Risultati finali Documents, reports (18) Best procedures of functionalization/assembly Final report on best procedure for functionalization and assembly suitable for WP3 and WP4. (M42 P4, P2-YP, P3, P5, P7) Surface functionalization procedures Report on surface functionalization procedures (M20, P4, P2-YP) Applied theory of computing by observables Applied theory of computing by observables and long time stability (M36, P2-RL, P1, P3-BF, P6). Design and modelling of prototype Report on prototype modelling and design (M12, P5,P7, P4, P2-YP,P3-EC,P1, P2-RDL) Technological roadmap Technological roadmap (M42, P7). Demonstration of parallel logic Demonstration of parallel logic for distinct units operating in parallel (M24), on arrays (M42) in a single and in several phase matching directions (P3-BF with P1, P2-RL). QD and core-shell nanostructure synthesis Report on procedures for the synthesis of QDs and core-shell with defined optical properties (M12, P4) Layered structures with high delocalization Fabricating a layered structure exhibiting nearest neighbor electronic delocalization at ambient conditions. (M24, P2-YP, P4) Multiscale modelling and model Hamiltonians Multiscale modelling and model Hamiltonians of organic dyes (M12) and arrays SC- QDs (M24) for feedback to WPs2&3, and for guiding data interpretation in WP3 (P1, P2-RL, P3-BF). All PM directions optical response simulations Simulation of the optical response in all phase matching directions of dyes (M18), arrays of SC- QDs (M36), and comparison with experimental spectra of P3-EC, in the perturbative limit (P3-BF) and to higher orders (P1, P2-RL). Scientific and Technical progress Report Scientific and Technical progress Report Theory of compiler targeting PMVL machines and virtual experiments Report on the theory of compiler targeting PLMV machine (M18) and virtual experiment (M30) P6, P1, P2-RL How PLMV functions could be use as instruction set and how they could be used to implement compound operations. Complete set of 2D data on multichromophoric systems and on arrays Complete set of 2D data on multi-chromophoric systems (networks of nanosystems) in solution (M30, P3-EC) and embedded in solid state matrices to characterized the inter unit coupling dynamics. (M24, P3-EC) Compiler targeting realistic PMVL machines Compiler targeting realistic PMLV machine A software simulator of feasible machine and compilers targeting this machine will be provided as well as program examples (M36, P6, P1, P2-RL). Complete set of 2D data on solutions Complete set of 2D data on solutions of organic dyes, SC-QD and dimers thereof to establish a correspondence between experimental results and logic operations. (M12, P3-EC). System design Report of system design (M42, P7, all) Multiphase matching experiment data set on complex systems Multi-phase matching experiment dataset on complex systems (M42, P3-EC) and implications to logic synthesis and architecture and device integration. Dissemination and Exploitation plan Dissemination and Exploitation plan (M12, P6) Websites, patent fillings, videos etc. (1) Website COPAC project website (restricted (P1) and public (P6), regularly updated) and a logo. Open Research Data Pilot (1) Data management plan Data Management plan, (M6, P1) Pubblicazioni Peer reviewed articles (23) Coupling effects in QD dimers at sub-nanometer interparticle distance Autori: Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Rosaria Brescia, Yuval Kolodny, Sergei Remennik, Annamaria Panniello, Nicoletta Depalo, Shira Yochelis, Roberto Comparelli, Angela Agostiano, Maria Lucia Curri, Yossi Paltiel, Marinella Striccoli Pubblicato in: Nano Research, Issue 13/4, 2020, Page(s) 1071-1080, ISSN 1998-0124 Editore: Tsinghua Univ Press DOI: 10.1007/s12274-020-2747-3 Tuning Quantum Dots Coupling Using Organic Linkers with Different Vibrational Modes Autori: Yuval Kolodny, Stav Fererra, Veniamin Borin, Shira Yochelis, Carlo Nazareno Dibenedetto, Morin Mor, Joanna Dehnel, Sergei Remmenik, Elisabetta Fanizza, Marinella Striccoli, Igor Schapiro, Efrat Lifshitz, Yossi Paltiel Pubblicato in: The Journal of Physical Chemistry C, Issue 124/29, 2020, Page(s) 16159-16165, ISSN 1932-7447 Editore: American Chemical Society DOI: 10.1021/acs.jpcc.0c03703 Massively parallel classical logic via coherent dynamics of an ensemble of quantum systems with dispersion in size. Autori: Hugo Gattuso; Raphael D. Levine; Raphael D. Levine; Françoise Remacle; Françoise Remacle Pubblicato in: Proc Natl Acad Sci U S A, Issue 4, 2020, ISSN 1091-6490 Editore: National Academy of Science DOI: 10.26434/chemrxiv.12370538.v1 Quantum Device Emulates the Dynamics of Two Coupled Oscillators Autori: Ksenia Komarova, Hugo Gattuso, R. D. Levine, F. Remacle Pubblicato in: The Journal of Physical Chemistry Letters, Issue 11/17, 2020, Page(s) 6990-6995, ISSN 1948-7185 Editore: American Chemical Society DOI: 10.1021/acs.jpclett.0c01880 Chirality of a rhodamine heterodimer linked to a DNA scaffold: an experimental and computational study Autori: P. S. Rukin, K. G. Komarova, B. Fresch, E. Collini, F. Remacle Pubblicato in: Physical Chemistry Chemical Physics, Issue 22/14, 2020, Page(s) 7516-7523, ISSN 1463-9076 Editore: Royal Society of Chemistry DOI: 10.1039/d0cp00223b Quantum Phenomena in Nanomaterials: Coherent Superpositions of Fine Structure States in CdSe Nanocrystals at Room Temperature Autori: Elisabetta Collini, Hugo Gattuso, Luca Bolzonello, Andrea Casotto, Andrea Volpato, Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Marinella Striccoli, Françoise Remacle Pubblicato in: The Journal of Physical Chemistry C, Issue 123/51, 2019, Page(s) 31286-31293, ISSN 1932-7447 Editore: American Chemical Society DOI: 10.1021/acs.jpcc.9b11153 Time resolved mechanism of the isotope selectivity in the ultrafast light induced dissociation in N 2 Autori: Ksenia G. Komarova, Francoise Remacle, R. D. Levine Pubblicato in: The Journal of Chemical Physics, Issue 151/11, 2019, Page(s) 114308, ISSN 0021-9606 Editore: American Institute of Physics DOI: 10.1063/1.5118990 Photocurrent-Detected 2D Electronic Spectroscopy Reveals Ultrafast Hole Transfer in Operating PM6/Y6 Organic Solar Cells Autori: Luca Bolzonello, Francisco Bernal-Texca, Luis G. Gerling, Jana Ockova, Elisabetta Collini, Jordi Martorell, Niek F. van Hulst Pubblicato in: The Journal of Physical Chemistry Letters, Issue 12/16, 2021, Page(s) 3983-3988, ISSN 1948-7185 Editore: American Chemical Society DOI: 10.1021/acs.jpclett.1c00822 Parallel Quantum Computation of Vibrational Dynamics Autori: Ksenia Komarova; Hugo Gattuso; R. D. Levine; R. D. Levine; R. D. Levine; F. Remacle; F. Remacle Pubblicato in: Frontiers in Physcis, Issue 4, 2020, ISSN 2296-424X Editore: Frontiers DOI: 10.26434/chemrxiv.12814793 Room-Temperature Inter-Dot Coherent Dynamics in Multilayer Quantum Dot Materials Autori: Elisabetta Collini, Hugo Gattuso, Yuval Kolodny, Luca Bolzonello, Andrea Volpato, Hanna T. Fridman, Shira Yochelis, Morin Mor, Johanna Dehnel, Efrat Lifshitz, Yossi Paltiel, Raphael D. Levine, Françoise Remacle Pubblicato in: The Journal of Physical Chemistry C, Issue 124/29, 2020, Page(s) 16222-16231, ISSN 1932-7447 Editore: American Chemical Society DOI: 10.1021/acs.jpcc.0c05572 Coherent Exciton Dynamics in Ensembles of Size-Dispersed CdSe Quantum Dot Dimers Probed via Ultrafast Spectroscopy: A Quantum Computational Study Autori: Hugo Gattuso, Barbara Fresch, Raphael D. Levine, Françoise Remacle Pubblicato in: Applied Sciences, Issue 10/4, 2020, Page(s) 1328, ISSN 2076-3417 Editore: mdpi DOI: 10.3390/app10041328 Spectral shift, electronic coupling and exciton delocalization in nanocrystal dimers: insights from all-atom electronic structure computations Autori: Maurizio Coden, Pietro De Checchi, Barbara Fresch Pubblicato in: Nanoscale, Issue 12/35, 2020, Page(s) 18124-18136, ISSN 2040-3364 Editore: Royal Society of Chemistry DOI: 10.1039/d0nr05601d Deciphering hot- and multi-exciton dynamics in core–shell QDs by 2D electronic spectroscopies Autori: Marcello Righetto, Luca Bolzonello, Andrea Volpato, Giordano Amoruso, Annamaria Panniello, Elisabetta Fanizza, Marinella Striccoli, Elisabetta Collini Pubblicato in: Physical Chemistry Chemical Physics, Issue 20/27, 2018, Page(s) 18176-18183, ISSN 1463-9076 Editore: Royal Society of Chemistry DOI: 10.1039/c8cp02574f Optimization and selection of time-frequency transforms for wave-packet analysis in ultrafast spectroscopy Autori: Andrea Volpato, Elisabetta Collini Pubblicato in: Optics Express, Issue 27/3, 2019, Page(s) 2975, ISSN 1094-4087 Editore: Optical Society of America DOI: 10.1364/OE.27.002975 Characterization of the coherent dynamics of bacteriochlorophyll a in solution Autori: Elena Meneghin, Danilo Pedron, Elisabetta Collini Pubblicato in: Chemical Physics, Issue 519, 2019, Page(s) 85-91, ISSN 0301-0104 Editore: Elsevier BV DOI: 10.1016/j.chemphys.2018.12.008 Spectroscopy data for the time and frequency characterization of vibrational coherences in bacteriochlorophyll a Autori: Elena Meneghin, Danilo Pedron, Elisabetta Collini Pubblicato in: Data in Brief, Issue 23, 2019, Page(s) 103707, ISSN 2352-3409 Editore: Elsevier BV DOI: 10.1016/j.dib.2019.103707 Effect of Different Conformational Distributions on the Ultrafast Coherence Dynamics in Porphyrin-Based Polymers Autori: Andrea Volpato, Mirco Zerbetto, Luca Bolzonello, Elena Meneghin, Barbara Fresch, Tiziana Benelli, Loris Giorgini, Elisabetta Collini Pubblicato in: The Journal of Physical Chemistry C, Issue 123/16, 2019, Page(s) 10212-10224, ISSN 1932-7447 Editore: American Chemical Society DOI: 10.1021/acs.jpcc.8b12562 Fast Energy Transfer in CdSe Quantum Dot Layered Structures: Controlling Coupling with Covalent-Bond Organic Linkers Autori: Eyal Cohen, Pavel Komm, Noa Rosenthal-Strauss, Joanna Dehnel, Efrat Lifshitz, Shira Yochelis, Raphael D. Levine, Francoise Remacle, Barbara Fresch, Gilad Marcus, Yossi Paltiel Pubblicato in: The Journal of Physical Chemistry C, Issue 122/10, 2018, Page(s) 5753-5758, ISSN 1932-7447 Editore: American Chemical Society DOI: 10.1021/acs.jpcc.7b11799 Spin-Exciton Delocalization Enhancement in Multilayer Chiral Linker/Quantum Dot Structures Autori: Hanna T. Fridman, Johanna Dehnel, Shira Yochelis, Efrat Lifshitz, Yossi Paltiel Pubblicato in: The Journal of Physical Chemistry Letters, Issue 10/14, 2019, Page(s) 3858-3862, ISSN 1948-7185 Editore: American Chemical Society DOI: 10.1021/acs.jpclett.9b01433 Quantum Dot Coupling in a Vertical Transport Device under Ambient Conditions Autori: Aviya Perlman Illouz, Eyal Cohen, Uri Peskin, Shira Yochelis, Yossi Paltiel Pubblicato in: ACS Omega, Issue 3/6, 2018, Page(s) 6224-6229, ISSN 2470-1343 Editore: ACS DOI: 10.1021/acsomega.8b00867 Coupling in quantum dot molecular hetero-assemblies Autori: Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Liberato De Caro, Rosaria Brescia, Annamaria Panniello, Raffaele Tommasi, Chiara Ingrosso, Cinzia Giannini, Angela Agostiano, Maria Lucia Curri, Marinella Striccoli Pubblicato in: Materials Research Bulletin, Issue 146, 2022, Page(s) 111578, ISSN 0025-5408 Editore: Pergamon Press Ltd. DOI: 10.1016/j.materresbull.2021.111578 Ultrafast fs coherent excitonic dynamics in CdSe quantum dots assemblies addressed and probed by 2D electronic spectroscopy Autori: Elisabetta Collini, Hugo Gattuso, R. D. Levine, F. Remacle Pubblicato in: The Journal of Chemical Physics, Issue 154/1, 2021, Page(s) 014301, ISSN 0021-9606 Editore: American Institute of Physics DOI: 10.1063/5.0031420 Surprisal of a Quantum State: Dynamics, Compact Representation and Coherence Effects Autori: K. Komarova; F. Remacle; R. D. Levine Pubblicato in: Surprisal of a quantum state: Dynamics, compact representation, and coherence effects. <i>The Journal of Chemical Physics, 153</i>(21), 214105. (2020)., Issue 4, 2020, ISSN 0021-9606 Editore: American Institute of Physics DOI: 10.26434/chemrxiv.12981857.v1 Conference proceedings (3) Lasers pumped quantum dynamics in nanostructured arrays for computing Autori: Ariela Donval, Noam Gross, Moshe Oron Pubblicato in: Quantum Information Science, Sensing, and Computation X, 2018, Page(s) 4, ISBN 9781-510618329 Editore: SPIE DOI: 10.1117/12.2299961 Computing using quantum dynamics of nanostructured arrays Autori: Noam Gross, Ariela Donval Pubblicato in: Quantum Information Science, Sensing, and Computation XI, 2019, Page(s) 2, ISBN 9781-510626348 Editore: SPIE DOI: 10.1117/12.2518299 An n-bit adder realized via coherent optical parallel computing Autori: Bogdan Reznychenko, Emmanuel Mazer, Maurizio Coden, Elisabetta Collini, Carlo Nazareno DiBenedetto, Ariela Donval, Barbara Fresch, Hugo Gattuso, Noam Gross, Yossi Paltiel, Francoise Remacle, Marinella Striccoli Pubblicato in: 2019 IEEE International Conference on Rebooting Computing (ICRC), 2019, Page(s) 146-152, ISBN 978-1-7281-5221-9 Editore: IEEE eXpress Conference Publishing È in corso la ricerca di dati su OpenAIRE... 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