Electrochemical Double-Layer Capacitors

Auteurs: Matteo GentileSebastiano Bellani*Marilena I. ZappiaAgnese GamberiniValentina MastronardiMatteo AbruzzeseLuca GabatelLea PasqualeSergio MarrasAhmad BagheriHossein BeydaghiEvie L. PapadopoulouGuglielmo LanzaniFrancesco Bonaccorso*
Publié dans: ACS Applied Materials & Interfaces, 2024, ISSN 1944-8252
Éditeur: American Chemical Society
DOI: 10.1021/ACSAMI.3C18629

Decoding Niobium Carbide MXene Dual-Functional Photoactive Cathode in Photoenhanced Hybrid Zinc-Ion Capacitor

Auteurs: Jalal Azadmanjiri; Jakub Regner; Jiri Sturala; Zdeněk Sofer
Publié dans: ACS Materials Letters, 2024, ISSN 2639-4979
Éditeur: American Chemical Society (ACS)
DOI: 10.5281/ZENODO.12543987

Highly efficient organic–graphene hybrid photodetectors via molecular peripheral editing

Auteurs: Shuting Dai, Miao Xie, Can Wang, Yuying Wang, Bin Han, Shunqi Xu, Kexin Wang, Anna Zhuravlova, Bin Xu, Lifeng Chi, Wenjing Tian, Paolo Samorì
Publié dans: Journal of Materials Chemistry C, Numéro 12, 36, 14667-14674, 2024, ISSN 2050-7534
Éditeur: Royal Society of Chemistry
DOI: 10.1039/D4TC02010C

Exotic Photothermal Response in Ti-Based MXene Optoelectronic Devices

Auteurs: Stefano Ippolito, Francesca Urban, Paolo Samorì, Jonathan E. Spanier, Yury Gogotsi
Publié dans: Advanced Electronic Materials, Numéro 11, 13, 2500017, 2025, ISSN 2199-160X
Éditeur: Wiley-VCH
DOI: 10.1002/AELM.202500017

Interface-Tailored Secondary Excitation and Ultrafast Charge/Energy Transfer in Ti3C2Tx-MoS2 Heterostructure Films

Auteurs: Jiaxu ZhangRafael Muñoz-MármolShuai FuXiaodong LiWenhao ZhengAndrea VillaGiuseppe M. PaternòDarius PohlAlexander TahnMike HambschStefan C. B. MannsfeldDongqi LiHao XuQuanquan GuoHai I. Wang*Francesco Scotognella*Minghao Yu*Xinliang Feng*
Publié dans: Journal of the American Chemical Society, 2025, ISSN 1520-5126
Éditeur: American Chemical Society
DOI: 10.1021/JACS.5C01826

Production of Ultrathin and High-Quality Nanosheet Networks via Layer-by-Layer Assembly at Liquid–Liquid Interfaces

Auteurs: Joseph Neilson; Eoin Caffrey; Oran Cassidy; Cian Gabbett; Kevin Synnatschke; Eileen Schneider; Jose Maria Munuera; Tian Carey; Max Rimmer; Zdeněk Sofer; Janina Maultzsch; Sarah J. Haigh; Jonathan N. Coleman
Publié dans: ACS Nano, 2024, ISSN 1936-086X
Éditeur: American Chemical Society (ACS)
DOI: 10.1021/ACSNANO.4C09745

Knot Architecture for Biocompatible and Semiconducting 2D Electronic Fiber Transistors

Auteurs: Tian Carey, Jack Maughan, Luke Doolan, Eoin Caffrey, James Garcia, Shixin Liu, Harneet Kaur, Cansu Ilhan, Shayan Seyedin, Jonathan N. Coleman
Publié dans: Small methods, 2024, ISSN 2366-9608
Éditeur: Wiley-VCH
DOI: 10.1002/SMTD.202301654

Inert Liquid Exfoliation and Langmuir-Type Thin Film Deposition of Semimetallic Metal Diborides

Auteurs: Synnatschke, Kevin
Publié dans: ACS Nano, 2024, ISSN 1936-086X
Éditeur: American Chemical Society (ACS)
DOI: 10.1021/ACSNANO.4C04626

Algorithm for Reproducible Analysis of Semiconducting 2D Nanomaterials based on UV/VIS Spectroscopy

Auteurs: Backes, Claudia
Publié dans: Advanced Materials Interfaces, 2024, ISSN 2196-7350
Éditeur: Wiley
DOI: 10.1002/ADMI.202400311

Solution-Processable Electronic-Grade 2D WTe2 Enabled by Synergistic Dual Ammonium Intercalation

Auteurs: Hyejung YangKevin SynnatschkeJiho YoonHossein MirhosseiniIlka M. HermesXiaodong LiChristof NeumannAhiud MoragAndrey TurchaninThomas D. KühneStuart S. P. ParkinSheng Yang*Ali Shaygan Nia*Xinliang Feng*
Publié dans: ACS Nano, 2025, ISSN 1936-086X
Éditeur: American Chemical Society (United States)
DOI: 10.1021/ACSNANO.5C01224

Boosting Zinc Hybrid Supercapacitor Performance via Thiol Functionalization of Graphene-Based Cathodes

Auteurs: Cataldo Valentini, Verónica Montes-García, Artur Ciesielski, Paolo Samorì
Publié dans: Advanced Science, Numéro 11, 22, 2309041, 2024, ISSN 2198-3844
Éditeur: Wiley-VCH
DOI: 10.1002/ADVS.202309041

Enhanced Photothermal Conversion through 2D/0D Nano-Heterojunction Engineering for Highly Efficient Solar Desalination

Auteurs: Honglei Wang, Yifan Bo, Hongguang Wang, Malte Klingenhof, Zhehao Tao, Dong Wang, Bing Wu, Adrián Tamayo, Bin Han, Pengfei Cheng, Peter A. van Aken, Zdenek Sofer, Runfeng Chen, Peter Strasser, Peter Schaaf, Dirk M. Guldi, Paolo Samorì
Publié dans: Journal of the American Chemical Society, Numéro 147, 29, 25750-25760, 2025, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/JACS.5C07491

Nature Communications

Auteurs: Laura Gambini; Cian Gabbett; Luke Doolan; Lewys Jones; Jonathan N. Coleman; Paddy Gilligan; Stefano Sanvito
Publié dans: Nature Communications, 2024, ISSN 2041-1723
Éditeur: Nature Portfolio
DOI: 10.1038/S41467-024-52260-2

Liquid Processed Nano As₄S₄/SWCNTs Composite Electrodes for High-Performance Li-Ion and Na-Ion Battery Anodes

Auteurs: Mark McCrystall; Cian Gabbett; Harneet Kaur; Tian Carey; Jose Munera; Lee Gannon; Cormac Mc Guinness; Valeria Nicolosi; Jonathan N. Coleman; Bharathi Konkena
Publié dans: ACS Nano, 2024, ISSN 1936-086X
Éditeur: American Chemical Society (ACS)
DOI: 10.1021/ACS.ENERGYFUELS.4C03525

Light-Modulated Humidity Sensing in Spiropyran Functionalized MoS2 Transistors

Auteurs: Adrián Tamayo, Wojciech Danowski, Bin Han, Yeonsu Jeong, Paolo Samorì
Publié dans: Small, 2024, ISSN 1613-6829
Éditeur: Wiley
DOI: 10.1002/SMLL.202404633

Entropy Engineering of 2D Materials

Auteurs: Hao Mei, Yuxuan Zhang, Panpan Zhang, Antonio Gaetano Ricciardulli, Paolo Samorì, Sheng Yang
Publié dans: Advanced Science, Numéro 11, 46, 2409404, 2024, ISSN 2198-3844
Éditeur: Wiley-VCH
DOI: 10.1002/ADVS.202409404

Tailoring electrochemically exfoliated graphene electroactive pathways in cementitious composites for structural health monitoring of constructions

Auteurs: Małgorzata Safuta, Cataldo Valentini, Artur Ciesielski, Paolo Samorì
Publié dans: Nanoscale, Numéro 16, 33, 15824-15833, 2024, ISSN 2040-3372
Éditeur: Royal Society of Chemistry
DOI: 10.1039/D4NR01764A

Venice's macroalgae-derived active material for aqueous, organic, and solid-state supercapacitors

Auteurs: bonaccorso, francesco; Bagheri, Ahmad; Mastronardi, Valentina; Bellani, Sebastiano
Publié dans: Chemical Engineering Journal, 2024, ISSN 1873-3212
Éditeur: Elsevier
DOI: 10.5281/ZENODO.14960903

Graphene Nanodots as Substrates for SEIRAS and SERS Studies on Membrane Proteins

Auteurs: Ariadna Murillo-Bello, Antonio Gaetano Ricciardulli, Abdul Rehman Umar, Tatjana Gerasimova, Thorsten Friedrich, Nicolas Javahiraly, Paolo Samorì, Petra Hellwig
Publié dans: Langmuir, Numéro 41, 25, 16468–16476, 2025, ISSN 0743-7463
Éditeur: American Chemical Society
DOI: 10.1021/ACS.LANGMUIR.5C01808