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Autonomous optimisation of general conditions for novel reaction

Project description

Efficient, autonomous identification of the best reaction conditions

Discovering optimal conditions for new chemical reactions traditionally relies on slow, costly trial-and-error experimentation across a vast chemical space. With the support of the Marie Skłodowska-Curie Actions programme, the AOGCNR project aims to transform this process by integrating two powerful techniques. ‘Self-driving laboratories’ are autonomous research systems integrating AI, robotics and automated instrumentation. Large language model-enhanced Bayesian optimisation efficiently finds the best solution to complex and poorly defined problems. With these tools, AOGCNR aims to reduce over three million possible combinations in a vast chemical space by 97 % and then autonomously identify reaction conditions that perform well across multiple substrates – a significant advance over single-substrate approaches.

Objective

This proposal, AOGCNR, proposes to develop a fully autonomous, data-driven methodology for optimising general conditions for a novel organic catalysis reaction. It integrates a self-driving laboratory (SDL) with a Large Language Model (LLM)-enhanced Bayesian Optimisation framework, combining cutting-edge robotics, machine learning and expert chemical reasoning. A two-phase approach is proposed. The first phase uses a statistical pipeline to screen a vast chemical space of over 3 million combinations, reducing it by over 97% to a manageable subspace. The second phase deploys the LLM-enhanced Bayesian Optimisation algorithm within this refined space to autonomously identify general reaction conditions that perform well across multiple substrates. This approach represents a significant advancement over current methods, which typically focus on single-substrate optimisation. The methodology will be validated on both a known reaction and a novel cyclisation discovered by researchers at the University of Liverpool, demonstrating its ability to accelerate the discovery of novel catalytic reactions.

This project's impact is significant on multiple levels. It advances chemical research by enabling data-efficient exploration of complex reaction spaces. Societally, it democratises access to advanced chemistry tools. Economically, this approach offers a scalable and cost-effective alternative to traditional trial-and-error methods, streamlining industrial research and development, and contributing to more sustainable and efficient innovation.

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HORIZON-TMA-MSCA-PF-EF - HORIZON TMA MSCA Postdoctoral Fellowships - European Fellowships

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Call for proposal

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(opens in new window) HORIZON-MSCA-2025-PF

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Coordinator

THE UNIVERSITY OF LIVERPOOL
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 260 347,92
Address
BROWNLOW HILL 765 FOUNDATION BUILDING
L69 7ZX LIVERPOOL
United Kingdom

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Region
North West (England) Merseyside Liverpool
Activity type
Higher or Secondary Education Establishments
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Total cost

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