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Coherent Optical Parallel Computing

Deliverables

Best procedures of functionalization/assembly

Final report on best procedure for functionalization and assembly suitable for WP3 and WP4. (M42 P4, P2-YP, P3, P5, P7)

Surface functionalization procedures

Report on surface functionalization procedures (M20, P4, P2-YP)

Applied theory of computing by observables

Applied theory of computing by observables and long time stability (M36, P2-RL, P1, P3-BF, P6).

Design and modelling of prototype

Report on prototype modelling and design (M12, P5,P7, P4, P2-YP,P3-EC,P1, P2-RDL)

Technological roadmap

Technological roadmap (M42, P7).

Demonstration of parallel logic

Demonstration of parallel logic for distinct units operating in parallel (M24), on arrays (M42) in a single and in several phase matching directions (P3-BF with P1, P2-RL).

QD and core-shell nanostructure synthesis

Report on procedures for the synthesis of QDs and core-shell with defined optical properties (M12, P4)

Layered structures with high delocalization

Fabricating a layered structure exhibiting nearest neighbor electronic delocalization at ambient conditions. (M24, P2-YP, P4)

Multiscale modelling and model Hamiltonians

Multiscale modelling and model Hamiltonians of organic dyes (M12) and arrays SC- QDs (M24) for feedback to WPs2&3, and for guiding data interpretation in WP3 (P1, P2-RL, P3-BF).

All PM directions optical response simulations

Simulation of the optical response in all phase matching directions of dyes (M18), arrays of SC- QDs (M36), and comparison with experimental spectra of P3-EC, in the perturbative limit (P3-BF) and to higher orders (P1, P2-RL).

Scientific and Technical progress Report

Scientific and Technical progress Report

Theory of compiler targeting PMVL machines and virtual experiments

Report on the theory of compiler targeting PLMV machine (M18) and virtual experiment (M30) P6, P1, P2-RL How PLMV functions could be use as instruction set and how they could be used to implement compound operations.

Complete set of 2D data on multichromophoric systems and on arrays

Complete set of 2D data on multi-chromophoric systems (networks of nanosystems) in solution (M30, P3-EC) and embedded in solid state matrices to characterized the inter unit coupling dynamics. (M24, P3-EC)

Compiler targeting realistic PMVL machines

Compiler targeting realistic PMLV machine A software simulator of feasible machine and compilers targeting this machine will be provided as well as program examples (M36, P6, P1, P2-RL).

Complete set of 2D data on solutions

Complete set of 2D data on solutions of organic dyes, SC-QD and dimers thereof to establish a correspondence between experimental results and logic operations. (M12, P3-EC).

System design

Report of system design (M42, P7, all)

Multiphase matching experiment data set on complex systems

Multi-phase matching experiment dataset on complex systems (M42, P3-EC) and implications to logic synthesis and architecture and device integration.

Dissemination and Exploitation plan

Dissemination and Exploitation plan (M12, P6)

Website

COPAC project website (restricted (P1) and public (P6), regularly updated) and a logo.

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Publications

Coupling effects in QD dimers at sub-nanometer interparticle distance

Author(s): Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Rosaria Brescia, Yuval Kolodny, Sergei Remennik, Annamaria Panniello, Nicoletta Depalo, Shira Yochelis, Roberto Comparelli, Angela Agostiano, Maria Lucia Curri, Yossi Paltiel, Marinella Striccoli
Published in: Nano Research, 13/4, 2020, Page(s) 1071-1080, ISSN 1998-0124
Publisher: Tsinghua Univ Press
DOI: 10.1007/s12274-020-2747-3

Tuning Quantum Dots Coupling Using Organic Linkers with Different Vibrational Modes

Author(s): Yuval Kolodny, Stav Fererra, Veniamin Borin, Shira Yochelis, Carlo Nazareno Dibenedetto, Morin Mor, Joanna Dehnel, Sergei Remmenik, Elisabetta Fanizza, Marinella Striccoli, Igor Schapiro, Efrat Lifshitz, Yossi Paltiel
Published in: The Journal of Physical Chemistry C, 124/29, 2020, Page(s) 16159-16165, ISSN 1932-7447
Publisher: American Chemical Society
DOI: 10.1021/acs.jpcc.0c03703

Massively parallel classical logic via coherent dynamics of an ensemble of quantum systems with dispersion in size.

Author(s): Hugo Gattuso; Raphael D. Levine; Raphael D. Levine; Françoise Remacle; Françoise Remacle
Published in: Proc Natl Acad Sci U S A, 4, 2020, ISSN 1091-6490
Publisher: National Academy of Science
DOI: 10.26434/chemrxiv.12370538.v1

Quantum Device Emulates the Dynamics of Two Coupled Oscillators

Author(s): Ksenia Komarova, Hugo Gattuso, R. D. Levine, F. Remacle
Published in: The Journal of Physical Chemistry Letters, 11/17, 2020, Page(s) 6990-6995, ISSN 1948-7185
Publisher: American Chemical Society
DOI: 10.1021/acs.jpclett.0c01880

Chirality of a rhodamine heterodimer linked to a DNA scaffold: an experimental and computational study

Author(s): P. S. Rukin, K. G. Komarova, B. Fresch, E. Collini, F. Remacle
Published in: Physical Chemistry Chemical Physics, 22/14, 2020, Page(s) 7516-7523, ISSN 1463-9076
Publisher: Royal Society of Chemistry
DOI: 10.1039/d0cp00223b

Quantum Phenomena in Nanomaterials: Coherent Superpositions of Fine Structure States in CdSe Nanocrystals at Room Temperature

Author(s): Elisabetta Collini, Hugo Gattuso, Luca Bolzonello, Andrea Casotto, Andrea Volpato, Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Marinella Striccoli, Françoise Remacle
Published in: The Journal of Physical Chemistry C, 123/51, 2019, Page(s) 31286-31293, ISSN 1932-7447
Publisher: American Chemical Society
DOI: 10.1021/acs.jpcc.9b11153

Time resolved mechanism of the isotope selectivity in the ultrafast light induced dissociation in N 2

Author(s): Ksenia G. Komarova, Francoise Remacle, R. D. Levine
Published in: The Journal of Chemical Physics, 151/11, 2019, Page(s) 114308, ISSN 0021-9606
Publisher: American Institute of Physics
DOI: 10.1063/1.5118990

Photocurrent-Detected 2D Electronic Spectroscopy Reveals Ultrafast Hole Transfer in Operating PM6/Y6 Organic Solar Cells

Author(s): Luca Bolzonello, Francisco Bernal-Texca, Luis G. Gerling, Jana Ockova, Elisabetta Collini, Jordi Martorell, Niek F. van Hulst
Published in: The Journal of Physical Chemistry Letters, 12/16, 2021, Page(s) 3983-3988, ISSN 1948-7185
Publisher: American Chemical Society
DOI: 10.1021/acs.jpclett.1c00822

Parallel Quantum Computation of Vibrational Dynamics

Author(s): Ksenia Komarova; Hugo Gattuso; R. D. Levine; R. D. Levine; R. D. Levine; F. Remacle; F. Remacle
Published in: Frontiers in Physcis, 4, 2020, ISSN 2296-424X
Publisher: Frontiers
DOI: 10.26434/chemrxiv.12814793

Room-Temperature Inter-Dot Coherent Dynamics in Multilayer Quantum Dot Materials

Author(s): Elisabetta Collini, Hugo Gattuso, Yuval Kolodny, Luca Bolzonello, Andrea Volpato, Hanna T. Fridman, Shira Yochelis, Morin Mor, Johanna Dehnel, Efrat Lifshitz, Yossi Paltiel, Raphael D. Levine, Françoise Remacle
Published in: The Journal of Physical Chemistry C, 124/29, 2020, Page(s) 16222-16231, ISSN 1932-7447
Publisher: American Chemical Society
DOI: 10.1021/acs.jpcc.0c05572

Coherent Exciton Dynamics in Ensembles of Size-Dispersed CdSe Quantum Dot Dimers Probed via Ultrafast Spectroscopy: A Quantum Computational Study

Author(s): Hugo Gattuso, Barbara Fresch, Raphael D. Levine, Françoise Remacle
Published in: Applied Sciences, 10/4, 2020, Page(s) 1328, ISSN 2076-3417
Publisher: mdpi
DOI: 10.3390/app10041328

Spectral shift, electronic coupling and exciton delocalization in nanocrystal dimers: insights from all-atom electronic structure computations

Author(s): Maurizio Coden, Pietro De Checchi, Barbara Fresch
Published in: Nanoscale, 12/35, 2020, Page(s) 18124-18136, ISSN 2040-3364
Publisher: Royal Society of Chemistry
DOI: 10.1039/d0nr05601d

Deciphering hot- and multi-exciton dynamics in core–shell QDs by 2D electronic spectroscopies

Author(s): Marcello Righetto, Luca Bolzonello, Andrea Volpato, Giordano Amoruso, Annamaria Panniello, Elisabetta Fanizza, Marinella Striccoli, Elisabetta Collini
Published in: Physical Chemistry Chemical Physics, 20/27, 2018, Page(s) 18176-18183, ISSN 1463-9076
Publisher: Royal Society of Chemistry
DOI: 10.1039/c8cp02574f

Optimization and selection of time-frequency transforms for wave-packet analysis in ultrafast spectroscopy

Author(s): Andrea Volpato, Elisabetta Collini
Published in: Optics Express, 27/3, 2019, Page(s) 2975, ISSN 1094-4087
Publisher: Optical Society of America
DOI: 10.1364/OE.27.002975

Characterization of the coherent dynamics of bacteriochlorophyll a in solution

Author(s): Elena Meneghin, Danilo Pedron, Elisabetta Collini
Published in: Chemical Physics, 519, 2019, Page(s) 85-91, ISSN 0301-0104
Publisher: Elsevier BV
DOI: 10.1016/j.chemphys.2018.12.008

Spectroscopy data for the time and frequency characterization of vibrational coherences in bacteriochlorophyll a

Author(s): Elena Meneghin, Danilo Pedron, Elisabetta Collini
Published in: Data in Brief, 23, 2019, Page(s) 103707, ISSN 2352-3409
Publisher: Elsevier BV
DOI: 10.1016/j.dib.2019.103707

Effect of Different Conformational Distributions on the Ultrafast Coherence Dynamics in Porphyrin-Based Polymers

Author(s): Andrea Volpato, Mirco Zerbetto, Luca Bolzonello, Elena Meneghin, Barbara Fresch, Tiziana Benelli, Loris Giorgini, Elisabetta Collini
Published in: The Journal of Physical Chemistry C, 123/16, 2019, Page(s) 10212-10224, ISSN 1932-7447
Publisher: American Chemical Society
DOI: 10.1021/acs.jpcc.8b12562

Fast Energy Transfer in CdSe Quantum Dot Layered Structures: Controlling Coupling with Covalent-Bond Organic Linkers

Author(s): Eyal Cohen, Pavel Komm, Noa Rosenthal-Strauss, Joanna Dehnel, Efrat Lifshitz, Shira Yochelis, Raphael D. Levine, Francoise Remacle, Barbara Fresch, Gilad Marcus, Yossi Paltiel
Published in: The Journal of Physical Chemistry C, 122/10, 2018, Page(s) 5753-5758, ISSN 1932-7447
Publisher: American Chemical Society
DOI: 10.1021/acs.jpcc.7b11799

Spin-Exciton Delocalization Enhancement in Multilayer Chiral Linker/Quantum Dot Structures

Author(s): Hanna T. Fridman, Johanna Dehnel, Shira Yochelis, Efrat Lifshitz, Yossi Paltiel
Published in: The Journal of Physical Chemistry Letters, 10/14, 2019, Page(s) 3858-3862, ISSN 1948-7185
Publisher: American Chemical Society
DOI: 10.1021/acs.jpclett.9b01433

Quantum Dot Coupling in a Vertical Transport Device under Ambient Conditions

Author(s): Aviya Perlman Illouz, Eyal Cohen, Uri Peskin, Shira Yochelis, Yossi Paltiel
Published in: ACS Omega, 3/6, 2018, Page(s) 6224-6229, ISSN 2470-1343
Publisher: ACS
DOI: 10.1021/acsomega.8b00867

Coupling in quantum dot molecular hetero-assemblies

Author(s): Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Liberato De Caro, Rosaria Brescia, Annamaria Panniello, Raffaele Tommasi, Chiara Ingrosso, Cinzia Giannini, Angela Agostiano, Maria Lucia Curri, Marinella Striccoli
Published in: Materials Research Bulletin, 146, 2022, Page(s) 111578, ISSN 0025-5408
Publisher: Pergamon Press Ltd.
DOI: 10.1016/j.materresbull.2021.111578

Ultrafast fs coherent excitonic dynamics in CdSe quantum dots assemblies addressed and probed by 2D electronic spectroscopy

Author(s): Elisabetta Collini, Hugo Gattuso, R. D. Levine, F. Remacle
Published in: The Journal of Chemical Physics, 154/1, 2021, Page(s) 014301, ISSN 0021-9606
Publisher: American Institute of Physics
DOI: 10.1063/5.0031420

Surprisal of a Quantum State: Dynamics, Compact Representation and Coherence Effects

Author(s): K. Komarova; F. Remacle; R. D. Levine
Published in: Surprisal of a quantum state: Dynamics, compact representation, and coherence effects. <i>The Journal of Chemical Physics, 153</i>(21), 214105. (2020)., 4, 2020, ISSN 0021-9606
Publisher: American Institute of Physics
DOI: 10.26434/chemrxiv.12981857.v1

Lasers pumped quantum dynamics in nanostructured arrays for computing

Author(s): Ariela Donval, Noam Gross, Moshe Oron
Published in: Quantum Information Science, Sensing, and Computation X, 2018, Page(s) 4, ISBN 9781-510618329
Publisher: SPIE
DOI: 10.1117/12.2299961

Computing using quantum dynamics of nanostructured arrays

Author(s): Noam Gross, Ariela Donval
Published in: Quantum Information Science, Sensing, and Computation XI, 2019, Page(s) 2, ISBN 9781-510626348
Publisher: SPIE
DOI: 10.1117/12.2518299

An n-bit adder realized via coherent optical parallel computing

Author(s): Bogdan Reznychenko, Emmanuel Mazer, Maurizio Coden, Elisabetta Collini, Carlo Nazareno DiBenedetto, Ariela Donval, Barbara Fresch, Hugo Gattuso, Noam Gross, Yossi Paltiel, Francoise Remacle, Marinella Striccoli
Published in: 2019 IEEE International Conference on Rebooting Computing (ICRC), 2019, Page(s) 146-152, ISBN 978-1-7281-5221-9
Publisher: IEEE eXpress Conference Publishing