Deliverables
Dedicated project website promoting the project activities through information including the project objectives, partner backgrounds, updates on project outcome, project meetings, project public, deliverables, news items
Organisation of a workshop on AEM- and BM-based devices for electrochemical energy conversionA workshop on AEM- and BM-based devices for electrochemical energy conversion with expected audience of 80-150 participants will have taken place or will have been announced and planned at M36. A website will inform on the workshop date, place and program.
The AEI ionomers developped by TECHNION, the bipolar membranes developed from such AEI combined with proton exchange membrane (FUMA, CNRS) and possibly with an interlayer of amphoteric polymers (UNITOV) will lead to a range of novel bipolar membranes (BM). These novel BMs will be characterized ex situ in identical conditions and the most promising one(s) at M27 will be supplied to WP5 for fabrication of BMFC and BMEL with the CRM-free catalysts developped in CREATE. The demonstrator will include at least one BM for a BMEL device and one BM for a BMFC device, with conductivity and stability characterized ex situ
First generation of AEM and AEI materials for AEMFC and AEMELFirst selection of AEI and AEM synthesized within CREATE and showing sufficient conductivity and stability for being used as a first generation of materials for short-term testing the catalysts in AEMFC and AEMEL. The conductivity and stability of this first generation of AEM and AEI will have been verified ex situ before being sent to WP5.
Second generation of AEM and AEI materials for improved AEMFC and AEMEL devicessecond generation of AEI and AEM synthesized within CREATE and showing sufficient conductivity and stability for being used for testing the catalysts in AEMFC and AEMEL. The conductivity and stability of these AEM and AEI will have been verified ex situ before being sent to WP5. The second generation of AEM and AEI should moreover have reached the target set in MS1 (M20) : AEMs with alkaline stability at 60 °C > 400 h & AEI conductivity > 3 S m-1 at 100% RH
Set of CRM-free OER and HER catalyst with activity verified by RDE sent to WP5 for AEMEL testingselection of a set of catalysts free of critical raw materials for oxygen evolution reaction and hydrogen evolution reaction ; synthesis performed and activity verified with rotating disk electrode method in liquid electrolyte ; catalysts sent to WP5 for further testing in AEM electrolyzer
Set of CRM-free ORR catalyst and CRM-free or ultralow-PGM HOR catalyst with activity verified by RDE sent to WP5 for AEMFC testingselection of a set of catalysts free of critical raw materials for oxygen evolution reaction and hydrogen evolution reaction ; synthesis performed and activity verified with rotating disk electrode method in liquid electrolyte ; catalysts sent to WP5 for further testing in AEM fuel cell
The document will report on the conductivity and stability properties obtained with the optimized AEM and AEI developped during CREATE. While the full synthesis and structural characterization of these optimized materials will probably not be divulgated in this public report for IP reasons, the conductivity and stability of these optimized AEM and AEI will. These properties will have been measured ex situ and also in situ in AEMFC and/or AEMEL.
CRM-free metal@carbon materials as HER catalysts: synthesis, characterization and performance in BMELThe report will extensively describe the different metal@carbon materials prepared and electrochemically tested for the HER reaction in liquid electrolyte and, for selected catalysts, at the cathode of BMEL.
CRM-free metal oxides as OER catalysts: synthesis, characterization and performance in AEMEL & BMELThe report will extensively describe the different metal oxide materials prepared and electrochemically tested for the OER reaction in liquid electorlyte and, for selected catalysts, at the anode of AEMEL and BMEL.
CRM-free Metal-N-C materials as ORR catalysts: synthesis, characterization and performance in AEMFC & BMFCThe report will extensively describe the different Metal-N-C materials prepared and electrochemically tested for the ORR reaction in liquid electorlyte and, for selected catalysts, at the cathode of AEMFC and BMFC.
Publication on the implementation of CRM-free catalysts in polymer electrolyte EL and FCThe document will be a scientific manuscript ready for submission reporting on the challenge and possibilities with CRM-free catalysts for low temperature electrolyzers and fuel cells. While the document is intended as a review paper, specific examples and learnings acquired during CREATE will illustrate the review paper, highlighting where and how the state of art of the field could be moved forward during the project.
CRM-free metal/metal (oxy)hydroxides as HOR / HER catalysts: synthesis, characterization and performance in AEMFC & AEMELThe report will extensively describe the different metal/metal(oxy)hydroxides prepared and electrochemically tested for the HER/HOR reaction in liquid electrolyte and, for selected catalysts, at the negative electrode of AEMEL and AEMFC.
Optimized BM: synthesis, ex situ characterization and testing in BMFC and BMELThe document will report on the conductivity and stability properties obtained with the optimized BM developped during CREATE. While the full synthesis and structural characterization of these optimized BMs will probably not be divulgated in this public report for IP reasons, the conductivity and stability of these optimized BMs will. These properties will have been measured ex situ and also in situ in BMFC and BMEL.
Publications
Author(s):
Peter K. R. Holzapfel, Melanie Bühler, Daniel Escalera‐López, Markus Bierling, Florian D. Speck, Karl J. J. Mayrhofer, Serhiy Cherevko, Chuyen V. Pham, Simon Thiele
Published in:
Small, Issue 16/37, 2020, Page(s) 2003161, ISSN 1613-6810
Publisher:
Wiley - V C H Verlag GmbbH & Co.
DOI:
10.1002/smll.202003161
Author(s):
Florian D. Speck, Farhan S. M. Ali, Michael T. Y. Paul, Ramesh K. Singh, Thomas Böhm, André Hofer, Olga Kasian, Simon Thiele, Julien Bachmann, Dario R. Dekel, Tanja Kallio, Serhiy Cherevko
Published in:
Chemistry of Materials, Issue 32/18, 2020, Page(s) 7716-7724, ISSN 0897-4756
Publisher:
American Chemical Society
DOI:
10.1021/acs.chemmater.0c02048
Author(s):
Nansi Gjineci, Sinai Aharonovich, Sapir Willdorf-Cohen, Dario R. Dekel, Charles E. Diesendruck
Published in:
European Journal of Organic Chemistry, Issue 2020/21, 2020, Page(s) 3161-3168, ISSN 1434-193X
Publisher:
John Wiley & Sons Ltd.
DOI:
10.1002/ejoc.202000435
Author(s):
Ramesh K. Singh, Elena S. Davydova, John Douglin, Andres O. Godoy, Haiyan Tan, Marco Bellini, Bryan J. Allen, Jasna Jankovic, Hamish A. Miller, Ana C. Alba‐Rubio, Dario R. Dekel
Published in:
Advanced Functional Materials, Issue 30/38, 2020, Page(s) 2002087, ISSN 1616-301X
Publisher:
John Wiley & Sons Ltd.
DOI:
10.1002/adfm.202002087
Author(s):
Van Men Truong, Julian Richard Tolchard, Jørgen Svendby, Maidhily Manikandan, Hamish A. Miller, Svein Sunde, Hsiharng Yang, Dario R. Dekel, Alejandro Oyarce Barnett
Published in:
Energies, Issue 13/3, 2020, Page(s) 582, ISSN 1996-1073
Publisher:
Multidisciplinary Digital Publishing Institute (MDPI)
DOI:
10.3390/en13030582
Author(s):
I. Zadok, D. R. Dekel, S. Srebnik
Published in:
The Journal of Physical Chemistry C, Issue 123/45, 2019, Page(s) 27355-27362, ISSN 1932-7447
Publisher:
American Chemical Society
DOI:
10.1021/acs.jpcc.9b07881
Author(s):
Pietro G. Santori, Abhishek N. Mondal, Dario R. Dekel, Frédéric Jaouen
Published in:
Sustainable Energy & Fuels, Issue 4/7, 2020, Page(s) 3300-3307, ISSN 2398-4902
Publisher:
Royal Society of Chemistry
DOI:
10.1039/d0se00483a
Author(s):
Nansi Gjineci, Sinai Aharonovich, Dario R. Dekel, Charles E. Diesendruck
Published in:
ACS Applied Materials & Interfaces, Issue 12/44, 2020, Page(s) 49617-49625, ISSN 1944-8244
Publisher:
American Chemical Society
DOI:
10.1021/acsami.0c14132
Author(s):
T. Rajala, R. Kronberg, R. Backhouse, M.E.M. Buan, M. Tripathi, A. Zitolo, H. Jiang, K. Laasonen, T. Susi, F. Jaouen, T. Kallio
Published in:
Applied Catalysis B: Environmental, Issue 265, 2020, Page(s) 118582, ISSN 0926-3373
Publisher:
Elsevier BV
DOI:
10.1016/j.apcatb.2019.118582
Author(s):
Simcha Srebnik, Srdjan Pusara, Dario R. Dekel
Published in:
The Journal of Physical Chemistry C, Issue 123/26, 2019, Page(s) 15956-15962, ISSN 1932-7447
Publisher:
American Chemical Society
DOI:
10.1021/acs.jpcc.9b03131
Author(s):
Reio Praats, Maike Käärik, Arvo Kikas, Vambola Kisand, Jaan Aruväli, Päärn Paiste, Maido Merisalu, Ave Sarapuu, Jaan Leis, Väino Sammelselg, John C. Douglin, Dario R. Dekel, Kaido Tammeveski
Published in:
Journal of Solid State Electrochemistry, Issue 25/1, 2021, Page(s) 57-71, ISSN 1432-8488
Publisher:
Springer Verlag
DOI:
10.1007/s10008-020-04543-z
Author(s):
Ulrike Krewer, Christine Weinzierl, Noga Ziv, Dario R. Dekel
Published in:
Electrochimica Acta, Issue 263, 2018, Page(s) 433-446, ISSN 0013-4686
Publisher:
Pergamon Press Ltd.
DOI:
10.1016/j.electacta.2017.12.093
Author(s):
Noga Ziv, William E. Mustain, Dario R. Dekel
Published in:
ChemSusChem, Issue 11/7, 2018, Page(s) 1136-1150, ISSN 1864-5631
Publisher:
Wiley - V C H Verlag GmbbH & Co.
DOI:
10.1002/cssc.201702330
Author(s):
Yiwei Zheng, Uri Ash, Ravi P. Pandey, Amobi G. Ozioko, Julia Ponce-González, Michael Handl, Thomas Weissbach, John R. Varcoe, Steven Holdcroft, Matthew W. Liberatore, Renate Hiesgen, Dario R. Dekel
Published in:
Macromolecules, Issue 51/9, 2018, Page(s) 3264-3278, ISSN 0024-9297
Publisher:
American Chemical Society
DOI:
10.1021/acs.macromol.8b00034
Author(s):
Noga Ziv, Dario R. Dekel
Published in:
Electrochemistry Communications, Issue 88, 2018, Page(s) 109-113, ISSN 1388-2481
Publisher:
Elsevier BV
DOI:
10.1016/j.elecom.2018.01.021
Author(s):
Elena S. Davydova, Sanjeev Mukerjee, Frédéric Jaouen, Dario R. Dekel
Published in:
ACS Catalysis, Issue 8/7, 2018, Page(s) 6665-6690, ISSN 2155-5435
Publisher:
American Chemical Society
DOI:
10.1021/acscatal.8b00689
Author(s):
Charles E. Diesendruck, Dario R. Dekel
Published in:
Current Opinion in Electrochemistry, 2018, ISSN 2451-9103
Publisher:
Elsevier BV
DOI:
10.1016/j.coelec.2018.03.019
Author(s):
Dario R. Dekel, Igal G. Rasin, Miles Page, Simon Brandon
Published in:
Journal of Power Sources, Issue 375, 2018, Page(s) 191-204, ISSN 0378-7753
Publisher:
Elsevier BV
DOI:
10.1016/j.jpowsour.2017.07.012
Author(s):
Srdjan Pusara, Simcha Srebnik, Dario R. Dekel
Published in:
The Journal of Physical Chemistry C, Issue 122/21, 2018, Page(s) 11204-11213, ISSN 1932-7447
Publisher:
American Chemical Society
DOI:
10.1021/acs.jpcc.8b00752
Author(s):
Chang Hyuck Choi, Hyung-Kyu Lim, Min Wook Chung, Gajeon Chon, Nastaran Ranjbar Sahraie, Abdulrahman Altin, Moulay-Tahar Sougrati, Lorenzo Stievano, Hyun Seok Oh, Eun Soo Park, Fang Luo, Peter Strasser, Goran Dražić, Karl J. J. Mayrhofer, Hyungjun Kim, Frédéric Jaouen
Published in:
Energy & Environmental Science, 2018, ISSN 1754-5692
Publisher:
Royal Society of Chemistry
DOI:
10.1039/C8EE01855C
Author(s):
Sandip Maurya, Joseph H. Dumont, Claudia Narvaez Villarrubia, Ivana Matanovic, Dongguo Li, Yu Seung Kim, Sangtaik Noh, Junyoung Han, Chulsung Bae, Hamish A. Miller, Cy H. Fujimoto, Dario R. Dekel
Published in:
ACS Catalysis, Issue 8/10, 2018, Page(s) 9429-9439, ISSN 2155-5435
Publisher:
American Chemical Society
DOI:
10.1021/acscatal.8b03227
Author(s):
Travis J. Omasta, Xiong Peng, Hamish A. Miller, Francesco Vizza, Lianqin Wang, John R. Varcoe, Dario R. Dekel, William E. Mustain
Published in:
Journal of The Electrochemical Society, Issue 165/15, 2018, Page(s) J3039-J3044, ISSN 0013-4651
Publisher:
Electrochemical Society, Inc.
DOI:
10.1149/2.0071815jes
Author(s):
Sapir Willdorf-Cohen, Abhishek N. Mondal, Dario R. Dekel, Charles E. Diesendruck
Published in:
Journal of Materials Chemistry A, 2018, ISSN 2050-7488
Publisher:
Royal Society of Chemistry
DOI:
10.1039/C8TA05785K
Author(s):
Elena Davydova, Jérémie Zaffran, Kapil Dhaka, Maytal Toroker, Dario Dekel
Published in:
Catalysts, Issue 8/10, 2018, Page(s) 454, ISSN 2073-4344
Publisher:
Multidisciplinary Digital Publishing Institute (MDPI)
DOI:
10.3390/catal8100454
Author(s):
Emanuela Sgreccia, Luca Pasquini, Gianfranco Ercolani, Philippe Knauth, Maria Luisa Di Vona
Published in:
European Polymer Journal, Issue 112, 2019, Page(s) 255-262, ISSN 0014-3057
Publisher:
Pergamon Press Ltd.
DOI:
10.1016/j.eurpolymj.2019.01.003
Author(s):
Haoran Yu, Elena S. Davydova, Uri Ash, Hamish A. Miller, Leonard Bonville, Dario R. Dekel, Radenka Maric
Published in:
Nano Energy, Issue 57, 2019, Page(s) 820-826, ISSN 2211-2855
Publisher:
Elsevier BV
DOI:
10.1016/j.nanoen.2018.12.098
Author(s):
Dario R. Dekel, Igal G. Rasin, Simon Brandon
Published in:
Journal of Power Sources, Issue 420, 2019, Page(s) 118-123, ISSN 0378-7753
Publisher:
Elsevier BV
DOI:
10.1016/j.jpowsour.2019.02.069
Author(s):
Nejc Hodnik, Serhiy Cherevko
Published in:
Current Opinion in Electrochemistry, Issue 15, 2019, Page(s) 73-82, ISSN 2451-9103
Publisher:
Elsevier B.V
DOI:
10.1016/j.coelec.2019.03.007
Author(s):
Pietro Giovanni Santori, Florian Dominik Speck, Jingkun Li, Andrea Zitolo, Qingying Jia, Sanjeev Mukerjee, Serhiy Cherevko, Frédéric Jaouen
Published in:
Journal of The Electrochemical Society, Issue 166/7, 2019, Page(s) F3311-F3320, ISSN 0013-4651
Publisher:
Electrochemical Society, Inc.
DOI:
10.1149/2.0371907jes
Author(s):
Jingkun Li, Qingying Jia, Sanjeev Mukerjee, Moulay-Tahar Sougrati, Goran Drazic, Andrea Zitolo, Frédéric Jaouen
Published in:
Catalysts, Issue 9/2, 2019, Page(s) 144, ISSN 2073-4344
Publisher:
Multidisciplinary Digital Publishing Institute (MDPI)
DOI:
10.3390/catal9020144
Author(s):
Dario R. Dekel
Published in:
Current Opinion in Electrochemistry, Issue 12, 2018, Page(s) 182-188, ISSN 2451-9103
Publisher:
Elsevier B.V
DOI:
10.1016/j.coelec.2018.11.013
Author(s):
Jiantao Fan, Sapir Willdorf-Cohen, Eric M. Schibli, Zoe Paula, Wei Li, Thomas J. G. Skalski, Ania Tersakian Sergeenko, Amelia Hohenadel, Barbara J. Frisken, Emanuele Magliocca, William E. Mustain, Charles E. Diesendruck, Dario R. Dekel, Steven Holdcroft
Published in:
Nature Communications, Issue 10/1, 2019, ISSN 2041-1723
Publisher:
Nature Publishing Group
DOI:
10.1038/s41467-019-10292-z
Author(s):
Elena Davydova, Florian D Speck, Michael T.Y. Paul, Dario R. Dekel, Serhiy Cherevko
Published in:
ACS Catalysis, 2019, ISSN 2155-5435
Publisher:
American Chemical Society
DOI:
10.1021/acscatal.9b01582
Author(s):
Marco Bellini, Maria V. Pagliaro, Anna Lenarda, Paolo Fornasiero, Marcello Marelli, Claudio Evangelisti, Massimo Innocenti, Qingying Jia, Sanjeev Mukerjee, Jasna Jankovic, Lianqin Wang, John R. Varcoe, Chethana B. Krishnamurthy, Ilya Grinberg, Elena Davydova, Dario R. Dekel, Hamish A. Miller, Francesco Vizza
Published in:
ACS Applied Energy Materials, 2019, ISSN 2574-0962
Publisher:
American Chemical Society
DOI:
10.1021/acsaem.9b00657
Author(s):
Tamar Zelovich, Leslie Vogt-Maranto, Michael A. Hickner, Stephen J. Paddison, Chulsung Bae, Dario R. Dekel, Mark E. Tuckerman
Published in:
Chemistry of Materials, 2019, ISSN 0897-4756
Publisher:
American Chemical Society
DOI:
10.1021/acs.chemmater.9b01824
Author(s):
Felipe A. Garcés-Pineda, Marta Blasco-Ahicart, David Nieto-Castro, Núria López, José Ramón Galán-Mascarós
Published in:
Nature Energy, Issue 4/6, 2019, Page(s) 519-525, ISSN 2058-7546
Publisher:
Springer Nature
DOI:
10.1038/s41560-019-0404-4
Author(s):
Hamish A. Miller, Francesco Vizza, Marcello Marelli, Anicet Zadick, Laetitia Dubau, Marian Chatenet, Simon Geiger, Serhiy Cherevko, Huong Doan, Ryan K. Pavlicek, Sanjeev Mukerjee, Dario R. Dekel
Published in:
Nano Energy, Issue 33, 2017, Page(s) 293-305, ISSN 2211-2855
Publisher:
Elsevier BV
DOI:
10.1016/j.nanoen.2017.01.051
Author(s):
Dario R. Dekel, Michal Amar, Sapir Willdorf, Monica Kosa, Shubhendu Dhara, Charles E. Diesendruck
Published in:
Chemistry of Materials, Issue 29/10, 2017, Page(s) 4425-4431, ISSN 0897-4756
Publisher:
American Chemical Society
DOI:
10.1021/acs.chemmater.7b00958
Author(s):
Marc Ledendecker, Jared Mondschein, Olga Kasian, Simon Geiger, Daniel Göhl, Max Schalenbach, Aleksandar Zeradjanin, Serhiy Cherevko, Raymond E. Schaak, Karl Mayrhofer
Published in:
Angewandte Chemie International Edition, 2017, ISSN 1433-7851
Publisher:
John Wiley & Sons Ltd.
DOI:
10.1002/anie.201704021
Author(s):
Karam Yassin, Igal G. Rasin, Simon Brandon, Dario R. Dekel
Published in:
Journal of Membrane Science, Issue 608, 2020, Page(s) 118206, ISSN 0376-7388
Publisher:
Elsevier BV
DOI:
10.1016/j.memsci.2020.118206
Author(s):
Avital Zhegur-Khais, Fabian Kubannek, Ulrike Krewer, Dario R. Dekel
Published in:
Journal of Membrane Science, Issue 612, 2020, Page(s) 118461, ISSN 0376-7388
Publisher:
Elsevier BV
DOI:
10.1016/j.memsci.2020.118461
Author(s):
Udit N. Shrivastava, Avital Zhegur-Khais, Maria Bass, Sapir Willdorf-Cohen, Viatcheslav Freger, Dario R. Dekel, Kunal Karan
Published in:
The Journal of Physical Chemistry C, Issue 124/43, 2020, Page(s) 23469-23478, ISSN 1932-7447
Publisher:
American Chemical Society
DOI:
10.1021/acs.jpcc.0c04278
Author(s):
Riccardo Narducci, Emanuela Sgreccia, Gianfranco Ercolani, Marco Sette, Simonetta Antonaroli, Luca Pasquini, Philippe Knauth, Maria Luisa Di Vona
Published in:
European Polymer Journal, Issue 119, 2019, Page(s) 45-51, ISSN 0014-3057
Publisher:
Pergamon Press Ltd.
DOI:
10.1016/j.eurpolymj.2019.07.001
Author(s):
Noam Ralbag, Elena S. Davydova, Meirav Mann-Lahav, Peixi Cong, Jin He, Andrew M. Beale, Gideon S. Grader, David Avnir, Dario R. Dekel
Published in:
Journal of The Electrochemical Society, Issue 167/5, 2020, Page(s) 054514, ISSN 1945-7111
Publisher:
IOP publishing
DOI:
10.1149/1945-7111/ab74be
Author(s):
Olli Sorsa, Rachel Backhouse, Santeri Saxelin, Taneli Rajala, Hua Jiang, Pertti Kauranen, Tanja Kallio
Published in:
International Journal of Hydrogen Energy, Issue 45/38, 2020, Page(s) 19121-19132, ISSN 0360-3199
Publisher:
Pergamon Press Ltd.
DOI:
10.1016/j.ijhydene.2020.04.285
Author(s):
R.-A. Becerra-Arciniegas, R. Narducci, G. Ercolani, S. Antonaroli, E. Sgreccia, L. Pasquini, P. Knauth, M.L. Di Vona
Published in:
Polymer, Issue 185, 2019, Page(s) 121931, ISSN 0032-3861
Publisher:
Elsevier BV
DOI:
10.1016/j.polymer.2019.121931
Author(s):
Pietro Giovanni Santori, Florian Dominik Speck, Serhiy Cherevko, Horie Adabi Firouzjaie, Xiong Peng, William E. Mustain, Frédéric Jaouen
Published in:
Journal of The Electrochemical Society, Issue 167/13, 2020, Page(s) 134505, ISSN 1945-7111
Publisher:
IOP publishing
DOI:
10.1149/1945-7111/abb7e0
Author(s):
Florian D. Speck, Pietro G. Santori, Frédéric Jaouen, Serhiy Cherevko
Published in:
The Journal of Physical Chemistry C, Issue 123/41, 2019, Page(s) 25267-25277, ISSN 1932-7447
Publisher:
American Chemical Society
DOI:
10.1021/acs.jpcc.9b07751
Author(s):
Israel Zadok, Hai Long, Bryan Pivovar, Aleksandra Roznowska, Artur Michalak, Dario R. Dekel, Simcha Srebnik
Published in:
Journal of Molecular Liquids, Issue 313, 2020, Page(s) 113485, ISSN 0167-7322
Publisher:
Elsevier BV
DOI:
10.1016/j.molliq.2020.113485
Author(s):
Noam Ralbag, Meirav Mann-Lahav, Elena S. Davydova, Uri Ash, Reuven Galed, Michael Handl, Renate Hiesgen, Emanuele Magliocca, William Mustain, Jin He, Peixi Cong, Andrew M. Beale, Gideon S. Grader, David Avnir, Dario R. Dekel
Published in:
Matter, Issue 1/4, 2019, Page(s) 959-975, ISSN 2590-2385
Publisher:
Elsevier
DOI:
10.1016/j.matt.2019.04.007
Intellectual Property Rights
Application/Publication number:
FI
20185970
Date:
2018-11-16
Application/Publication number:
FI
20185970
Date:
2018-11-16
Applicant(s):
AALTO KORKEAKOULUSAATIO SR
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